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arXiv:2210.13241 · New Journal of Physics

Initial correlations in open quantum systems: constructing linear dynamical maps and master equations

Alessandra Colla, Niklas Neubrand, Heinz‐Peter Breuer

Published Nov 30, 2022• 22 citations
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Abstract

Abstract We investigate the dynamics of open quantum systems which are initially correlated with their environment. The strategy of our approach is to analyze how given, fixed initial correlations modify the evolution of the open system with respect to the corresponding uncorrelated dynamical behavior with the same fixed initial environmental state, described by a completely positive dynamical map. We show that, for any predetermined initial correlations, one can introduce a linear dynamical map on the space of operators of the open system which acts like the proper dynamical map on the set of physical states and represents its unique linear extension. Furthermore, we demonstrate that this construction leads to a linear, time-local quantum master equation with generalized Lindblad structure involving time-dependent, possibly negative transition rates. Thus, the general non-Markovian dynamics of an open quantum system can be described by means of a time-local master equation even in the case of arbitrary, fixed initial system–environment correlations. We present some illustrative examples and explain the relation of our approach to several other approaches proposed in the literature.

DOI
10.1088/1367-2630/aca709

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Abstract We investigate the dynamics of open quantum systems which are initially correlated with their environment. The strategy of our approach is to analyze how given, fixed initial correlations modify the evolution of the open system with respect to the corresponding uncorrelated dynamical behavior with the same fixed initial environmental state, described by a completely positive dynamical map. We show that, for any predetermined initial correlations, one can introduce a linear dynamical map on the space of operators of the open system which acts like the proper dynamical map on the set of physical states and represents its unique linear extension. Furthermore, we demonstrate that this construction leads to a linear, time-local quantum master equation with generalized Lindblad structure involving time-dependent, possibly negative transition rates. Thus, the general non-Markovian dynamics of an open quantum system can be described by means of a time-local master equation even in the case of arbitrary, fixed initial system–environment correlations. We present some illustrative examples and explain the relation of our approach to several other approaches proposed in the literature.
We study the role of correlations with the environment as the source of non-Markovian quantum evolutions. We first focus on the impact that correlations with the environment can have on the dynamical map that evolve the system. We expand the set of initial states of a system and its environment that are known to guarantee completely positive reduced dynamics for the system when the combined state evolves unitarily. We characterize the correlations in the initial state in terms of its quantum discord. The induced maps can be not completely positive when quantum correlations including, but not limited to, entanglement are present. We discuss the implications and limitations of the Markov approximation necessary to derive the Kossakowski-Lindblad master equation. A generalized non-Markovian master equation is derived from the dynamical map of systems correlated with their environment. The physical meaning of not completely positive maps is studied to obtain a consistent theory of non-Markovian quantum dynamics. These are associated to inverse maps necessary to establish correlations and they give rise to a canonical embedding map that is local in time. This master equation goes beyond the Kossakowski-Lindblad master equation. Non-equilibrium quantum thermodynamics can be be studied within this theory. Through out this discussion, the general dynamics of two interacting qubits is used as an example for illustrations.
We show that the dynamics of any open quantum system that is initially correlated with its environment can be described by a set of d2{d}^{2}d2 (or less) completely positive maps, where ddd is the dimension of the system. Only one such map is required for the special case of no initial correlations. The same maps describe the dynamics of any system-environment state obtained from the initial state by a local operation on the system. The reduction of the system dynamics to a set of completely positive maps allows known numerical and analytic tools for uncorrelated initial states to be applied to the general case of initially correlated states, which we exemplify by solving the qubit dephasing model for such states, and provides a natural approach to quantum Markovianity for this case. We show that this set of completely positive maps can be experimentally characterized using only local operations on the system, via a generalization of noise spectroscopy protocols. As further applications, we first consider the problem of retrodicting the dynamics of an open quantum system which is in an arbitrary state when it becomes accessible to the experimenter and explore the conditions under which retrodiction is possible. We also introduce a related one-sided or limited-access tomography protocol for determining an arbitrary bipartite state, evolving under a sufficiently rich Hamiltonian, via local operations and measurements on just one component. We simulate this protocol for a physical model of particular relevance to nitrogen-vacancy centers and in particular show how to reconstruct the density matrix of a set of three qubits, interacting via dipolar coupling and in the presence of local magnetic fields, by measuring and controlling only one of them.
We construct a non-Markovian canonical dynamical map that accounts for systems correlated with the environment. The physical meaning of not completely positive maps is studied to obtain a theory of non-Markovian quantum dynamics. The relationship between inverse maps and correlations with the environment is established. A generalized non-Markovian master equation is derived from the canonical dynamical map that goes beyond the Kossakowski-Lindblad Markovian master equation. Non-equilibrium quantum thermodynamics can be be studied within this theory.
We construct a non-Markovian dynamical map that accounts for systems correlated to the environment. We refer to it as a canonical dynamical map, which forms an evolution family. The relationship between inverse maps and correlations with the environment is established. The mathematical properties of complete positivity is related to classical correlations, according to quantum discord, between the system and the environment. A generalized non-Markovian master equation is derived from the canonical dynamical map.
Standard theoretical descriptions of the dynamics of open quantum systems rely on the assumption that the correlations with the environment can be neglected at some reference (initial) time. While being reasonable in specific instances, such as when the coupling between the system and the environment is weak or when the interaction starts at a distinguished time, the use of initially uncorrelated states is questionable if one wants to deal with general models, taking into account the mutual influence that the open-system and environmental evolutions perform on each other. Here we introduce a perturbative method that can be applied to any microscopic modeling of the system-environment interaction, including fully general initial correlations. Extending the standard technique based on projection operators that single out the relevant part of the global dynamics, we define a family of projections adapted to a convenient decomposition of the initial state, which involves a convex mixture of product operators with proper environmental states. This leads us to characterize the open-system dynamics via an uncoupled system of differential equations, which are homogeneous and whose number is limited by the dimensionality of the open system, for any kind of initial correlations. Our method is further illustrated by means of two case studies, for which it reproduces the expected dynamical behavior in the long-time regime more consistently than the standard projection technique.
Understanding system-environment correlations in open quantum systems is vital for various quantum information and technology applications. However, these correlations are often overlooked or hidden in derivations of open-quantum-system master equations, especially when applying the Born approximation. To address this issue, given a microscopic model, we demonstrate how to retain system-environment correlation within commonly used master equations, such as the Markovian Lindblad, Redfield, second-order time convolutionless, second-order Nakajima-Zwanzig, and second-order universal Lindblad-like equations. We show that each master equation corresponds to a particular approximation on the system-environment correlation operator. In particular, our analysis exposes the form of the hidden system-environment correlation in the Markovian Lindblad equation derived using the Born approximation. We also identify that the processes leading to the Redfield equation yield an inaccurate initial-time system-environment correlation approximation. By fixing this problem, we propose a corrected Redfield equation with an improved prediction for early stages of the time evolution. We further illustrate our results in two examples, which imply that the second-order universal Lindblad-like equation captures correlation more accurately than the other standard master equations. Published by the American Physical Society 2024