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arXiv:2502.02466

Frequency auto-homogenization using group-velocity-matched downconversion

Dylan A. Heberle, Christopher C. Tison, James Schneeloch, A. Matthew Smith, Paul M. Alsing, Jeffrey Moses, Michael L. Fanto

Published Feb 4, 2025• 0 citations
arXivHTMLPDF

Abstract

With the stability of integrated photonics at network nodes and the advantages of photons as flying qubits, photonic quantum information processing (PQIP) makes quantum networks increasingly scalable. However, scaling up PQIP requires the preparation of many identical single photons which is limited by the spectral distinguishability of integrated single-photon sources due to variations in fabrication or local environment. To address this, we introduce frequency auto-homogenization via group-velocity-matched downconversion to remove spectral distinguishability in varying quantum emitters. We present our theory using $χ^{(2)}$ quantum frequency conversion and show proof-of-principle data in a free-space optical setup.

DOI
10.48550/arxiv.2502.02466

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With the stability of integrated photonics at network nodes and the advantages of photons as flying qubits, photonic quantum information processing (PQIP) makes quantum networks increasingly scalable. However, scaling up PQIP requires the preparation of many identical single photons which is limited by the spectral distinguishability of integrated single-photon sources due to variations in fabrication or local environment. To address this, we introduce frequency auto-homogenization via group-velocity-matched downconversion to remove spectral distinguishability in varying quantum emitters. We present our theory using χ(2)χ^{(2)}χ(2) quantum frequency conversion and show proof-of-principle data in a free-space optical setup.
Long-distance transmission of quantum information between various systems, such as single-photon sources, quantum memories or matter-based quantum information processing units is hampered by disparate spectral-temporal properties of photons that can be efficiently emitted or absorbed by such systems. Quantum frequency conversion, i.e. low noise nonlinear optical frequency conversion, is an established method to address photon central frequency distinguishability. However, it does not address the issue of single-photon spectral bandwidth and timescale variations, which can range from single picoseconds to hundreds of nanoseconds.
Abstract Low-noise frequency conversion of single photons is a critical tool in establishing fibre-based quantum networks. We show that a single photonic crystal fibre can achieve frequency conversion by Bragg-scattering four-wave mixing of source photons from an ultra-broad wavelength range by engineering a symmetric group velocity profile. Furthermore, we discuss how pump tuning can mitigate realistic discrepancies in device fabrication. This enables a single highly adaptable frequency conversion interface to link disparate nodes in a quantum network via the telecoms band.
Efficiently generating photon pairs with high heralding efficiency and high single photon purity that are bandwidth matched to quantum emitters, quantum memories, and other matter-based qubits is critical for quantum networking applications. However, nonlinear optics-based sources require substantial spectral engineering to overcome the orders of magnitude bandwidth mismatch between those sources and qubit systems. A popular solution is cavity-enhanced spontaneous parametric down conversion (SPDC) where the cavity sets the photon bandwidth and simultaneously enhances the spectral brightness of the SPDC. Bulk, free-space configurations are generally required to achieve the MHz-scale bandwidths required to interface with most qubit systems. Replicating these in scalable integrated photonic architectures is an ongoing challenge due to the much higher propagation losses that limit the size and linewidth of chip-based resonators. We show here how an intra-cavity slow light medium, acting as an ultra-narrow filter, would enable narrowband photon pair generation in broadband cavities with high single photon purity and without compromising the heralding efficiency. We show that such metrics can be readily realized in erbium doped thin-film lithium niobate microrings using realistic design parameters.
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Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. Practicable QFC interfaces connecting ultraviolet and telecommunication bands are of great significance but have remained elusive, constrained by the dual challenges of a high-performance frequency converter and effective noise suppression in short-wavelength pumping configurations. We address this by demonstrating the phase-matching mechanism with domain defects and differential-tuning behavior of the spontaneous parametric down-conversion noises. Based on a quantitative analysis of performance degradation induced by domain defects, we propose specific fabrication guidelines and experimentally achieve an ultrahigh normalized conversion efficiency of 839%/(W cm^{2}) for the fundamental guided mode in thin-film lithium niobate waveguides. Meanwhile, we reveal a new noise control mechanism for short-wavelength pumping by utilizing the differential-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion processes. Then a single-stage QFC from 393 nm to the telecom C band with a record-high external efficiency of 28.8% and an ultralow noise level of 35 counts per second is achieved experimentally. The proposed mechanisms would enable other QFCs with higher efficiency and lower noise, advancing the development of scalable quantum networks. Furthermore, it holds significant potential for driving progress in both classical and integrated nonlinear photonics.
Time-bin encoding of photons offers a robust kind of long-distance quantum communication over lossy channels. The diversity of material nodes in quantum networks operating at natural frequencies requires coherent frequency and wave-form conversion of information-carrying photons to provide an efficient quantum interface with optical fibers and various quantum memories, which has been extensively studied. However, the quantum frequency conversion with transfer of time-bin encoding between single photons of different wavelengths has not yet been explored. In this paper, we present a method for efficiently exchanging time-bin encoding in the conversion process between two photons propagating in cold tripod atoms driven by a strong laser field. The latter is designed to slow down photons and suppress their absorption due to electromagnetically induced transparency. Photons interact parametrically through modified atomic coherence, which is utilized also to achieve equal group velocities of photons. We demonstrate the ability of our model to generate entanglement between distant atoms that equally share the original quantum information stored in the ground-state polarization qubits of both atoms. The proposed method for frequency conversion based on modified atomic coherence is promising because it can simplify the implementation of reliable and high-speed quantum communication protocols based on single-photon entanglement.