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arXiv:1901.09826 · Optics Express

Quantum optical frequency up-conversion for polarisation entangled qubits: towards interconnected quantum information devices

Florian Kaiser, Panagiotis Vergyris, Anthony Martin, Djeylan Aktas, Marc de Micheli, Olivier Alibart, Sébastien Tanzilli

Published Aug 26, 2019• 28 citations
arXivHTMLPDF

Abstract

Realising a global quantum network requires combining individual strengths of different quantum systems to perform universal tasks, notably using flying and stationary qubits. However, transferring coherently quantum information between different systems is challenging as they usually feature different properties, notably in terms of operation wavelength and wavepacket. To circumvent this problem for quantum photonics systems, we demonstrate a polarisation-preserving quantum frequency conversion device in which telecom wavelength photons are converted to the near infrared, at which a variety of quantum memories operate. Our device is essentially free of noise, which we demonstrate through near perfect single photon state transfer tomography and observation of high-fidelity entanglement after conversion. In addition, our guided-wave setup is robust, compact, and easily adaptable to other wavelengths. This approach therefore represents a major building block towards advantageously connecting quantum information systems based on light and matter.

DOI
10.1364/oe.27.025603

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Realising a global quantum network requires combining individual strengths of different quantum systems to perform universal tasks, notably using flying and stationary qubits. However, transferring coherently quantum information between different systems is challenging as they usually feature different properties, notably in terms of operation wavelength and wavepacket. To circumvent this problem for quantum photonics systems, we demonstrate a polarisation-preserving quantum frequency conversion device in which telecom wavelength photons are converted to the near infrared, at which a variety of quantum memories operate. Our device is essentially free of noise, which we demonstrate through near perfect single photon state transfer tomography and observation of high-fidelity entanglement after conversion. In addition, our guided-wave setup is robust, compact, and easily adaptable to other wavelengths. This approach therefore represents a major building block towards advantageously connecting quantum information systems based on light and matter.
In a typical quantum repeater scenario, remote quantum memories have to be interconnected by flying qubits transmitted in quantum channels. e.g. single photons in photonic fiber links. To establish long-distance communication, photons in the low-loss telecom wavlength regime are desirable. However, the majority of the candidates for quantum memories such as trapped atoms or ions, rare earth ensembles, color centers in diamond, atomic ensembles etc. possess optical transitions merely in the visible or near-infrared spectral regime below 1000 nm. One possible solution is the transduction of these wavelengths to the telecom region via quantum frequency conversion (QFC) based on three-wave-mixing processes in a nonlinear χ(2)-medium. Technical achievements in recent years enabled high conversion efficiencies and low conversion-induced noise contributions resulting in signal-to-background ratios high enough to demonstrate the preservation of several classical and quantum properties of the photons, e.g. first- and second-order coherence [1], time-bin entanglement [2], polarization entanglement [3] or indistinguishability [4]. QFC thus provides a powerful toolbox to interface quantum systems to the telecom bands and beyond that yet to interconnect dissimilar quantum systems.
Abstract Entanglement between a stationary quantum system and a flying qubit is an essential ingredient of a quantum-repeater network. It has been demonstrated for trapped ions, trapped atoms, color centers in diamond, or quantum dots. These systems have transition wavelengths in the blue, red or near-infrared spectral regions, whereas long-range fiber-communication requires wavelengths in the low-loss, low-dispersion telecom regime. A proven tool to interconnect flying qubits at visible/NIR wavelengths to the telecom bands is quantum frequency conversion. Here we use an efficient polarization-preserving frequency converter connecting 854 nm to the telecom O-band at 1310 nm to demonstrate entanglement between a trapped 40Ca+ ion and the polarization state of a telecom photon with a high fidelity of 98.2 ± 0.2%. The unique combination of 99.75 ± 0.18% process fidelity in the polarization-state conversion, 26.5% external frequency conversion efficiency and only 11.4 photons/s conversion-induced unconditional background makes the converter a powerful ion–telecom quantum interface.
A key enabling feature of future quantum networks is interoperability between platforms that operate at different wavelengths and with different qubit encodings. We demonstrate an interface that converts atom-photon entanglement from polarization encoding at an atomic wavelength to time-bin encoding in the telecom C-band. Atom-entangled photons at 854 nm are generated from a single 40^{40}40Ca+^++ ion. After quantum frequency conversion to 1550 nm, the photonic polarization qubit is converted into a time-bin qubit using a fiber-based Mach--Zehnder-like encoder. Full quantum tomography of the final state verifies that the process preserves entanglement with 96.3(4.2)% fidelity. Together with the independent work of Ferrari et al. [arXiv:2607.07805 (2026)], this is the first demonstration of polarization-to-time-bin conversion of photons entangled with a single atomic quantum memory. The telecom-compatible interface enables robust qubit transmission over optical fibers and provides a key building block for heterogeneous quantum networking architectures.
Abstract Entanglement between a stationary quantum system and a flying qubit is an essential ingredient of a quantum-repeater network. It has been demonstrated for trapped ions, trapped atoms, color centers in diamond, or quantum dots. These systems have transition wavelengths in the blue, red or near-infrared spectral regions, whereas long-range fiber-communication requires wavelengths in the low-loss, low-dispersion telecom regime. A proven tool to interconnect flying qubits at visible/NIR wavelengths to the telecom bands is quantum frequency conversion. Here we use an efficient polarization-preserving frequency converter connecting 854 nm to the telecom O-band at 1310 nm to demonstrate entanglement between a trapped 40Ca+ ion and the polarization state of a telecom photon with a high fidelity of 98.2 ± 0.2%. The unique combination of 99.75 ± 0.18% process fidelity in the polarization-state conversion, 26.5% external frequency conversion efficiency and only 11.4 photons/s conversion-induced unconditional background makes the converter a powerful ion–telecom quantum interface.
The ability to control the optical frequency of quantum state carriers (i.e. photons) is an important functionality for future quantum networks. It allows all matter quantum systems - nodes of the network - to be compatible with the telecommunication C-band, therefore enabling long distance fiber quantum communication between them. It also allows dissimilar nodes to be connected with each other, thus resulting in heterogeneous networks that can take advantage of the different capabilities offered by the diversity of its constituents. Quantum memories are one of the building blocks of a quantum network, enabling the storage of quantum states of light and the entanglement distribution over long distances. In our group, two different types of memories are investigated: a cold atomic ensemble and an ion-doped crystal. In this thesis I investigate the quantum frequency conversion of narrow-band photons, emitted or absorbed by optical quantum memories, with two different objectives: the first one is to connect quantum memories emitting or absorbing visible single photons with the telecommunication wavelengths, where fiber transmission loss is minimum. The second and main goal is to study the compatibility between disparate quantum nodes, emitting or absorbing photons at different wavelengths. More precisely the objective is to achieve a quantum connection between the two optical memories studied using quantum frequency conversion techniques. The main core of this work is the quantum frequency conversion interface that bridges the gap between the cold ensemble of Rubidium atoms, emitting photons at 780nm, and the Praseodymium ion doped crystal, absorbing photons at 606nm. This interface is composed of two different frequency conversion devices, where a cascaded conversions takes place: the first one converts 780nm photons to the telecommunication C-band, and the second one converts them back to visible, at 606nm. This comes with several challenges such as conversion efficiency, phase stability and parasitic noise reduction, which are important considerations to show the conservation of quantum behaviors through the conversion process. This work can be divided in three parts. In a first one, we built a quantum frequency conversion interface between 606nm and the C-band wavelength, capable of both up and down-conversion of single photon level light. We also characterized the noise processes involved in this specific conversion. In the down-conversion case we showed that memory compatible heralded single photons emitted from a photon pair source preserve their non-classical properties through the conversion process. In the up-conversion case, we showed the storage of converted telecom photons in the praseodymium doped crystal, and their retrieval with high signal to noise ratio. The second part of the work was devoted to the conversion of photons from an emissive Rubidium atomic quantum memory to the telecom C band. In this work we converted the heralding photons from the atomic ensemble and measured non-classical correlations between a stored excitation and a C-band photon, necessary for quantum repeater applications. In the last part of the thesis, we setup the full frequency conversion interface and showed that heralded photons emitted by the atomic ensemble are converted, stored in the solid state memory and retrieved with high signal to noise ratio. We demonstrated that a single collective excitation stored in the atomic ensemble is transfered to the crystal by mean of a single photon at telecom wavelength. We also showed time-bin qubit transfer between the two quantum memories. This work represents the first proof of principle of a photonic quantum connection between disparate quantum memory nodes. The results presented in this thesis pave the way towards the realization of modular and hybrid quantum networks.
Single-photon sources based on quantum dots have been shown to exhibit almost ideal properties such as high brightness and purity in terms of clear anti-bunching as well as high two-photon interference visibilities of the emitted photons, making them promising candidates for different quantum information applications such as quantum computing, quantum communication and quantum teleportation. However, as most single-photon sources also quantum dots typically emit light at wavelengths of electronic transitions within the visible or the near infrared range. In order to establish quantum networks with remote building blocks, low-loss single photons at telecom wavelengths are preferable, though. Despite recent progress on emitters of telecom-photons, the most efficient single-photon sources still work at shorter wavelengths. On that matter, quantum frequency down-conversion, being a nonlinear optical process, has been used in recent years to alter the wavelength of single photons to the telecom wavelength range while conserving their nonclassical properties. Characteristics such as lifetime, first-order coherence, anti-bunching and entanglement have been shown to be conserved or even improved due to background suppression during the conversion process, while the conservation of indistinguishability was yet to be shown. Here we present our experimental results on quantum frequency down-conversion of single photons emitted by an InAs/GaAs quantum dot at 903.6 nm following a pulsed excitation of a p-shell exciton at 884 nm. The emitted fluorescence photons are mixed with a strong pump-field at 2155 nm inside a periodically poled lithium niobate ridge waveguide and converted to 1557 nm. Common issues of a large background due to Raman-scattered pump-light photons spectrally overlapping with the converted single photons could largely be avoided, as the pump-wavelength was chosen to be fairly longer than the target wavelength. Additional narrowband spectral filtering at the telecom regime as a result of the small conversion bandwidth and using a high-performance fiber-Bragg-grating solely left the detector dark counts as the only noise source in our setup. Therefore, we could achieve conversion efficiencies of more than 20 %. In order to test the indistinguishability, sequentially emitted photons were fed into a Mach-Zehnder interferometer and spatially as well as temporally overlapped at the output beam splitter. Cross-correlation measurements between both output-ports of the beam splitter exhibit two-photon interference contrasts of more than 40 % prior to and after the down-conversion step. Accordingly, we demonstrate that the process of quantum frequency conversion preserves photon indistinguishability and can be used to establish a versatile source of indistinguishable single photons at the telecom C-Band. Furthermore our scheme allows for converting photons in a wavelength band from 900 nm to 910 nm to the same telecom target wavelength. This enables us to test indistinguishability of frequency-converted photons, originally stemming from different sources with dinstinguishable wavelengths.