We report on the study of itinerant magnetism of lattice-trapped magnetic atoms, driven by magnetic dipole-dipole interactions, in the low-entropy and close-to-unit filling regime. We have used advanced dynamical decoupling techniques to efficiently suppress the sensitivity to magnetic field fluctuations. We have thus measured the spin coherence of an itinerant spin 3 Bose dipolar gas throughout a quantum phase transition from a superfluid phase to a Mott insulating phase. In the superfluid phase, a metastable ferromagnetic behavior is observed below a dynamical instability that occurs at lattice depths below the phase transition. In the insulating phase, the thermalization toward a paramagnetic state is driven by an interplay between intersite and superexchange interactions.We report on the study of itinerant magnetism of lattice-trapped magnetic atoms, driven by magnetic dipole-dipole interactions, in the low-entropy and close-to-unit filling regime. We have used advanced dynamical decoupling techniques to efficiently suppress the sensitivity to magnetic field fluctuations. We have thus measured the spin coherence of an itinerant spin 3 Bose dipolar gas throughout a quantum phase transition from a superfluid phase to a Mott insulating phase. In the superfluid phase, a metastable ferromagnetic behavior is observed below a dynamical instability that occurs at lattice depths below the phase transition. In the insulating phase, the thermalization toward a paramagnetic state is driven by an interplay between intersite and superexchange interactions.

Physical Review LettersFeb 2, 20261 citation

Probing spin dynamics from the Mott insulating to the superfluid regime in a dipolar lattice gas

A. de Paz, P. Pedri, Arijit Sharma +6 more

We analyze the spin dynamics of an out-of-equilibrium large spin dipolar atomic Bose gas in an optical lattice. We observe a smooth crossover from a complex oscillatory behavior to an exponential behavior throughout the Mott-to-superfluid transition. While both of these regimes are well described by our theoretical models, we provide data in the intermediate regime where dipolar interactions, contact interactions, and superexchange mechanisms compete. In this strongly correlated regime, spin dynamics and transport are coupled, which challenges theoretical models for quantum magnetism.We analyze the spin dynamics of an out-of-equilibrium large spin dipolar atomic Bose gas in an optical lattice. We observe a smooth crossover from a complex oscillatory behavior to an exponential behavior throughout the Mott-to-superfluid transition. While both of these regimes are well described by our theoretical models, we provide data in the intermediate regime where dipolar interactions, contact interactions, and superexchange mechanisms compete. In this strongly correlated regime, spin dynamics and transport are coupled, which challenges theoretical models for quantum magnetism.

arXiv:1507.04273Physical Review AFeb 2, 201632 citations

Magnetic phase transition in coherently coupled Bose gases in optical lattices

Luca Barbiero, Marta Abad, Alessio Recati

We describe the ground state of a gas of bosonic atoms with two coherently coupled internal levels in a deep optical lattice in a one-dimensional geometry. In the single-band approximation this system is described by a Bose-Hubbard Hamiltonian. The system has a superfluid and a Mott insulating phase that can be either paramagnetic or ferromagnetic. We characterize the quantum phase transitions at unit filling by means of a density-matrix renormalization-group technique and compare the results with a mean-field approach and an effective spin Hamiltonian. The presence of the ferromagnetic Ising-like transition modifies the Mott lobes. In the Mott insulating region the system maps to the ferromagnetic spin-1/2 $XXZ$ model in a transverse field and the numerical results compare very well with the analytical results obtained from the spin model. In the superfluid regime quantum fluctuations strongly modify the phase transition with respect to the well-established mean-field three-dimensional classical bifurcation.We describe the ground state of a gas of bosonic atoms with two coherently coupled internal levels in a deep optical lattice in a one-dimensional geometry. In the single-band approximation this system is described by a Bose-Hubbard Hamiltonian. The system has a superfluid and a Mott insulating phase that can be either paramagnetic or ferromagnetic. We characterize the quantum phase transitions at unit filling by means of a density-matrix renormalization-group technique and compare the results with a mean-field approach and an effective spin Hamiltonian. The presence of the ferromagnetic Ising-like transition modifies the Mott lobes. In the Mott insulating region the system maps to the ferromagnetic spin-1/2 $XXZ$ model in a transverse field and the numerical results compare very well with the analytical results obtained from the spin model. In the superfluid regime quantum fluctuations strongly modify the phase transition with respect to the well-established mean-field three-dimensional classical bifurcation.

arXiv:1403.4185Physical Review AMar 25, 201611 citations

Mott phases and superfluid-insulator transition of dipolar spin-three bosons in an optical lattice: Implications for Cr52 atoms

Jean-Sébastien Bernier, K. Sengupta, Yong Baek Kim

We study the Mott phases and superfluid-insulator transition of spin-three bosons in an optical lattice with an anisotropic two-dimensional optical trap. We chart out the phase diagrams for Mott states with $n=1$ and $n=2$ atoms per lattice site. It is shown that the long-range dipolar interaction stabilizes a state where the chains of the ferromagnetically aligned spins run along the longer trap direction while the spin ordering is staggered between nearby chains, leading to an antiferromagnetic ordering along the shorter trap direction. We also obtain the mean-field phase boundary for the superfluid-insulator transition in these systems and study the nature of spin ordering in the superfluid state near the transition. We show that, inside the superfluid phase and near the superfluid-insulator phase boundary, the system undergoes a first-order antiferromagnetic-ferromagnetic spin ordering transition. We discuss implications of our results for $^{52}\mathrm{Cr}$ atoms and suggest possible experiments to detect different phases in such systems.We study the Mott phases and superfluid-insulator transition of spin-three bosons in an optical lattice with an anisotropic two-dimensional optical trap. We chart out the phase diagrams for Mott states with $n=1$ and $n=2$ atoms per lattice site. It is shown that the long-range dipolar interaction stabilizes a state where the chains of the ferromagnetically aligned spins run along the longer trap direction while the spin ordering is staggered between nearby chains, leading to an antiferromagnetic ordering along the shorter trap direction. We also obtain the mean-field phase boundary for the superfluid-insulator transition in these systems and study the nature of spin ordering in the superfluid state near the transition. We show that, inside the superfluid phase and near the superfluid-insulator phase boundary, the system undergoes a first-order antiferromagnetic-ferromagnetic spin ordering transition. We discuss implications of our results for $^{52}\mathrm{Cr}$ atoms and suggest possible experiments to detect different phases in such systems.

arXiv:cond-mat/0612044Physical Review BJul 5, 20079 citations

Extended Bose-Hubbard models with ultracold magnetic atoms

Simon Baier, Mark, Manfred, Daniel Petter +7 more

The Hubbard model underlies our understanding of strongly correlated materials. Whereas its standard form only comprises interactions between particles at the same lattice site, extending it to encompass long-range interactions is predicted to profoundly alter the quantum behavior of the system. We realize the extended Bose-Hubbard model for an ultracold gas of strongly magnetic erbium atoms in a three-dimensional optical lattice. Controlling the orientation of the atomic dipoles, we reveal the anisotropic character of the onsite interaction and hopping dynamics and their influence on the superfluid-to-Mott insulator quantum phase transition. Moreover, we observe nearest-neighbor interactions, a genuine consequence of the long-range nature of dipolar interactions. Our results lay the groundwork for future studies of exotic many-body quantum phases.The Hubbard model underlies our understanding of strongly correlated materials. Whereas its standard form only comprises interactions between particles at the same lattice site, extending it to encompass long-range interactions is predicted to profoundly alter the quantum behavior of the system. We realize the extended Bose-Hubbard model for an ultracold gas of strongly magnetic erbium atoms in a three-dimensional optical lattice. Controlling the orientation of the atomic dipoles, we reveal the anisotropic character of the onsite interaction and hopping dynamics and their influence on the superfluid-to-Mott insulator quantum phase transition. Moreover, we observe nearest-neighbor interactions, a genuine consequence of the long-range nature of dipolar interactions. Our results lay the groundwork for future studies of exotic many-body quantum phases.

Apr 1, 2016276 citations

Extended Bose-Hubbard models with ultracold magnetic atoms

Simon Baier, M. J. Mark, Daniel Petter +6 more

arXiv:1507.03500ScienceApr 7, 2016332 citations

XXZ

model in a transverse field and the numerical results compare very well with the analytical results obtained from the spin model. In the superfluid regime quantum fluctuations strongly modify the phase transition with respect to the well-established mean-field three-dimensional classical bifurcation.

n=1

and

n=2

atoms per lattice site. It is shown that the long-range dipolar interaction stabilizes a state where the chains of the ferromagnetically aligned spins run along the longer trap direction while the spin ordering is staggered between nearby chains, leading to an antiferromagnetic ordering along the shorter trap direction. We also obtain the mean-field phase boundary for the superfluid-insulator transition in these systems and study the nature of spin ordering in the superfluid state near the transition. We show that, inside the superfluid phase and near the superfluid-insulator phase boundary, the system undergoes a first-order antiferromagnetic-ferromagnetic spin ordering transition. We discuss implications of our results for

^{52}\mathrm{Cr}

atoms and suggest possible experiments to detect different phases in such systems.