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arXiv:2501.11259

The origin of anomalous non-linear microwave absorption in Josephson junction qubits: mysterious nature of two level systems or their dynamic interaction?

Alexander L. Burin

Published Jan 20, 2025• 0 citations
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Abstract

Quantum two-level systems (TLSs) commonly found at low temperature in amorphous and disordered materials are responsible for decoherence in superconducting Josephson junction qubits particularly because they absorb energy of coherent qubit oscillations in the microwave frequency range. In planar Josephson resonators with oxide interfaces this absorption is characterized by an anomalously weak loss tangent dependence on the field in the non-linear regime that conflicts with the theoretical expectations and the observations in amorphous dielectrics. It was recently suggested that this anomalous absorption is due to TLS dynamic interactions. Here we show that such interactions cannot lead to the observed loss-tangent field dependence and suggest the alternative explanation assuming that TLS dipole moments $p$ are distributed according to the specific power law $P(p) \propto 1/p^{3-η}$ ($0\leq η<1$). This assumption, indeed, results in the observed loss tangent behavior. The hypothesis of a power law distribution is supported both by the recent measurements of individual TLS dipole moments and the theoretical model of TLS formation due to the long-range dipole-dipole interaction, thus connecting the anomalous absorption with the possible solution of the long-standing problem of the nature of TLSs.

DOI
10.48550/arxiv.2501.11259

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Quantum two-level systems (TLSs) commonly found at low temperature in amorphous and disordered materials are responsible for decoherence in superconducting Josephson junction qubits particularly because they absorb energy of coherent qubit oscillations in the microwave frequency range. In planar Josephson resonators with oxide interfaces this absorption is characterized by an anomalously weak loss tangent dependence on the field in the non-linear regime that conflicts with the theoretical expectations and the observations in amorphous dielectrics. It was recently suggested that this anomalous absorption is due to TLS dynamic interactions. Here we show that such interactions cannot lead to the observed loss-tangent field dependence and suggest the alternative explanation assuming that TLS dipole moments ppp are distributed according to the specific power law P(p)∝1/p3−ηP(p) \propto 1/p^{3-η}P(p)∝1/p3−η (0≤η<10\leq η<10≤η<1). This assumption, indeed, results in the observed loss tangent behavior. The hypothesis of a power law distribution is supported both by the recent measurements of individual TLS dipole moments and the theoretical model of TLS formation due to the long-range dipole-dipole interaction, thus connecting the anomalous absorption with the possible solution of the long-standing problem of the nature of TLSs.
The microwave absorption and noise caused by quantum two-level systems (TLSs) dramatically suppress the coherence in Josephson junction qubits that are promising candidates for quantum information applications. It is a challenge to understand microwave absorption by TLSs because of the spectral diffusion resulting from fluctuations in their resonant frequencies induced by their long-range interactions. Here we treat the spectral diffusion explicitly using the generalized master equation formalism. The proposed theory predicts that the linear absorption regime holds while a TLS Rabi frequency is smaller than their phase decoherence rate. At higher external fields, a nonlinear absorption regime is found with the loss tangent inversely proportional to the intensity of the field. The theory can be generalized to acoustic absorption and lower dimensions realized in superconducting qubits.
While several experiments claim that two-level system (TLS) defects in amorphous surfaces and interfaces are responsible for energy relaxation in superconducting resonators and qubits, none can provide quantitative explanation of their data in terms of the conventional noninteracting TLS model. Here a model that interpolates between the interacting and noninteracting TLS loss tangent is proposed to perform numerical analysis of experimental data and extract information about TLS parameters and their distribution. As a proof of principle, the model is applied to TESLA cavities that contain only a single lossy material in their interior, the niobium-niobium oxide interface. The best fits show interacting TLSs with a sharp modulus of electric dipole moment for both thin (5nm5\phantom{\rule{0.2em}{0ex}}\mathrm{nm}5nm) and thick (100nm100\phantom{\rule{0.2em}{0ex}}\mathrm{nm}100nm) oxides, indicating that the TLSs are ``atomic'' instead of ``glassy.'' The proposed method can be applied to other devices with multiple material interfaces and substrates, with the goal of elucidating the nature of TLSs causing energy loss in resonators and qubits.
Quantum two-level systems (TLSs) intrinsic to glasses induce decoherence in many modern quantum devices, such as superconducting qubits. Although the low-temperature physics of these TLSs is usually well-explained by a phenomenological standard tunneling model of independent TLSs, the nature of these TLSs, as well as their behavior out of equilibrium and at high energies above 1 K, remain inconclusive. Here we measure the non-equilibrium dielectric loss of TLSs in amorphous silicon using a superconducting resonator, where energies of TLSs are varied in time using a swept electric field. Our results show the existence of two distinct ensembles of TLSs, interacting weakly and strongly with phonons, where the latter also possesses anomalously large electric dipole moment. These results may shed new light on the low temperature characteristics of amorphous solids, and hold implications to experiments and applications in quantum devices using time-varying electric fields.
It is frequently observed that even at very low temperatures, the number of quasiparticles in superconducting materials is higher than predicted by standard BCS theory. These quasiparticles can interact with two-level systems, such as superconducting qubits or two-level systems (TLS) in the amorphous oxide layer of a Josephson junction. This interaction leads to decay and decoherence of the TLS, with specific results, such as time dependence, depending on the distribution of quasiparticles and the form of interaction. We study the resulting decay laws for different experimentally relevant protocols.
Increasing and stabilizing the coherence of superconducting quantum circuits and resonators is of utmost importance for various technologies, ranging from quantum information processors to highly sensitive detectors of low-temperature radiation in astrophysics. A major source of noise in such devices is a bath of quantum two-level systems (TLSs) with broad distribution of energies, existing in disordered dielectrics and on surfaces. Here we study the dielectric loss of superconducting resonators in the presence of a periodic electric bias field, which sweeps near-resonant TLSs in and out of resonance with the resonator, resulting in a periodic pattern of Landau–Zener transitions. We show that at high sweep rates compared to the TLS relaxation rate, the coherent evolution of the TLS over multiple transitions yields a significant reduction in the dielectric loss relative to the intrinsic value. This behavior is observed both in the classical high-power regime and in the quantum single-photon regime, possibly suggesting a viable technique to dynamically decouple TLSs from a qubit.
Superconducting microwave resonators are critical to quantum computing and sensing technologies. Additionally, they are common proxies for superconducting qubits when determining the effects of performance-limiting loss mechanisms such as from two-level systems (TLSs). The extraction of these loss mechanisms is often performed by measuring the internal quality factor Qi as a function of power or temperature. In this work, we investigate large temporal fluctuations of Qi at low powers over periods of 12–16 h (relative standard deviation σQi/Qi=13%). These fluctuations are ubiquitous across multiple resonators, chips, and cooldowns. We are able to attribute these fluctuations to variations in the TLS loss tangent due to two main indicators. First, measured fluctuations decrease as power and temperature increase. Second, for interleaved measurements, we observe correlations between low- and medium-power Qi fluctuations and an absence of correlations with high-power fluctuations. Agreement with the TLS loss tangent mean is obtained by performing measurements over a time span of a few hours. We hypothesize that, in addition to decoherence, due to coupling to individual near-resonant TLS, superconducting qubits are affected by these observed TLS loss tangent fluctuations.