Resonance fluorescence spectra of a driven Kerr nonlinear resonator is investigated both theoretically and experimentally. When the Kerr nonlinear resonator is driven strongly such that the induced Rabi frequency is comparable to or larger than the Kerr nonlinearity, the system cannot be approximated as a two-level system. We theoretically derive characteristic features in the fluorescence spectra such as the decrease of the center-peak intensity and the asymmetric sideband peaks in the presence of finite dephasing. Those features are consistently explained by the population of the initial dressed state and its transition matrix element to the final dressed state of the transition corresponding to each peak. Finally, we experimentally measure the resonance fluorescence spectra of a driven superconducting Kerr nonlinear resonator and find a quantitative agreement with our theory.
Resonance fluorescence spectra of a driven Kerr nonlinear resonator is investigated both theoretically and experimentally. When the Kerr nonlinear resonator is driven strongly such that the induced Rabi frequency is comparable to or larger than the Kerr nonlinearity, the system cannot be approximated as a two-level system. We theoretically derive characteristic features in the fluorescence spectra such as the decrease of the center-peak intensity and the asymmetric sideband peaks in the presence of finite dephasing. Those features are consistently explained by the population of the initial dressed state and its transition matrix element to the final dressed state of the transition corresponding to each peak. Finally, we experimentally measure the resonance fluorescence spectra of a driven superconducting Kerr nonlinear resonator and find a quantitative agreement with our theory.
The interaction of a resonant light field with a quantum two-level system is of key interest both for fundamental quantum optics and quantum technological applications employing resonant excitation. While emission under resonant continuous-wave excitation has been well-studied, the more complex emission spectrum of dynamically dressed states, a quantum two-level system driven by resonant pulsed excitation, has so far been investigated in detail only theoretically. Here, we present the first experimental observation of the complete resonance fluorescence emission spectrum of a single quantum two-level system, in form of an excitonic transition in a semiconductor quantum dot, driven by finite Gaussian pulses. We observe multiple emerging sidebands as predicted by theory with an increase of their number and spectral detuning with excitation pulse intensity and a dependence of their spectral shape and intensity on the pulse length. Detuning-dependent measurements provide additional insights into the emission features. The experimental results are in excellent agreement with theoretical calculations of the emission spectra, corroborating our findings.
The interaction of a resonant light field with a quantum two-level system is of key interest both for fundamental quantum optics and quantum technological applications employing resonant excitation. While emission under resonant continuous-wave excitation has been well studied, the more complex emission spectrum of dynamically dressed states-a quantum two-level system driven by resonant pulsed excitation-has so far been investigated in detail only theoretically. Here, we present the first experimental observation of the complete resonance fluorescence emission spectrum of a single quantum two-level system, in the form of an excitonic transition in a semiconductor quantum dot, driven by finite Gaussian pulses. We observe multiple emerging sidebands as predicted by theory, with an increase of their number and spectral detuning with excitation pulse intensity and a dependence of their spectral shape and intensity on the pulse length. Detuning-dependent measurements provide additional insights into the emission features. The experimental results are in excellent agreement with theoretical calculations of the emission spectra, corroborating our findings.
We study the fluorescence spectrum of a strongly driven two-level system (TLS) with modulated transition frequency, which is a bichromatically driven TLS and has multiple resonance frequencies. We are aiming to provide a reliable description of the fluorescence in a regime that is difficult to tackle with perturbation theory and the rotating-wave approximation (RWA), and illustrate the spectral features of the fluorescence under off- and multiphoton-resonance conditions. To go beyond the RWA, we use a semianalytical counter-rotating-hybridized rotating-wave method that combines a unitary transformation and Floquet theory to calculate the two-mode Floquet states and quasienergies for the bichromatically driven TLS. We then solve the master equation accounting for the spontaneous decay in the bases of the two-mode Floquet states, and derive a physically transparent fluorescence spectrum. In comparison with the numerically exact spectrum from the generalized Floquet-Liouville approach, the present spectrum is found to be applicable in a wide range of the parameters where the RWA and the secular approximation may break down. We find that the counter-rotating (CR) terms of the transverse field omitted in the RWA have non-negligible contributions to the spectrum under certain conditions. Particularly, at the multiphoton resonance the width of which is comparable with the Bloch-Siegert shift, the RWA and non-RWA spectra markedly differ from each other because of the CR-induced shift. We also analyze the symmetry of the spectrum in terms of the transition matrix elements between the two-mode Floquet states. We show that the strict symmetry of the spectrum cannot be expected without the RWA but the almost symmetric spectrum can be obtained at the single-photon resonance that takes the Bloch-Siegert shift into account if the driving is moderately strong and at the multiphoton resonance with a sufficiently weak transverse field.
We present the theory of resonance fluorescence from an asymmetric quantum dot driven by a two-component electromagnetic field with two different frequencies, polarizations, and amplitudes (bichromatic field) in the regime of strong light-matter coupling. It follows from the elaborated theory that the broken inversion symmetry of the driven quantum system and the bichromatic structure of the driving field result in unexpected features of the resonance fluorescence, including the infinite set of Mollow triplets, the quench of fluorescence peaks induced by the dressing field, and the oscillating behavior of the fluorescence intensity as a function of the dressing field amplitude. These quantum phenomena are of general physical nature and, therefore, can take place in various double-driven quantum systems with broken inversion symmetry.
Intersubband transitions are unbound electronic transitions of doped quantum wells, semiconductors heterostructures with a planar symmetry. I theoretically studied the fluorescence of a strongly pumped intersubband transition, finding that the many electron nature of such a system leads to a modification of the usual Mollow triplet. In particular, the intensity of the central peak in the fluorescence spectrum becomes a function of the electron coherence, allowing access to the coherence time of a quasi two-dimensional electron gas through a fluorescence intensity measurement. Moreover, while transitions between the two states of the ac Stark-split doublet are forbidden in centrosymmetric systems, and thus almost impossible to observe in experiments performed with atoms they become allowed in asymmetric quantum wells, in which the wave function symmetry can be broken. I developed a many-body theory describing also this intradoublet emission, showing that by using doped asymmetry, the emission can be orders of magnitude higher than in previously studied systems. This opens the way to the realization of monolithic and tunable terahertz emitters since the Rabi frequency at which this emission occurs lies in the terahertz range and can be tuned by the pump power. Finally, I have investigated if superfluorescence can occur in intersubband transitions. In order to do so I used a general quantum master equation that includes dephasing and nonradiative emission to model the many-body system in solid state. Performing a second-order approximation allowed to obtain a closed system of equations that were studied analytically and numerically, verifying that in the regimes characteristic of intersubband transitions cooperative effects leading to powerful bursts of light could be observed experimentally.
The Kerr parametric oscillator (KPO) has recently attracted considerable attention from the perspective of its applications to quantum information processing, and understanding its properties is an important challenge. Spectroscopic measurements serve as an effective means of elucidating detailed information about the system, such as the energy-level structure and the transition matrix elements of the KPO. Conventional spectroscopy requires the drive frequency to match an energy spacing with a nonzero transition matrix element. In recent years, a phenomenon called photonic resonance (PR) has been theoretically predicted in KPO spectroscopy. Specifically, resonance occurs under the condition that the detuning is set to n/2 times the Kerr nonlinearity, where n is a natural number. However, under this condition the transition matrix element vanishes, and thus the mechanism by which photonic resonance (PR) arises has remained unclear. In this work, we aim to elucidate the physical origin of PR observed in KPO spectroscopy. We first performed theoretical calculations and experiments of spectroscopic measurements, confirming that PR can indeed be observed and that the theoretical and experimental results are in qualitative agreement. We then carried out an analytical study under the assumption of an ideal noiseless environment. Our analysis revealed that, although the transition matrix element of the external field expressed in the system's energy eigenbasis is zero, higher-order perturbative effects induce Rabi oscillations between the ground and excited states. Furthermore, numerical simulations in a time domain including the effect of decoherence demonstrated that coherent oscillations decay, leading to the appearance of PR.