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arXiv:2412.11370

Experimental Acceleration of Spin Transition in Nitrogen-Vacancy Center

Chen, Si-Qi, Lu, He

Published Dec 16, 2024• 0 citations
arXivHTMLPDF

Abstract

Shortcuts to adiabaticity~(STA) enables fast and robust coherent control of quantum system, which has been well placed in quantum technologies. In particular, inverse engineering STA provides much more freedom for the optimization of shortcut, which alleviates the complexity for experimental realization. Here, we implement a STA technique, known as invariant-based inverse engineering, to speed up the adiabatic control of the electron triplet ground state of a single nitrogen-vacancy~(NV) center. The microwave pulses to drive inversely engineered STA are obtained with space curve quantum control, where the evolution of spin transition is mapped to a three-dimensional closed space curve and the design of shortcut is obtained by optimization over the space curve. We demonstrate the fast and high-fidelity drive of dipole-forbidden transition between two spin sublevels of the ground state. Moreover, we demonstrate the robustness of the spin transition by introducing the detuning of driving microwave field. The acceleration and robustness is further confirmed by the comparison with two traditional Raman control schemes. Our results suggest invariant-based inverse engineering is powerful for fast and robust manipulation of NV system, and thus benefits quantum sensing and quantum computation based on the NV platform.

DOI
10.48550/arxiv.2412.11370

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•Mar 23, 2021•0 citations
Shortcuts to adiabaticity~(STA) enables fast and robust coherent control of quantum system, which has been well placed in quantum technologies. In particular, inverse engineering STA provides much more freedom for the optimization of shortcut, which alleviates the complexity for experimental realization. Here, we implement a STA technique, known as invariant-based inverse engineering, to speed up the adiabatic control of the electron triplet ground state of a single nitrogen-vacancy~(NV) center. The microwave pulses to drive inversely engineered STA are obtained with space curve quantum control, where the evolution of spin transition is mapped to a three-dimensional closed space curve and the design of shortcut is obtained by optimization over the space curve. We demonstrate the fast and high-fidelity drive of dipole-forbidden transition between two spin sublevels of the ground state. Moreover, we demonstrate the robustness of the spin transition by introducing the detuning of driving microwave field. The acceleration and robustness is further confirmed by the comparison with two traditional Raman control schemes. Our results suggest invariant-based inverse engineering is powerful for fast and robust manipulation of NV system, and thus benefits quantum sensing and quantum computation based on the NV platform.
Shortcuts to adiabaticity (STA) enables fast and robust coherent control of quantum system, which has been well placed in quantum technologies. In particular, inverse-engineering STA provides much more freedom for the optimization of shortcut, which alleviates the complexity for experimental realization. Here, we implement a STA technique, known as invariant-based inverse engineering, to speed up the adiabatic control of the electron triplet ground state of a single nitrogen-vacancy (N-VVV) center. The microwave pulses to drive inversely engineered STA are obtained with space-curve quantum control, where the evolution of spin transition is mapped to a three-dimensional closed space curve and the design of shortcut is obtained by optimization over the space curve. We demonstrate the fast and high-fidelity drive of dipole-forbidden transition between two spin sublevels of the ground state. Moreover, we demonstrate the robustness of the spin transition by introducing the detuning of driving microwave field. The acceleration and robustness is further confirmed by the comparison with two traditional Raman control schemes. Our results suggest invariant-based inverse engineering is powerful for fast and robust manipulation of N-VVV system, and thus benefits quantum sensing and quantum computation based on the N-VVV platform.
Optimal control of quantum system is significant for information science and technology. Here, an efficient scheme is proposed for implementing fast population transfer in a spin qutrit of nitrogen-vacancy center via shortcuts to adiabaticity (STA) with simplified drivings. At two-photon resonance, a Λ\Lambda Λ -configuration interaction between the spin qutrit and driving fields can be obtained effectively. By the invariant-based STA, the reversible population transfer can be realized using the Rabi pulses with sine and cosine waveforms. Compared with the superadiabatic transitionless driving, the present pulses in our strategy become simplified technically, contributing to reduce the error effect of control parameter deviations. Moreover, the high-fidelity quantum operations can be performed with the accessible decoherence rates. The protocol could offer an optimized avenue towards the STA-based quantum control of spin qutrit experimentally.
Microwave pulse sequences are the basis of coherent manipulation of the electronic spin ground state in nitrogen vacancy (NV) centers. In this work we demonstrate stimulated Raman transitions (SRTs) and stimulated Raman adiabatic passage (STIRAP), two ways to drive the dipole-forbidden transition between two spin sublevels in the electronic triplet ground state of the NV center. This driving is achieved by a two-photon Raman microwave pulse which simultaneously drives two detuned transitions via a virtual level for SRTs or via two adiabatic and partially overlapping resonant microwave pulses for STIRAP. We lay the theoretical framework of SRT and STIRAP dynamics and verify experimentally the theoretical predictions of population inversion by observing the dipole-forbidden transition in the ground state of a single NV center. A comparison of the two schemes showed better robustness and success of the spin swap for STIRAP compared to SRT.
We propose a fast mixed-state control scheme to transfer the quantum state along designable trajectories in Hilbert space, which is robust to multiple decoherence noises. Starting with the dynamical invariants of open quantum systems, we present the shortcuts to adiabaticity (STA) of open quantum systems at first, then apply the STA to speed up the adiabatic steady process. Our scheme drives open systems from a initial steady state to a target steady state by a controlled Liouvillian that possesses the same form as the reference (original) one that is accessible in present-day experiments. An experimental design with currently available parameters for the nitrogen-vacancy (N-VVV) center in diamond is suggested and discussed.
Accurate population transfer of uncoupled or weakly coupled spin states is crucial for many quantum-information-processing tasks. In this paper, we propose a fast and robust scheme for population transfer which combines invariant-based inverse engineering and geometric formalism for robust quantum control. Our scheme is not constrained by the adiabatic condition and therefore can be implemented quickly. It can also effectively suppress the dominant noise in spin systems, which together with the fast feature guarantees the accuracy of the population transfer. Moreover, the control parameters of the driving Hamiltonian in our scheme are easy to design because they correspond to the curvature and torsion of a three-dimensional visual space curve derived by using geometric formalism for robust quantum control. We test the efficiency of our scheme by numerically simulating the ground-state population transfer in 15N^{15}\mathrm{N}15N nitrogen-vacancy centers and comparing our scheme with stimulated Raman transition, stimulated Raman adiabatic passage, and conventional shortcuts to adiabaticity based schemes, three types of schemes popularly used for population transfer. The numerical results clearly show that our scheme is advantageous over these previous ones.
Pure-state inverse engineering among the schemes of shortcuts to adiabaticity is a widespread utility in applications to quantum computation and quantum simulation. While in principle it can realise the fast control of quantum systems with high fidelity, in practice this fast control is severely hindered by infinite energy gaps and impractical control fields. To circumvent this problem, we propose a scheme of shortcuts to adiabaticity of mixed state based on the dynamical invariant of open quantum system. Our scheme can drives a steady state to a target steady state of the open system by a controlled Liouvillian that possesses the same form as the reference (original) one. We apply this scheme to stimulated Raman adiabatic passage (STIRAP) and find that an almost perfect population transfer can be obtained. The experimental observation with currently available parameters for the nitrogen-vacancy (NV) center in diamond is suggested and discussed.