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arXiv:2412.08811

TLS and Quasiparticle Loss in Thin-Film Aluminum CPW Resonators: A Modified Model and Design Implications

Carolyn G. Volpert, Emily M. Barrentine, Alberto D. Bolatto, Ari-David Brown, Jake Connors, Thomas Essinger-Hileman, Larry A. Hess, Vilem Mikula, Stevenson, Thomas R., Eric R. Switzer

Published Dec 11, 2024• 0 citations
arXivHTMLPDF

Abstract

As superconducting kinetic inductance detectors (KIDs) continue to grow in popularity for sensitive submillimeter detection and other applications, there is a drive to advance toward lower-loss devices. We present measurements of diagnostic thin-film aluminum coplanar waveguide (CPW) resonators designed to inform ongoing KID development at NASA Goddard Space Flight Center. The resonance frequencies span $f_0$ = 3.5-4 GHz and include quarter-wave and half-wave resonators with varying coupling capacitor designs. We present measurements of the device film properties and an analysis of the dominant mechanisms of loss in the resonators measured in a dark environment, demonstrating quality factors of $Q_i^{-1} \approx 3.64-8.57\ \times 10^{-8}$. We observe an enhanced level of suppression in the loss contributions from two-level systems (TLS) at intermediate-to-high read powers, and a regime at these powers and low temperatures where contributions from intrinsic processes $Q_i^{-1}$,other dominate the total loss. We also observe deviations from the standard TLS loss model at low powers and temperatures below 60 mK, and use a modified model to describe this behavior.

DOI
10.48550/arxiv.2412.08811

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As superconducting kinetic inductance detectors (KIDs) continue to grow in popularity for sensitive submillimeter detection and other applications, there is a drive to advance toward lower-loss devices. We present measurements of diagnostic thin-film aluminum coplanar waveguide (CPW) resonators designed to inform ongoing KID development at NASA Goddard Space Flight Center. The resonance frequencies span f0f_0f0​ = 3.5-4 GHz and include quarter-wave and half-wave resonators with varying coupling capacitor designs. We present measurements of the device film properties and an analysis of the dominant mechanisms of loss in the resonators measured in a dark environment, demonstrating quality factors of Qi−1≈3.64−8.57 ×10−8Q_i^{-1} \approx 3.64-8.57\ \times 10^{-8}Qi−1​≈3.64−8.57 ×10−8. We observe an enhanced level of suppression in the loss contributions from two-level systems (TLS) at intermediate-to-high read powers, and a regime at these powers and low temperatures where contributions from intrinsic processes Qi−1Q_i^{-1}Qi−1​,other dominate the total loss. We also observe deviations from the standard TLS loss model at low powers and temperatures below 60 mK, and use a modified model to describe this behavior.
Superconducting resonators are widely used in many applications such as qubit readout for quantum computing applications, and kinetic inductance detectors. These resonators are susceptible to numerous loss and noise mechanisms under microwave excitation, especially the dissipation due to non-equilibrium quasi-particles and two-level systems (TLS), which can result in a decrease of the superconducting intrinsic quality factor (QiQ_iQi​) in high quality superconducting resonators. Particularly in the few-photon and low temperature (T) regime, TLS losses can become a dominant loss mechanism. In this study, novel aluminum half-wavelength resonators are investigated, focusing on the loss properties at extra-low power and low temperature. An unusual increase of Qi(T)Q_i(T)Qi​(T) with deceasing temperature is observed. This behavior is attributed to the increase of TLS coherence time (T2T_2T2​) at ultra-low temperatures and powers. This T2T_2T2​ increase is consistent with other work on resonant frequency noise in resonators and measurements of individual TLS, and likely arises from interacting TLS in the aluminum half-wavelength resonators.
Superconducting resonators are widely used in many applications such as qubit readout for quantum computing, and kinetic inductance detectors. These resonators are susceptible to numerous loss and noise mechanisms, especially the dissipation due to two-level systems (TLS) which become the dominant source of loss in the few-photon and low temperature regime. In this study, capacitively-coupled aluminum half-wavelength coplanar waveguide resonators are investigated. Surprisingly, the loss of the resonators is observed to decrease with a lowering temperature at low excitation powers and temperatures below the TLS saturation. This behavior is attributed to the reduction of the TLS resonant response bandwidth with decreasing temperature and power to below the detuning between the TLS and the resonant photon frequency in a discrete ensemble of TLS. When response bandwidths of TLS are smaller than their detunings from the resonance, the resonant response and thus the loss is reduced. At higher excitation powers, the loss follows a logarithmic power dependence, consistent with predictions from the generalized tunneling model (GTM). A model combining the discrete TLS ensemble with the GTM is proposed and matches the temperature and power dependence of the measured internal loss of the resonator with reasonable parameters.
Measuring the internal quality factor of coplanar waveguide superconducting resonators is an established method of determining small losses in superconducting devices. Often, resonator losses are attributed to two-level system (TLS) defects using a power dependent model for the quality factor. However, excess non-equilibrium quasiparticles can also limit the quality factor of superconducting resonators. Here, a two-temperature, power and temperature dependent model is used to evaluate resonator losses for titanium nitride and aluminum coplanar waveguide resonators with loss tangents of 10−5–10−6. This model enables a set of parameters to describe both the internal quality factor and fractional frequency shift of the resonator across a broad range of average cavity photon numbers, from 1 to 106, and temperatures between those limited by the experimental apparatus near 50 mK and thermal quasiparticle dominated. The presented model also offers potential insight into observing the temperature and power dependence of TLS–TLS interactions in these resonators.
The complex conductivity of a superconducting thin film is related to the quasiparticle density, which depends on the physical temperature and can also be modified by external pair breaking with photons and phonons. This relationship forms the underlying operating principle of Kinetic Inductance Detectors (KIDs), where the detection threshold is governed by the superconducting energy gap. We investigate the electromagnetic properties of thin-film aluminum that is proximitized with either a normal metal layer of copper or a superconducting layer with a lowerTCT_{C}TC​, such as iridium, in order to extend the operating range of KIDs. Using the Usadel equations along with the Nam expressions for complex conductivity, we calculate the density of states and the complex conductivity of the resulting bilayers to understand the dependence of the pair breaking threshold, surface impedance, and intrinsic quality factor of superconducting bilayers on the relative film thicknesses. The calculations and analyses provide theoretical insights in designing aluminum-based bilayer kinetic inductance detectors for detection of microwave photons and athermal phonons at the frequencies well below the pair breaking threshold of a pure aluminum film.
In this thesis I describe work on developing theoretical and numerical models of supercon- ducting thin-film microwave resonators. Superconducting resonators are used in a variety of applications, one of which is as kinetic inductance detectors (KIDs). KIDs are ultra-low noise, highly sensitive, multiplexable detectors, with uses in a wide variety of fields including astrophysics, medical imaging, and particle physics. Resonators are also crucial for supercon- ducting qubit readout, superconducting mixers and parametric amplifiers, and as multiplexers for other devices. The results described in this thesis apply to all thin film resonators, but are primarily described in the context of KIDs. I develop models of how constant absorbed power affects superconducting thin films, driving them out of thermal equilibrium with the bath. Using the Chang & Scalapino equations, I calculate numerically the steady-state quasiparticle and phonon distributions for various sources of power (sub-gap and above-gap photons and phonons, single frequency and broadband). Many new results emerge, a few of which are: the quasiparticle heating effects of microwave power, explaining the experimentally measured saturation of resonator performance; the frequency dependence of the quasiparticle generation efficiency in the sub-mm wavelength range; and the importance of phonon trapping in thin films at low temperatures. I then use these nonequilibrium results in higher-level device models. Starting from a generic framework for resonators, I present and implement a model of a KID with variable thermal isolation. I calculate the effects of quasiparticle heating on both the large-signal and small-signal behaviour, highlighting the effects of electrothermal feedback caused by readout power. Electrothermal feedback is shown to be able to increase or decrease the magnitude and bandwidth of the responsivity and noise, depending on the operating point. Finally, I propose an experimental measurement of quasiparticle heating effects in a new device – a four-port ring resonator. In such a device, unlike in the standard two-port resonator, the device can be heated and read out independently. I develop detailed models for the thermal and electrical behaviour of these devices, and suggest a scheme by which the quasiparticle heating effects of microwave power, predicted in this thesis, can be measured.
The objective of this thesis is to evaluate a generic process for fabrication and characterization of the Superconductive coplanar waveguide (CPW) resonators. Superconductive CPW resonators with various lengths and shapes are designed to investigate their electrical and magnetic properties as well as resonance properties and sensitivities. In the first part of thesis, two different models are introduced in order to estimate the nonlinear kinetic inductance of a superconducting CPW resonator. The first model is based on Bean critical-state model and the second one is based on current dependence of London penetration depth. The existence of a shift in resonant frequency of Superconductive CPW resonator caused by a non-linear kinetic inductance is also shown experimentally. Simulations were carried out to estimate the nonlinear kinetic inductance due to the self- induced magnetic field penetration. The rest of the thesis is concerned with development of very smooth Aluminum (Al) thin films with RMS (Root Mean Square) roughness 1~nm and CAD (Computer Aid Design) of superconductive CPW resonators. Experimental investigation of a generic fabrication technique for superconductive CPW resonator is carried out. Many resonators are fabricated with different design parameters, such as centerline or gap width, film thickness and gap capacitors length. The fabrication process is described in detail. Electron Beam Lithography is used to fabricate Nb and Al CPW resonators which are coupled to outer conductors via gap capacitors. We have fabricated GHz frequency CPW resonators with quality factors, Q up 5X10^5.