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arXiv:2412.01503 · Physical Review Letters

Phase Transitions and Remnants of Fractionalization at Finite Temperature in the Triangular Lattice Quantum Loop Model

Xiaoxue Ran, Sylvain Capponi, Junchen Rong, Fabien Alet, Zi Yang Meng

Published Aug 27, 2025• 1 citation
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Abstract

The quantum loop and dimer models are archetypal correlated systems with local constraints. With natural foundations in statistical mechanics, they are of direct relevance to various important physical concepts and systems, such as topological order, lattice gauge theories, geometric frustrations, or more recently Rydberg array quantum simulators. However, how the thermal fluctuations interact with constraints has not been explored in the important class of nonbipartite geometries. Here we study, via unbiased quantum Monte Carlo simulations and field theoretical analysis, the finite-temperature phase diagram of the quantum loop model on the triangular lattice. We discover that the recently identified, "hidden" vison plaquette (VP) quantum crystal [X. Ran et al., Hidden orders and phase transitions for the fully packed quantum loop model on the triangular lattice, Commun. Phys. 7, 207 (2024)CMPYEL0868-316610.1038/s42005-024-01680-z] experiences a finite-temperature continuous transition, which smoothly connects to the (2+1)d Cubic* quantum critical point separating the VP and Z_{2} quantum spin liquid phases. This finite-temperature phase transition acquires a unique property of "remnants of fractionalization" at finite temperature, in that, both the cubic order parameter-the plaquette loop resonance-and its constituent-the vison field-exhibit independent criticality signatures. This phase transition is connected to a three-state Potts transition between the lattice nematic phase and the high-temperature disordered phase. We discuss the relevance of our results for current experiments on quantum simulation platforms.

DOI
10.1103/tp8x-dscx

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The quantum loop and dimer models are archetypal correlated systems with local constraints. With natural foundations in statistical mechanics, they are of direct relevance to various important physical concepts and systems, such as topological order, lattice gauge theories, geometric frustrations, or more recently Rydberg array quantum simulators. However, how the thermal fluctuations interact with constraints has not been explored in the important class of nonbipartite geometries. Here we study, via unbiased quantum Monte Carlo simulations and field theoretical analysis, the finite-temperature phase diagram of the quantum loop model on the triangular lattice. We discover that the recently identified, "hidden" vison plaquette (VP) quantum crystal [X. Ran et al., Hidden orders and phase transitions for the fully packed quantum loop model on the triangular lattice, Commun. Phys. 7, 207 (2024)CMPYEL0868-316610.1038/s42005-024-01680-z] experiences a finite-temperature continuous transition, which smoothly connects to the (2+1)d Cubic* quantum critical point separating the VP and Z_{2} quantum spin liquid phases. This finite-temperature phase transition acquires a unique property of "remnants of fractionalization" at finite temperature, in that, both the cubic order parameter-the plaquette loop resonance-and its constituent-the vison field-exhibit independent criticality signatures. This phase transition is connected to a three-state Potts transition between the lattice nematic phase and the high-temperature disordered phase. We discuss the relevance of our results for current experiments on quantum simulation platforms.
Abstract Quantum loop and dimer models are prototypical correlated systems with local constraints, which are not only intimately connected to lattice gauge theories and topological orders but are also widely applicable to the broad research areas of quantum materials and quantum simulation. Employing our sweeping cluster quantum Monte Carlo algorithm, we reveal the complete phase diagram of the triangular-lattice fully packed quantum loop model. Apart from the known lattice nematic (LN) solid and the even Z2{{\mathbb{Z}}}_{2}Z2​ Z 2 quantum spin liquid (QSL) phases, we discover a hidden vison plaquette (VP) phase, which had been overlooked and misinterpreted as a QSL for more than a decade. Moreover, the VP-to-QSL continuous transition belongs to the (2 + 1)D cubic* universality class, which offers a lattice realization of the (fractionalized) cubic fixed point that had long been considered as irrelevant towards the O(3) symmetry until corrected recently by conformal bootstrap calculations. Our results are therefore of relevance to recent developments in both experiments and theory, and facilitate further investigations of hidden phases and transitions.
Quantum loop and dimer models are archetypal examples of correlated systems with local constraints. Obtaining generic solutions for these models is difficult due to the lack of controlled methods to solve them in the thermodynamic limit. Nevertheless, these solutions are of immediate relevance to both statistical and quantum field theories, as well as the rapidly growing experiments in Rydberg atom arrays and quantum moir\'e materials, where the interplay between correlation and local constraints gives rise to a plethora of novel phenomena. In a recent work [X. Ran et al., arXiv:2205.04472], it was found through sweeping cluster quantum Monte Carlo (QMC) simulations and field theory analysis that the triangular lattice quantum loop model (QLM) hosts a rich ground-state phase diagram with lattice nematic, vison plaquette (VP) crystals, and the Z2{\mathbb{Z}}_{2}Z2​ quantum spin liquid (QSL) close to the Rokhsar-Kivelson point. Here, we focus on the continuous quantum critical point separating the VP and QSL phases and demonstrate via both static and dynamic probes in QMC simulations that this transition is of the (2+12+12+1)D cubic* universality. In this transition, the fractionalized visons in QSL condense to give rise to the crystalline VP phase, while leaving their trace in the anomalously large anomalous dimension exponent and pronounced continua in the dimer and vison spectra compared with those at the conventional cubic or O(3) quantum critical points.
The quantum dimer and loop models attract great attention, partially because the fundamental importance in the phases and phase transitions emerging in these prototypical constrained systems, and partially due to their intimate relevance toward the on-going experiments on Rydberg atom arrays in which the blockade mechanism naturally enforces the local constraint. Here we show, by means of the sweeping cluster quantum Monte Carlo method, the complete ground state phase diagram of the fully packed quantum loop model on the square lattice. We find between the lattice nematic (LN) phase with strong dimer attraction and the staggered phase (SP) with strong dimer repulsion, there emerges a resonating plaquette (RP) phase with off-diagonal translational symmetry breaking. Such a quantum phase is separated from the LN via a first order transition and from the SP by the famous Rokhsar-Kivelson point. Our renormalization group analysis reveals the different flow directions, fully consistent with the order parameter histogram in Monte Carlo simulations. The realization and implication of our phase diagram in Rydberg experiments are proposed.
Recent work [Kundu, Damle, Phys. Rev. X 15, 011018 (2025)] has demonstrated that a class of S=1S=1S=1 kagome lattice antiferromagnets with competing anisotropies can exhibit unusual low-temperature behavior that is best described in terms of the statistical mechanics of an interesting interpolation between the fully-packed dimer model and the fully-packed loop model on the bipartite honeycomb lattice. On this and other bipartite lattices in two and three dimension, such fully-packed dimer-loop models generically have two distinct power-law correlated Coulomb phases, both of which admit a low-energy description in terms of a fluctuating divergence-free polarization vector field [Phys. Rev. X 15, 011018 (2025); arXiv:2510.11607]. The transition between these phases corresponds to a confinement transition for the Z2Z_2Z2​ part of the corresponding U(1)U(1)U(1) flux [Phys. Rev. X 15, 011018 (2025); arXiv:2510.11607]. Here we demonstrate that a variant of such a topological confinement transition can also exist in dimer-loop models on non-bipartite lattices such as the kagome and triangular lattices although the low-energy description does not feature any conserved U(1)U(1)U(1) flux. In these non-bipartite dimer-loop models, both phases are short-range correlated liquids, and the topological distinction between them is in terms of a Z2Z_2Z2​-valued winding number instead of the flux of a divergence-free polarization field. In spite of this key difference, this transition appears to be in the same Ising universality class as the analogous transition of the bipartite dimer-loop models. These kagome and triangular lattice dimer-loop models correspond respectively to the low-energy limit of a class of S=1S=1S=1 antiferromagnets with competing anisotropies on the ruby lattice comprising a corner-sharing arrangement of fully-frustrated squares and a lattice of corner-sharing fully-frustrated hexagons.
In the field of frustrated magnetism, Kitaev models provide prototypical examples of exactly solvable quantum spin liquids, in which the spin degrees of freedom fractionalize into Majorana fermions coupled to an emergent Z2 gauge field. While the ground states of these models are already well understood as exhibiting different kinds of Majorana (semi)metals, it has still been an open task to achieve a detailed understanding of the thermodynamics, and, namely, the low-temperature ordering of the gauge field into different Z2 flux configurations. In this thesis, we investigate the thermodynamics of Kitaev systems in two and three spatial dimensions with sign-problem-free quantum Monte Carlo simulations. In a first study of elementary 3D Kitaev models, we verify that the ground state Z2 flux sectors of these systems are entirely determined by their elementary plaquette length – a result which shows the validity of Lieb’s theorem for lattice geometries which lack the geometric requirements for its proof. We closely investigate the low-temperature phase transition associated with gauge-ordering, which is a particular realization of an inverted Ising phase transition, as it occurs in general lattice Z2 gauge theories. Our results corroborate the understanding of this transition as separating different regimes in terms of vison-loop excitations, by showing a clear correlation between the critical temperature and the vison gap. We also introduce the concept of “gauge frustration”, which, for a particular 3D Kitaev model, leads to the suppression of the phase transition and a more complex physical behavior at low temperatures. A second quantum Monte Carlo study focuses on a generalized 2D Kitaev model on a five-coordinated lattice system. Here, the gauge ordering is accompanied by the spontaneous breaking of time-reversal symmetry, a scenario which not only allows for a variety of topological ground states, but also for the occurrence of a phase transition in two spatial dimensions. We show that this model exhibits such a transition at a particularly high temperature scale. Moreover, the system possesses a number of phases where the Z2 fluxes are only partially ordered.
In the field of frustrated magnetism, Kitaev models provide a unique framework to study the phenomena of spin fractionalization and emergent lattice gauge theories in two and three spatial dimensions. Their ground states are quantum spin liquids, which can typically be described in terms of a Majorana band structure and an ordering of the underlying Z2{\mathbb{Z}}_{2}Z2​ gauge structure. Here we provide a comprehensive classification of the ``gauge physics'' of a family of elementary three-dimensional Kitaev models, discussing how their thermodynamics and ground state order depends on the underlying lattice geometry. Using large-scale, sign-free quantum Monte Carlo simulations we show that the ground-state gauge order can generally be understood in terms of the length of elementary plaquettes---a result which extends the applicability of Lieb's theorem to lattice geometries beyond its original scope. At finite temperatures, the proliferation of (gapped) vison excitations destroys the gauge order at a critical temperature scale, which we show to correlate with the size of vison gap for the family of three-dimensional Kitaev models. We also discuss two notable exceptions where the lattice structure gives rise to ``gauge frustration'' or intertwines the gauge ordering with time-reversal symmetry breaking. In a more general context, the thermodynamic gauge transitions in such 3D Kitaev models are one of the most natural settings for phase transitions beyond the standard Landau-Ginzburg-Wilson paradigm.