An Improved Bound on Nonlinear Quantum Mechanics using a Cryogenic Radio Frequency Experiment
Oleksandr Melnychuk, Bianca Giaccone, Nicholas Bornman, Raphael Cervantes, Anna Grassellino, Roni Harnik, David E. Kaplan, Geev Nahal, Roman Pilipenko, Sam Posen, Surjeet Rajendran, Alexander O. Sushkov
There are strong arguments that quantum mechanics may be nonlinear in its dynamics. A discovery of nonlinearity would hint at a novel understanding of the interplay between gravity and quantum field theory, for example. As such, experiments searching for potential nonlinear effects in the electromagnetic sector are important. Here we outline such an experiment, consisting of a stream of random bits (which were generated using Rigetti's Aspen-M-3 chip) as input to an RF signal generator coupled to a cryogenic detector. Projective measurements of the qubit state, which is originally prepared in an equal superposition, serve as the random binary output of a signal generator. Thereafter, spectral analysis of the RF detector would yield a detectable excess signal predicted to arise from such a nonlinear effect. A comparison between the projective measurements of the quantum bits vs the classical baseline showed no power excess. This sets a new limit on the electromagnetic nonlinearity parameter $|ε| \lessapprox 1.15 \times 10^{-12}$, at a 90.0% confidence level. This is the most stringent limit on nonlinear quantum mechanics thus far and an improvement by nearly a factor of 50 over the previous experimental limit.
There are strong arguments that quantum mechanics may be nonlinear in its dynamics. A discovery of nonlinearity would hint at a novel understanding of the interplay between gravity and quantum field theory, for example. As such, experiments searching for potential nonlinear effects in the electromagnetic sector are important. Here we outline such an experiment, consisting of a stream of random bits (which were generated using Rigetti's Aspen-M-3 chip) as input to an RF signal generator coupled to a cryogenic detector. Projective measurements of the qubit state, which is originally prepared in an equal superposition, serve as the random binary output of a signal generator. Thereafter, spectral analysis of the RF detector would yield a detectable excess signal predicted to arise from such a nonlinear effect. A comparison between the projective measurements of the quantum bits vs the classical baseline showed no power excess. This sets a new limit on the electromagnetic nonlinearity parameter ∣ε∣⪅1.15×10−12, at a 90.0% confidence level. This is the most stringent limit on nonlinear quantum mechanics thus far and an improvement by nearly a factor of 50 over the previous experimental limit.
Linear time evolution is one of the fundamental postulates of quantum theory. Past theoretical attempts to introduce nonlinearity into quantum evolution have violated causality. However, a recent theory has introduced nonlinear state-dependent terms in quantum field theory, preserving causality [D. E. Kaplan and S. Rajendran, Phys. Rev. D 105, 055002 (2022)PRVDAQ2470-001010.1103/PhysRevD.105.055002]. We report the results of an experiment that searches for such terms. Our approach, inspired by the Everett many-worlds interpretation of quantum theory, correlates a binary macroscopic classical voltage with the outcome of a projective measurement of a quantum bit, prepared in a coherent superposition state. Measurement results are recorded in a bit string, which is used to control a voltage switch. Presence of a nonzero voltage reading in cases of no applied voltage is the experimental signature of a nonlinear state-dependent shift of the electromagnetic field operator. We implement blinded measurement and data analysis with three control bit strings. Control of systematic effects is realized by producing one of the control bit strings with a classical random-bit generator. The other two bit strings are generated by measurements performed on a superconducting qubit in an IBM Quantum processor and on a ^{15}N nuclear spin in a nitrogen-vacancy center in diamond. Our measurements find no evidence for electromagnetic quantum state-dependent nonlinearity. We set a bound on the parameter that quantifies this nonlinearity |ε_{γ}|<4.7×10^{-11}, at 90% confidence level.
Having accurate gate generation is essential for precise control of a quantum system. The generated gate usually suffers from linear and nonlinear distortion. Previous works have demonstrated how to use a qubit to correct linear frequency distortions but have not commented on how to handle nonlinear distortions. This is an important issue as we show that nonlinear amplitude distortions from the RF electronics can affect Rabi pulses by as much as 10%. We present work that demonstrates how a transmon qubit can be used as a highly sensitive cryogenic detector to characterize these nonlinear amplitude distortions. We show that a correction can drive these errors down to <1% over a 700 MHz range. This correction technique provides a method to minimize the effects of signal distortions and can be easily applied to broadband control pulses to produce higher fidelity arbitrary quantum gates.
Recent advancements in quantum technologies and advanced detection experiments have underscored the pressing need for the detection of exceedingly weak signals within the microwave frequency spectrum. Addressing this challenge, the Josephson Traveling Wave Parametric Amplifier (JTWPA) has been proposed as a cryogenic front-end amplifier capable of approaching the quantum noise limit while providing a relevant bandwidth. This research is centered on a comprehensive numerical investigation of the JTWPA, without resorting to simplifications regarding the nonlinearity of the essential components. Specifically, this study focuses on a thorough examination of the system, characterized by coupled nonlinear differential equations representing all components of the device. Proper input and output signals at the device's boundaries are considered. The analysis of the output signals undergoing the parametric amplification process involves a detailed exploration of phase-space dynamics and Fourier spectral analysis of the output voltage. This study is conducted while considering the parameters ruling the response of the device under pump and signal excitations. In addition to the expected signal amplification, the findings reveal that the nonlinear nature of the system can give rise to unforeseen phenomena, depending on the system's operational conditions, which include: the generation of pump tone harmonics, modulation of the signal gain, and incommensurate frequency generation—effects that are not easily accommodated by simplistic linearized approaches.
We add nonlinear and state-dependent terms to quantum field theory. We show that the resulting low-energy theory, nonlinear quantum mechanics, is causal, preserves probability and permits a consistent description of the process of measurement. We explore the consequences of such terms and show that nonlinear quantum effects can be observed in macroscopic systems even in the presence of decoherence. We find that current experimental bounds on these nonlinearities are weak and propose several experimental methods to significantly probe these effects. The locally exploitable effects of these nonlinearities have enormous technological implications. For example, they would allow large-scale parallelization of computing (in fact, any other effort) and enable quantum sensing beyond the standard quantum limit. We also expose a fundamental vulnerability of any nonlinear modification of quantum mechanics---these modifications are highly sensitive to cosmic history and their locally exploitable effects can dynamically disappear if the observed universe has a tiny overlap with the overall quantum state of the universe, as is predicted in conventional inflationary cosmology. We identify observables that should persist in this case and discuss opportunities to detect them in cosmic ray experiments, tests of strong field general relativity and current probes of the equation of state of the universe. Nonlinear quantum mechanics also enables novel gravitational phenomena and may open new directions to solve the black hole information problem and to uncover the theory underlying quantum field theory and gravitation.
Advances in the field of nanoscale quantum engineered systems depend crucially on the ability to make quantum limited measurements. Current capabilities are limited by technical and quantum noise introduced by devices used for transduction and amplification of the inherently small signals of interest. Many experimental implementations, including nano-mechanical systems, solid-state quantum bits (qubits), and circuit quantum-electrodynamics (c-QED) devices, utilize transmitted or reflected microwave signals to measure the field quadratures of signals composed of few photons. Traditional low-noise cryogenic HEMT amplifiers provide an unsatisfactory solution to this quantum measurement problem because the targeted signal is often much smaller than the added noise. In principle, c-QED devices can be used for quantum-limited amplification, particularly as a parametric amplifier (PA). An ideal parametric amplifier should amplify signals without introducing additional noise, which would allow for the attainment of quantum feedback algorithms. In this thesis, I describe the characterization of a c-QED device, known as a tunable resonator, with the goal of quantifying its limits when used as a parametric amplifier. Tunable resonators are currently being used as PAs in quantum limited experiments, however, some of the underlying dynamics of these devices have not yet been fully characterized. I investigated the frequency, internal loss, power dependent frequency shift (nonlinearity) of a tunable microwave co-planar waveguide (CPW) resonator as a function of external magnetic flux biasing, which changes the effective length of the resonator. By looking at multiple samples with different design parameters, I observed that nonlinear damping is inherent to this device. Nonlinear damping had previously been observed but not described in sufficient detail to provide insight into its origins, which may explain some underlying dynamics of the tunable resonator. My measurements of the nonlinear damping shows that at larger flux biases, the nonlinear damping dominates linear internal losses and represent the main contribution to the total internal loss rate. I then operated this device as a parametric oscillator (PO) and found that the nonlinear damping and large Kerr (or quartic) nonlinearity likely cause an increase in the above-threshold switching rates between π-phase shifted steady states, which in turn may be associated with anomalous above-threshold squeezing in these devices. The results of my thesis show that nonlinear damping is present in these devices and affects performance in them dearly. This result is important for future work in PAs as improved understanding of the nonlinear damping will enable engineering of a device which can act as a PA with maximal gain and minimum noise.
The recent developments in quantum technologies, as well as advanced detection experiments, have raised the need to detect extremely weak signals in the microwave frequency spectrum. To this aim, the Josephson travelling wave parametric amplifier, a device capable of reaching the quantum noise limit while providing a wide bandwidth, has been proposed as a suitable cryogenic front-end amplifier. This work deals with the numerical study of a Josephson travelling wave parametric amplifier, without approximations regarding the nonlinearity of the key elements. In particular, we focus on the investigation of the system of coupled nonlinear differential equations representing all the cells of the Josephson travelling wave parametric amplifier, with proper input and output signals at the boundaries. The investigation of the output signals generated by the parametric amplification process explores the phase-space and the Fourier spectral analysis of the output voltage, as a function of the parameters describing the pump and signal tones that excite the device. Beside the expected behavior, i.e., the signal amplification, we show that, depending on the system operation, unwanted effects (such as pump tone harmonics, incommensurate frequency generation, and noise rise), which are not accounted for in simple linearized approaches, can be generated in the whole nonlinear system.