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arXiv:2411.08964

Many-Body Photon Blockade and Quantum Light Generation from Cavity Quantum Materials

Benjamin Kass, Spenser Talkington, Ajit Srivastava, Martin Claassen

Published Nov 13, 2024• 0 citations
arXivHTMLPDF

Abstract

The strong coupling regime of photons and quantum materials inside optical cavities has emerged as a promising environment for manipulating states of matter with light. Here, in turn, we show that photons bear witness to cavity quantum-electrodynamical modifications of the material, leading to profoundly non-classical properties of light passing through the cavity. By generalizing quantum-optical input-output relations to correlated quantum materials, we study the second-order photon coherence g2(t) and demonstrate that antibunching of transmitted photons serves as direct evidence of light-induced changes to the cavity-embedded material. We show that materials near a quantum critical point can realize a collective many-body photon blockade, enabling the generation of single photons or Einstein-Podolsky-Rosen pairs via leveraging strong matter fluctuations. Our findings provide new routes for interrogating and harnessing cavity-embedded quantum materials as quantum light sources, as a resource for photon-based computation and quantum sensing.

DOI
10.48550/arxiv.2411.08964

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The strong coupling regime of photons and quantum materials inside optical cavities has emerged as a promising environment for manipulating states of matter with light. Here, in turn, we show that photons bear witness to cavity quantum-electrodynamical modifications of the material, leading to profoundly non-classical properties of light passing through the cavity. By generalizing quantum-optical input-output relations to correlated quantum materials, we study the second-order photon coherence g2(t) and demonstrate that antibunching of transmitted photons serves as direct evidence of light-induced changes to the cavity-embedded material. We show that materials near a quantum critical point can realize a collective many-body photon blockade, enabling the generation of single photons or Einstein-Podolsky-Rosen pairs via leveraging strong matter fluctuations. Our findings provide new routes for interrogating and harnessing cavity-embedded quantum materials as quantum light sources, as a resource for photon-based computation and quantum sensing.
Analogous to Coulomb blockade for electrons, photon blockade is a key quantum optical effect in which the presence of one photon prevents the transmission of subsequent ones through a nonlinear medium. Beyond its fundamental interest, photon and multi-photon blockade are actively studied as mechanisms for generating technologically-relevant quantum states of light. Although photon blockade typically requires achieving strong light-matter coupling, increasing the number of atoms fails to enhance antibunching. Here, we analyze the optical transmission properties of a quantum resonator that embeds a two-photon-coupled ensemble of emitters, combining an approximate analytical approach with full quantum numerical simulations. We show that when light and matter are coupled via a two-photon interaction, both single- and multi-photon blockade can benefit from a collective enhancement. We propose different driving schemes in which the second or third-order correlation functions are strongly suppressed with increasing atom number. Differently from established methods, this collective enhancement of non-classical properties occurs with unitary transmission and is ultimately constrained only by decoherence. This demonstrates that collective two-photon couplings are a powerful mechanism for realizing photon blockade even in platforms where individual strong coupling is not achievable.
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The antibunching effect generated in a cavity containing first a single two-level atomic system and then two identical atoms is explored for off-resonant interactions, in strong- and weak-coupling regimes. The cavity is driven by coherent and squeezed sources. Using the second-order correlation function analytically derived in the weak-excitation regime, we show that squeezed light achieves and improves strong antibunching, leading to a photon blockade. This enhancement is due to a destructive quantum interference mechanism induced by the nonclassical light, creating a supplementary transition pathway. The best effect is obtained for equal frequency detunings in the strong-coupling regime. More interestingly, our investigation reveals that the two-atom-cavity system can further improve the antibunching effect compared to the single-atom cavity. It turns out that the additional couplings appearing in the cavity due to the implementation of the two atoms, combined with the squeezed light, could substantially enhance the photon-blockade effect.
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A quantum critical point develops when matter undergoes a continuous transformation between distinct ground states at absolute zero. It hosts pronounced quantum fluctuations, which render the system highly susceptible to external perturbations. While light-matter coupling has rapidly moved forward as a means to probe and control quantum materials, the capacity of quantum critical fluctuations in the photon-mediated responses has been largely unexplored. Here we advance the notion that directly coupling a quantum critical mode to a quantized cavity field dramatically facilitates the realization of the elusive superradiant phase transition in equilibrium, circumventing at once the key obstacles that have prevented its attainment in spite of decades of pursuit. The superradiant phase transition develops far below the ultrastrong regime of light-matter couplings, and the transition is accompanied by the light-matter hybrid system showing strongly enhanced intrinsic squeezing and amplified quantum Fisher information. We also identify candidate cavity quantum materials platforms for validating the proposed effect. Our findings suggest a general principle by which quantum criticality amplifies the response to cavity photons. They also demonstrate that cavity coupling accesses the elevated quantum entanglement of the underlying matter at quantum criticality, thereby pointing to a pathway towards realizing the potential of highly collective quantum materials to expand the capacities of quantum information science. Quantum critical systems host strong fluctuations that can enhance their response to external fields. Here the authors show that directly coupling cavity-bound photons to a quantum critical material produces highly correlated light-matter states at modest light-matter couplings that access the matter’s enhanced quantum entanglement.
The on-chip generation of nonclassical states of light is a key requirement for future optical quantum hardware. In solid-state cavity quantum electrodynamics, such nonclassical light can be generated from self-assembled quantum dots strongly coupled to photonic crystal cavities. Their anharmonic strong light-matter interaction results in large optical nonlinearities at the single photon level, where the admission of a single photon into the cavity may enhance (photon tunneling) or diminish (photon blockade) the probability for a second photon to enter the cavity. Here, we demonstrate that detuning the cavity and quantum-dot resonances enables the generation of high-purity nonclassical light from strongly coupled systems. For specific detunings we show that not only the purity but also the efficiency of single-photon generation increases significantly, making high-quality single-photon generation by photon blockade possible with current state-of-the-art samples.