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arXiv:2410.24047 · Physical Review A

Impact of micromotion and field-axis misalignment on the excitation of Rydberg states of ions in a Paul trap

Wilson S. Martins, Joseph W. P. Wilkinson, Markus Hennrich, Igor Lesanovsky

Published Apr 7, 2025• 3 citations
arXivHTMLPDF

Abstract

The authors theoretically investigate how micromotion influences the transition energies and laser excitation probabilities of Rydberg states of ions confined within Paul traps. The results could help understand the conditions to combine trapped ions with Rydberg interactions as a platform for quantum simulation.
DOI
10.1103/physreva.111.043106

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We report on the observation of interactions between ultracold Rydberg atoms and ions in a Paul trap. The rate of observed inelastic collisions, which manifest themselves as charge transfer between the Rydberg atoms and ions, exceeds that of Langevin collisions for ground state atoms by about 3 orders of magnitude. This indicates a huge increase in interaction strength. We study the effect of the vacant Paul trap's electric fields on the Rydberg excitation spectra. To quantitatively describe the exhibited shape of the ion loss spectra, we need to include the ion-induced Stark shift on the Rydberg atoms. Furthermore, we demonstrate Rydberg excitation on a dipole-forbidden transition with the aid of the electric field of a single trapped ion. Our results confirm that interactions between ultracold atoms and trapped ions can be controlled by laser coupling to Rydberg states. Adding dynamic Rydberg dressing may allow for the creation of spin-spin interactions between atoms and ions, and the elimination of collisional heating due to ionic micromotion in atom-ion mixtures.
Trapped Rydberg ions are a promising new system for quantum information processing. They have the potential to join the precise quantum operations of trapped ions and the strong, long-range interactions between Rydberg atoms. Technically, the ion trap will need to stay active while exciting the ions into the Rydberg state, else the strong Coulomb repulsion will quickly push the ions apart. Thus, a thorough understanding of the trap effects on Rydberg ions is essential for future applications. Here we report the observation of two fundamental trap effects. First, we investigate the interaction of the Rydberg electron with the quadrupolar electric trapping field. This effect leads to Floquet sidebands in the spectroscopy of Rydberg D-states whereas Rydberg S-states are unaffected due to their symmetry. Second, we report on the modified trapping potential in the Rydberg state compared to the ground state which results from the strong polarizability of the Rydberg ion. We observe the resultant energy shifts as a line broadening which can be suppressed by cooling the ion to the motional ground state in the directions orthogonal to the excitation laser.
Trapped Rydberg ions are a promising new system for quantum information processing. They have the potential to join the precise quantum operations of trapped ions and the strong, long-range interactions between Rydberg atoms. Combining the two systems is not at all straightforward. Rydberg atoms are severely affected by electric fields which may cause Stark shifts and field ionization, while electric fields are used to trap ions. Thus, a thorough understanding of the physical properties of Rydberg ions due to the trapping electric fields is essential for future applications. Here we report the observation of two fundamental trap effects. First, we investigate the interaction of the Rydberg electron with the trapping electric quadrupole fields which leads to Floquet sidebands in the excitation spectra. Second, we report on the modified trapping potential in the Rydberg state compared to the ground state which results from the strong polarizability of the Rydberg ion. By controlling both effects we observe resonance lines close to their natural linewidth demonstrating an unprecedented level of control of this novel quantum platform.
Usually the influence of the quadratic Stark effect on an ion's trapping potential is minuscule and only needs to be considered in atomic clock experiments. In this work we excite a trapped ion to a Rydberg state with polarizability ∼8 orders of magnitude higher than a low-lying electronic state; we find that the highly polarizable ion experiences a vastly different trapping potential owing to the Stark effect. We observe changes in trap stiffness, equilibrium position, and minimum potential, which can be tuned using the trapping electric fields. These effects lie at the heart of several proposed studies, including a high-fidelity submicrosecond entangling operation; in addition we demonstrate these effects may be used to minimize ion micromotion. Mitigation of Stark effects is important for coherent control of Rydberg ions; we illustrate this by carrying out the first Rabi oscillations between a low-lying electronic state and a Rydberg state of an ion.
Laser cooling of a single trapped ion in a Paul trap is discussed theoretically in the Lamb-Dicke limit, with full consideration of the time dependence of the trapping potential. Resulting mean kinetic energies are defined as time averages over one period of the micromotion and are compared with final temperatures expected from the laser-cooling treatment with harmonic traps. For laser-atom detunings close to the micromotion frequency the results differ significantly from those expected for a harmonic trap potential. A physical interpretation is given and simple formulas are derived for the strong confinement case.
We present a detailed theoretical and conceptual study of a planned experiment to excite Rydberg states of ions trapped in a Paul trap. The ultimate goal is to exploit the strong state-dependent interactions between Rydberg ions to implement quantum information processing protocols and simulate the dynamics of strongly interacting spin systems. We highlight the promise of this approach when combining the high degree of control and readout of quantum states in trapped ion crystals with the novel and fast gate schemes based on interacting giant Rydberg atomic dipole moments. We discuss anticipated theoretical and experimental challenges on the way to its realization.