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arXiv:2409.07428

Quantum trajectories and output field properties for two-photon input field

Anita Magdalena Dąbrowska, Gniewomir Sarbicki

Published Sep 11, 2024• 0 citations
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Abstract

The excitation of atomic and molecular systems by propagating light in a two-photon state within the Wigner-Weisskopf approximation has been described using stochastic tools. The problem of a stochastic evolution of the quantum system, depending on the results of the measurement of the output field, was formulated and solved making use of the model of repeated interactions and measurement. We defined the discrete in-time interaction between the quantum system and its environment being the electromagnetic field approximated by a chain or chains of harmonic oscillators. We determined analytical formulae for quantum trajectories associated with one-dimensional and two-dimensional counting processes, corresponding respectively to unidirectional or bidirectional input field prepared in the two-photon states. We derived the formulae for the exclusive probability densities of photon counts that allow us to completely characterize the photon statistics of the output field. Finally, we showed how to apply the quantum trajectories to obtain the formula for the probability of the two-photon absorption for a three-level atom in a ladder configuration. The paper also includes a discussion on the optimal two-photon state that maximizes the two-photon absorption probability.

DOI
10.48550/arxiv.2409.07428

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The excitation of atomic and molecular systems by propagating light in a two-photon state within the Wigner-Weisskopf approximation has been described using stochastic tools. The problem of a stochastic evolution of the quantum system, depending on the results of the measurement of the output field, was formulated and solved making use of the model of repeated interactions and measurement. We defined the discrete in-time interaction between the quantum system and its environment being the electromagnetic field approximated by a chain or chains of harmonic oscillators. We determined analytical formulae for quantum trajectories associated with one-dimensional and two-dimensional counting processes, corresponding respectively to unidirectional or bidirectional input field prepared in the two-photon states. We derived the formulae for the exclusive probability densities of photon counts that allow us to completely characterize the photon statistics of the output field. Finally, we showed how to apply the quantum trajectories to obtain the formula for the probability of the two-photon absorption for a three-level atom in a ladder configuration. The paper also includes a discussion on the optimal two-photon state that maximizes the two-photon absorption probability.
Abstract The excitation of atomic and molecular systems by propagating light in a two-photon state within the Wigner–Weisskopf approximation has been described using stochastic tools. The problem of a stochastic evolution of the quantum system, depending on the results of the measurement of the output field, was formulated and solved making use of the model of repeated interactions and measurement. We defined the discrete in-time interaction between the quantum system and its environment being the electromagnetic field approximated by a chain or chains of harmonic oscillators. We determined analytical formulae for quantum trajectories associated with one-dimensional and two-dimensional counting processes, corresponding respectively to unidirectional or bidirectional input field prepared in the two-photon states. We derived the formulae for the exclusive probability densities of photon counts that allow us to completely characterize the photon statistics of the output field. Finally, we showed how to apply the quantum trajectories to obtain the formula for the probability of the two-photon absorption for a three-level atom in a ladder configuration. The paper also includes a discussion on the optimal two-photon state that maximizes the two-photon absorption probability.
In this paper, photon-counting statistics for an output field of a single-photon wave packet interacting with a quantum system was derived. The problem was formulated using a collision model with a bidirectional field approximated by two sequences of qubits. It was shown that the collision model formulated for the light with the temporal correlations allows deriving formulae for quantum trajectories in an effective and intuitive way. Starting from the discrete in-time evolution of the composed system, we determined the conditional and unconditional evolution of the quantum system, provided a physical interpretation of quantum trajectories, and determined the analytical formulae for the exclusive probability densities for the reflected and transmitted fields. Finally, our results were applied to a two-level atom, and we also determined analytical expressions for probability densities of arrival times of the successive counts.
This work discusses the problem of optimal excitation of a three-level atom of ladder configuration by light in the two-photon state and coherent light carrying an average of two photons. The applied atom-light interaction model is based on the Wigner-Weisskopf approximation. We characterize the properties of the optimal two-photon state that excites an atom perfectly, i.e., with probability equal to one. We find that the spectrotemporal shape of the optimal state of light is determined by the lifetimes of the atomic states, with the degree of photonic entanglement in the optimal state depending on the lifetime ratio. In consequence, two distinct interaction regimes can be identified in which the entanglement of the input state of light has a qualitatively different impact. As the optimal states may be challenging to prepare in general, we compare the results with those obtained for photon pairs of selected experimentally relevant pulse shapes. As these shapes are optimized for maximal atomic excitation probability, the results can be interpreted in terms of the overlap between the optimal and investigated pulse shapes.
Abstract We derive stochastic master equation for a quantum system interacting with an environment prepared in a continuous-mode N -photon state. To determine the conditional evolution of the quantum system depending on continuous in time measurements of the output field the model of repeated interactions and measurements is applied. The environment is defined as an infinite chain of harmonic oscillators which do not interact between themselves and they are prepared initially in an entangled state being a discrete analogue of a continuous-mode N -photon state. We provide not only the quantum trajectories but also the analytical formulae for the whole statistics of the output photons and the solution to the master equation. The solution in the continuous case is represented by a simple diagrammatic technique with very transparent ‘Feynmann rules’. This technique considerably simplifies the structure of the solution and enables one to find physical interpretation for the solution in terms of a few elementary processes.
We investigate the excitation of a three-level ladder-type atom by a unidirectional field with a pair of indistinguishable photons. Starting from an analytical expression for the two-photon absorption probability, we determine the two-photon state that maximizes the population of the upper atomic state at a chosen time and show that in the limit of an infinitely long pulse, perfect excitation is possible. The optimal state is identified as the time-reversed counterpart of the two-photon state emitted in spontaneous cascade decay. We then compare this ideal excitation strategy with experimentally accessible families of states, including symmetrized Gaussian product states, temporally correlated Gaussian states, and coherent pulses. We analyze how the optimal excitation conditions depend on the ratio of atomic decay rates and on the separation of the atomic transition frequencies. For indistinguishable photons, quantum interference may shift the maxima of the marginal spectral distribution away from the atomic resonances and qualitatively modify the optimal excitation strategy. Our results clarify the role of indistinguishability and correlations in two-photon absorption and provide guidance for designing realistic excitation schemes in quantum-optical light-matter interfaces.
Abstract One of the greatest successes in quantum theory, and certainly one of the more important parts for application to devices and applications is the prediction of the emission of light through the quantization of an electromagnetic field. Broadly, this is the field of quantum electrodynamics. In this chapter, we develop the Hamiltonian for the classical electromagnetic field. It is seen that the Hamiltonian for each mode (identified by the k-vector and polarization of the field) of the plane wave electromagnetic field is identical to that of the harmonic oscillator. One unit of energy, ℏω, in a mode is a called a photon. The eigenkets for the system are number states (Fock states). We then consider a two-level system described by a Hamiltonian which couples the two-level quantum system to the quantized electromagnetic field. Using the Weisskopf–Wigner formalism developed in Chapter 14, we solve the equations of motion for the time dependent Schrödinger equation assuming the system starts in the excited state with no radiation present in the vacuum field. The results show the creation of one unit of energy in an electromagnetic mode corresponding to the emission of a photon. The excited state probability decays exponentially with the emission of this photon. We consider the important and special case of such a two-level system but in a cavity restricting the radiation field to a single mode. The Jaynes–Cummings Hamiltonian shows that this system, if started in the excited state, Rabi oscillates with no radiation incident on the system.