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arXiv:2408.15433 · Physical Review A

Decoherence and Brownian motion of a polarizable particle near a medium

Clemens Jakubec, Christopher Jarzynski, Kanu Sinha

Published Sep 18, 2025• 2 citations
arXivHTMLPDF

Abstract

Optically levitated nanoparticles are ideal experimental testbeds for investigating macroscopic superpositions and microscopic thermodynamics. Integrating such levitated nanoparticles with photonic structures can enable strong coupling between their center-of-mass motion and guided photonic modes, facilitating enhanced control and probing of their motion. When coupling a particle to a photonic structure, such as a waveguide, the effects of fluctuations become prominent at nanoscales. In this work, we analyze the classical and quantized center-of-mass motion of a polarizable particle interacting with the fluctuations of the electromagnetic field in the presence of a medium. We derive a position localization master equation for the particle's quantized center of mass, and examine its classical center-of-mass momentum diffusion, elucidating correspondences between classical and quantum Brownian motion of polarizable particles near media. We study the decoherence rate of the particle in the presence of a planar surface as a function of temperature and distance from the surface, comparing it to common sources of decoherence. Our results are pertinent to experiments aimed at preparing levitated nanospheres in macroscopic quantum states and investigating their Brownian dynamics.

DOI
10.1103/6m4t-jm4x

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We study the fluctuation-induced dissipative dynamics of the quantized center-of-mass motion of a polarizable dielectric particle trapped near a surface. The particle's center of mass is treated as an open quantum system coupled to the electromagnetic field acting as its environment, with the resulting system dynamics described by a quantum Brownian motion master equation. The dissipation and decoherence of the particle's center of mass are characterized by the modified spectral density of the electromagnetic field that depends on surface losses and the strength of the classical trap field. Our results are relevant to experiments with levitated dielectric particles near surfaces, illustrating potential ways of mitigating fluctuation-induced decoherence while preparing such systems in macroscopic quantum states.
Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence [1-4]. Quantum control of mechanical motion has been achieved by engineering the radiation pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator [5-8]. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states [9]. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects [10,11], since their trapping potential is fully controllable. In this work, we optically levitate a femto-gram dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its center-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 43%. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales [12,13].
This chapter introduces cavity quantum optomechanics with levitated nanospheres with some emphasis on preparing mesoscopic quantum superpositions and testing collapse models. It is divided into three parts: levitated quantum optomechanics: atoms vs. sphere; decoherence in levitated nanospheres; and wave-packet dynamics: coherence vs. decoherence. It is first shown how the master equation describing the dynamics of a polarizable object in a cavity along the cavity axis and that of the cavity mode is derived. Optical levitation is also discussed. It is then shown how most of the decoherence sources in levitated nanospheres can be cast into a relatively simple master equation describing position localization type of decoherence. Such decoherence tends to suppress the centre-of-mass position coherences. Finally, a discussion of wave-packet dynamics is given, with the motivation of using levitated nanospheres for matter-wave interferometry, that is, to create macroscopic quantum superpositions for testing quantum mechanics in unprecedented parameter regimes.
We analyze the decoherence of a particle's spatial superposition moving along a stationary worldline through the Minkowski vacuum. The particle is modeled via an internal degree of freedom that couples to a scalar field, and an external degree of freedom, i.e., its quantized center-of-mass motion around the stationary worldline. Assuming a separation of time scales between the particle's internal and external dynamics, we first obtain an effective red-shifted polarizability of the particle, characterizing the trajectory-dependent linear response of the internal oscillator to the field. We then derive a quantum Brownian motion master equation for the particle's center of mass, under the Born-Markov approximation, which describes its decoherence in the position basis, as well as, Hamiltonian modifications corresponding to a dispersive potential. The resulting decoherence has two components: (1) arising from a modified field spectrum observed by the particle; and (2) due to a differential time-dilation over the particle's extended spatial wavefunction. For stationary trajectories, both contributions take an effectively thermal form. We evaluate the decoherence rates for two specific cases of hyperbolic and uniform circular motion.
Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence1–3. Quantum control of mechanical motion has been achieved by engineering the radiation–pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator4–7. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states8. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects9, 10, since their trapping potential is fully controllable. Here we optically levitate a femtogram (10−15 grams) dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its centre-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 0.43. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales11.