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arXiv:2408.14988 · Physical Review Research

Dichroic mirror pulses for optimized higher-order atomic Bragg diffraction

Dominik Pfeiffer, M. Dietrich, Patrik Schach, G. Birkl, Enno Giese

Published Feb 5, 2025• 4 citations
arXivHTMLPDF

Abstract

Increasing the sensitivity of light-pulse atom interferometers progressively relies on large-momentum transfer techniques. Precise control of such methods is imperative to exploit the full capabilities of these quantum sensors. One key element is the mitigation of deleterious effects such as parasitic paths deteriorating the interferometric signal. In this Letter, we present the experimental realization of dichroic mirror pulses for atom interferometry, its scalability to higher-order Bragg diffraction, and its robustness against initial momentum spread. Our approach selectively reflects resonant atom paths into the detected interferometer output, ensuring that these contribute to the signal with intent. Simultaneously, parasitic paths are efficiently transmitted by the mirror and not directed to the relevant interferometer outputs. This method effectively isolates the desired interferometric signal from noise induced by unwanted paths. It can be readily applied to existing setups capable of higher-order Bragg diffraction.

DOI
10.1103/physrevresearch.7.l012028

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Increasing the sensitivity of light-pulse atom interferometers progressively relies on large-momentum transfer techniques. Precise control of such methods is imperative to exploit the full capabilities of these quantum sensors. One key element is the mitigation of deleterious effects such as parasitic paths deteriorating the interferometric signal. In this Letter, we present the experimental realization of dichroic mirror pulses for atom interferometry, its scalability to higher-order Bragg diffraction, and its robustness against initial momentum spread. Our approach selectively reflects resonant atom paths into the detected interferometer output, ensuring that these contribute to the signal with intent. Simultaneously, parasitic paths are efficiently transmitted by the mirror and not directed to the relevant interferometer outputs. This method effectively isolates the desired interferometric signal from noise induced by unwanted paths. It can be readily applied to existing setups capable of higher-order Bragg diffraction.
Spin squeezing in atomic ensembles enables atom interferometry with sensitivities below the shot-noise limit, but the associated entanglement is highly susceptible to loss, making imperfections in atom optics a central limitation. Bragg diffraction is an established technique for driving transitions between atomic momentum states and enables large-momentum transfer through higher-order diffraction while preserving the internal state. However, it is intrinsically limited by two competing mechanisms: Short light pulses induce parasitic diffraction into off-resonant orders beyond an effective two-level description, while long pulses face velocity selectivity. We derive analytical expressions in a second-quantized framework for the atom optics and phase uncertainty of a Mach-Zehnder interferometer including these effects. We demonstrate that sub-shot-noise scaling is achieved only in a regime of intermediate pulse duration. Furthermore, we show that deleterious effects of higher-order diffraction are partially mitigated by optimizing the input quantum state.
Bragg diffraction of matter waves is an established technique used in the most accurate quantum sensors. It is also the method of choice to operate large-momentum-transfer, high-sensitivity atom interferometers. It suffers, however, from an intrinsic multi-path character. Optimal control theory (OCT) has recently led to an improved robustness of atom interferometers to a range of challenging environmental effects such as vibrations or platform accelerations. In this theoretical work, we apply OCT protocols to control the Bragg diffraction phase shifts, thereby enhancing the metrological accuracy of the interferometer. We show a minimization of the diffraction phase for realistic conditions of finite temperature of the incoming wavepacket in a multi-path, high-order Bragg interferometer in a Mach–Zehnder configuration. We study input states with different momentum widths and find that our approach mitigates diffraction phases below the microradian level in the case of 1% of the photon recoil, thereby eliminating one of the leading systematic effects in atom interferometry.
Bragg diffraction has been used in atom interferometers because it allows signal enhancement through multiphoton momentum transfer and suppression of systematics by not changing the internal state of atoms. Its multiport nature, however, can lead to parasitic interferometers, allows for intensity-dependent phase shifts in the primary interferometers, and distorts the ellipses used for phase extraction. We study and suppress these unwanted effects. Specifically, phase extraction by ellipse fitting and the resulting systematic phase shifts are calculated by Monte Carlo simulations. Phase shifts arising from the thermal motion of the atoms are controlled by spatial selection of atoms and an appropriate choice of Bragg intensity. In these simulations, we found that Gaussian Bragg pulse shapes yield the smallest systematic shifts. Parasitic interferometers are suppressed by a ``magic'' Bragg pulse duration. The sensitivity of the apparatus was improved by the addition of ac Stark shift compensation, which permits direct experimental study of sub-part-per-billion (ppb) systematics. This upgrade allows for a $310\ensuremath{\hbar}k$ momentum transfer, giving 6.6 Mrad measured in a Ramsey-Bord\'e interferometer.
We theoretically consider the effect of the atomic source's momentum width on the efficiency of Bragg mirrors and beamsplitters and, more generally, on the phase sensitivity of Bragg pulse atom interferometers. By numerical optimization, we show that an atomic cloud's momentum width places a fundamental upper bound on the maximum transfer efficiency of a Bragg mirror pulse, and furthermore limits the phase sensitivity of a Bragg pulse atom interferometer. We quantify these momentum width effects, and precisely compute how mirror efficiencies and interferometer phase sensitivities vary as functions of Bragg order and source type. Our results and methodology allow for an efficient optimization of Bragg pulses and the comparison of different atomic sources, and will help in the design of large momentum transfer Bragg mirrors and beamsplitters for use in atom-based inertial sensors.
Atom interferometers require both high efficiency and robust performance in their mirror pulses under experimental inhomogeneities. In this work, we demonstrated that quantum optimal control designed mirror pulse significantly enhance interferometer performance by using novel adaptive sliced structure. Using gradient ascent pulse engineering (GRAPE), optimized mirror pulse for a Mach-Zehnder light-pulse atom interferometer was designed by discretizing the control into non-uniform phase slices. This design broadened the tolerence to experimentally relevant variations in detuning [−Ω0,Ω0][-Ω_0,Ω_0][−Ω0​,Ω0​] and Rabi frequency [0.1×Ω0,1.9×Ω0][0.1\timesΩ_0,1.9\timesΩ_0][0.1×Ω0​,1.9×Ω0​] (Ω0=2π×25Ω_0=2π\times25Ω0​=2π×25 kHz), while maintaining high transfer efficiency even when the response-time delays up to 1.6 μs\rm{μs}μs. The optimized pulse was found to be robust to coupling inhomogeneity and velocity spread, offering a significant improvement in robustness over conventional pulse. The adaptive pulse slicing method provides a minimalist strategy that reduces experimental complexity while enhancing robustness and scalability, offering an innovative scheme for quantum optimal control in high precision atom interferometry.
Abstract Multi-photon Bragg diffraction is a powerful method for fast, coherent momentum transfer of atom waves. However, laser noise, Doppler detunings, and cloud expansion limit its efficiency in large momentum transfer (LMT) pulse sequences. We present simulation studies of robust Bragg pulses developed through numerical quantum optimal control. Optimized pulse performance under noise and cloud inhomogeneities is analyzed and compared to analogous Gaussian and adiabatic rapid passage pulses in simulated LMT Mach–Zehnder interferometry sequences. The optimized pulses maintain robust population transfer and phase response over a broader range of noise, resulting in superior contrast in LMT sequences with thermal atom clouds and intensity inhomogeneities. Large optimized LMT sequences use lower pulse area than Gaussian pulses, making them less susceptible to spontaneous emission loss. The optimized sequences maintain over five times better contrast with tens of ℏ k momentum separation and offer more improvement with greater LMT. Such pulses could allow operation of Bragg atom interferometers with unprecedented sensitivity, improved contrast, and hotter atom sources.