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arXiv:2408.12640

Time-resolved pairing gap spectroscopy in a quantum simulator of fermionic superfluidity inside an optical cavity

Dylan J. Young, Eric Yilun Song, Anjun Chu, Diego Barberena, Zhijing Niu, Vera M. Schäfer, Robert J. Lewis-Swan, Ana María Rey, James K. Thompson

Published Aug 22, 2024• 0 citations
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Abstract

We use an ensemble of laser-cooled strontium atoms in a high-finesse cavity to cleanly emulate the technique of rf spectroscopy employed in studies of BEC-BCS physics in fermionic superfluids of degenerate cold gases. Here, we leverage the multilevel internal structure of the atoms to study the physics of Cooper pair breaking in this system. In doing so, we observe and distinguish the properties of two distinct many-body gaps, the BCS pairing gap and the spectral gap, using nondestructive readout techniques. The latter is found to depend on the populations of the internal atomic states, reflecting the chemical potential dependence predicted in fermionic superfluids. This work opens the path for more fully exploiting the rich internal structure of atoms in cavity QED emulators to study both analogous systems and also more exotic states yet to be realized.

DOI
10.48550/arxiv.2408.12640

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We use an ensemble of laser-cooled strontium atoms in a high-finesse cavity to cleanly emulate the technique of rf spectroscopy employed in studies of BEC-BCS physics in fermionic superfluids of degenerate cold gases. Here, we leverage the multilevel internal structure of the atoms to study the physics of Cooper pair breaking in this system. In doing so, we observe and distinguish the properties of two distinct many-body gaps, the BCS pairing gap and the spectral gap, using nondestructive readout techniques. The latter is found to depend on the populations of the internal atomic states, reflecting the chemical potential dependence predicted in fermionic superfluids. This work opens the path for more fully exploiting the rich internal structure of atoms in cavity QED emulators to study both analogous systems and also more exotic states yet to be realized.
We use an ensemble of laser-cooled strontium atoms in a high-finesse cavity to cleanly emulate the technique of rf spectroscopy employed in studies of BEC-BCS physics in fermionic superfluids of degenerate cold gases. Here, we leverage the multilevel internal structure of the atoms to study the physics of Cooper pair breaking in this system. In doing so, we observe and distinguish the properties of two distinct many-body gaps, the BCS pairing gap and the spectral gap, using nondestructive readout techniques. The latter is found to depend on the populations of the internal atomic states, reflecting the chemical potential dependence predicted in fermionic superfluids. This work opens the path for more fully exploiting the rich internal structure of atoms in cavity QED emulators to study both analogous systems and also more exotic states yet to be realized.
Ultracold atomic gases are a powerful tool to experimentally study strongly correlated quantum many-body systems. In particular, ultracold Fermi gases with tunable interactions have allowed to realize the famous BEC-BCS crossover from a Bose-Einstein condensate (BEC) of molecules to a Bardeen-Cooper-Schrieffer (BCS) superfluid of weakly bound Cooper pairs. However, large parts of the excitation spectrum of fermionic superfluids in the BEC-BCS crossover are still unexplored. In this work, we use Bragg spectroscopy to measure the full momentum-resolved low-energy excitation spectrum of strongly interacting ultracold Fermi gases. This enables us to directly observe the smooth transformation from a bosonic to a fermionic superfluid that takes place in the BEC-BCS crossover. We also use our spectra to determine the evolution of the superfluid gap and find excellent agreement with previous experiments and self-consistent T-matrix calculations both in the BEC and crossover regime. However, toward the BCS regime a calculation that includes the effects of particle-hole correlations shows better agreement with our data.
We propose to simulate dynamical phases of a BCS superconductor using an ensemble of cold atoms trapped in an optical cavity. Effective Cooper pairs are encoded via the internal states of the atoms, and attractive interactions are realized via the exchange of virtual photons between atoms coupled to a common cavity mode. Control of the interaction strength combined with a tunable dispersion relation of the effective Cooper pairs allows exploration of the full dynamical phase diagram of the BCS model as a function of system parameters and the prepared initial state. Our proposal paves the way for the study of the nonequilibrium features of quantum magnetism and superconductivity by harnessing atom-light interactions in cold atomic gases.
Understanding how pairing correlations in superconductors evolve out of equilibrium is a central challenge in quantum many-body physics. In systems with sss-wave pairing, the character of Cooper pairing evolves continuously from a BCS regime of weakly bound, overlapping pairs to a BEC regime of tightly bound molecules, each with distinct excitation spectra. Here we realize and probe pairing dynamics across these regimes using cold, non-degenerate 87^{87}87Rb atoms coupled to an optical cavity with Floquet dressing. Our cavity-QED platform emulates fermionic superfluids through a mapping onto Anderson pseudospins, while optical and microwave control tunes the ratio of interactions to single-particle energies, providing a flexible approach complementary to ultracold Feshbach and ultrafast solid-state platforms. Following a quench, we observe persistent pairing and transient oscillations of the order parameter associated with a collective amplitude (Higgs) mode. We find that the decay of these oscillations sharply distinguishes weak- and strong-pairing regimes: in the weak-pairing regime, oscillations decay with a power-law exponent ∣α∣=0.65(8)|α|=0.65(8)∣α∣=0.65(8), whereas in the strong-pairing regime the decay is substantially faster, with ∣α∣>1|α|>1∣α∣>1. The oscillation frequency is set by the minimum quasiparticle excitation energy, directly linking nonequilibrium dynamics to the underlying excitation spectrum. Our results establish nonequilibrium dynamics as a direct probe of pairing character and collective excitations in interacting quantum systems.
This thesis studies radio-frequency spectroscopy of superfluid alkali Fermi gases. Radio-frequency and laser fields provide a coherent and well understood tool for manipulating atomic gases. However, new phenomena are expected and have already been seen experimentally when the alkali atoms become strongly interacting. Here we use a simple perturbative treatment of the atom-rf-field coupling for studying the spectroscopy of a strongly interacting gas. At ultracold temperatures fermionic atoms become paired in analogy to electrons in superconductors. The resulting binding energy, or the pairing gap, can be observed as a shift in the radio-frequency spectrum. With strong interactions, the fermions begin pairing already above the critical superfluid transition temperature. The radio-frequency spectroscopy grants a way to study these fluctuation effects quantitatively. The inhomogeneous trapping potential of the atom cloud also adds its own flavour, resulting in distinct mesoscopic effects in the radio-frequency spectra. Our theoretical models are in very good agreement with the experimental results. First order perturbation theory provides qualitatively correct lineshapes, and our generalised perturbative approach gives quantitatively correct magnitudes for the transfer rates. The inhomogeneity plays an important part also in more exotic systems in which the simple BCS-type pairing of atoms is prevented by polarising the gas. Superfluidity and phase separation in such spin-imbalanced gases has been experimentally observed. We have suggested the use of radio-frequency spectroscopy for observing exotic polarised superfluid states, present at the edges of the atom cloud.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.