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arXiv:2407.14018

Energy efficient coherent quantum control of nitrogen vacancy (NV) spin with nanoscale magnets

Md. Fahim F. Chowdhury, Adi Jung, Léa La Spina, Ausrine Bartasyte, Samuel H. Margueron, Jayasimha Atulasimha

Published Jul 19, 2024• 1 citation
arXivHTMLPDF

Abstract

We investigate coherent quantum control of a nitrogen vacancy (NV) center in diamond with microwave fields generated from a nanoscale magnet that is proximal to the NV center. Our results show remarkable coherent control with high contrast Rabi oscillations using nearfield microwaves from shape anisotropic nanomagnets of lateral dimensions down to 200 nm x 180 nm, driven remotely by surface acoustic wave (SAW) excitation that is at least 400 times and potentially 4 orders of magnitude more energy efficient than generating microwaves with an antenna. Furthermore, we show that varying the acoustic power driving such nanomagnets can achieve control over Rabi frequency. We also report spin-lattice relaxation time T1 is 103 +/-0.5 micro-seconds, the spin-spin relaxation time T2 is 1.23+/-0.29 micro-seconds, and the Ramsey coherence time T2* is 218+/-27 nanoseconds measured using microwave pulses generated by such nanomagnets. The use of the nanoscale magnets to implement highly localized and energy efficient coherent quantum control can replace thermally noisy microwave circuits and demonstrate a path to scalable quantum computing and sensing with NV-defects in diamond and other spin qubits.

DOI
10.48550/arxiv.2407.14018

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We investigate coherent quantum control of a nitrogen vacancy (NV) center in diamond with microwave fields generated from a nanoscale magnet that is proximal to the NV center. Our results show remarkable coherent control with high contrast Rabi oscillations using nearfield microwaves from shape anisotropic nanomagnets of lateral dimensions down to 200 nm x 180 nm, driven remotely by surface acoustic wave (SAW) excitation that is at least 400 times and potentially 4 orders of magnitude more energy efficient than generating microwaves with an antenna. Furthermore, we show that varying the acoustic power driving such nanomagnets can achieve control over Rabi frequency. We also report spin-lattice relaxation time T1 is 103 +/-0.5 micro-seconds, the spin-spin relaxation time T2 is 1.23+/-0.29 micro-seconds, and the Ramsey coherence time T2* is 218+/-27 nanoseconds measured using microwave pulses generated by such nanomagnets. The use of the nanoscale magnets to implement highly localized and energy efficient coherent quantum control can replace thermally noisy microwave circuits and demonstrate a path to scalable quantum computing and sensing with NV-defects in diamond and other spin qubits.
Abstract Nitrogen vacancy (NV) centers, optically active atomic defects in diamond, have attracted tremendous interest for quantum sensing, network, and computing applications due to their excellent quantum coherence and remarkable versatility in a real, ambient environment. One of the critical challenges to develop NV-based quantum operation platforms results from the difficulty in locally addressing the quantum spin states of individual NV spins in a scalable, energy-efficient manner. Here, we report electrical control of the coherent spin rotation rate of a single-spin qubit in NV-magnet based hybrid quantum systems. By utilizing electrically generated spin currents, we are able to achieve efficient tuning of magnetic damping and the amplitude of the dipole fields generated by a micrometer-sized resonant magnet, enabling electrical control of the Rabi oscillation frequency of NV spins. Our results highlight the potential of NV centers in designing functional hybrid solid-state systems for next-generation quantum-information technologies. The demonstrated coupling between the NV centers and the propagating spin waves harbored by a magnetic insulator further points to the possibility to establish macroscale entanglement between distant spin qubits.
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Nitrogen-vacancy (NV) centers in diamond have been used as platforms for quantum information, magnetometry and imaging of microwave (MW) fields. The spatial distribution of the MW fields used to drive the electron spin of NV centers plays a key role for these applications. Here, we report a system for the control and characterization of MW magnetic fields used for the NV spin manipulation. The control of the MW field in the vicinity of a diamond surface is mediated by an exchangeable lumped resonator, coupled inductively to a MW planar ring antenna. The characterization of the MW fields in the near-field is performed by an FFT imaging of Rabi oscillations, by using an ensemble of NV centers. We have found that the Rabi frequency over a lumped resonator is enhanced 22 times compared to the Rabi frequency without the presence of the lumped resonator. Our system may find applications in quantum information and magnetometry where a precise and controlled spin manipulation is required, showing NV centers as good candidates for imaging MW fields and characterization of MW devices.
High spatial resolution quantum sensing of near-surface nitrogen vacancy (NV) centers in diamond has enabled detection of magnetic, electrical, and thermal signals at the nanoscale. At depths of just a few nanometers, NV centers serve as localized quantum probes for external spins or low-dimensional materials, but their proximity to the surface also enhances decoherence caused by fluctuating nuclear spins. While advances in surface engineering have stabilized the charge state of NV centers at depths of tens of nanometers, achieving both ultra-shallow implantation (0.5-2 nm) and long-term spin coherence remains a central challenge. In this work, we show using first-principles modeling that, by exploiting the interaction of surface-induced strain and weak dc magnetic fields, the spin coherence times of 1-nm-deep NV centers can be greatly improved near the spin-phonon-confined regime at room temperature in 12C-rich diamonds. We also demonstrate that this protocol benefits ~ 10-nm-deep NV centers in natural diamond, enabling vector magnetometry at the nanoscale. Shallow NV centers in diamond are advantageous for quantum sensing but suffer from surface magnetic noise. Using first-principles simulations supported by experiments, the authors show that a combination of small magnetic fields and surface strain can significantly enhance spin coherence of 1 nm-deep NV centers.
Nitrogen-Vacancy (NV) centers in diamond are attractive tools for sensing and quantum information. Realization of this potential requires effective tools for controlling the spin degree of freedom by microwave (mw) magnetic fields. In this work, we present a planar microwave resonator optimized for microwave-optical double resonance experiments on single NV centers in diamond. It consists of a piece of wide microstrip line, which is symmetrically connected to two 50 Ω microstrip feed lines. In the center of the resonator, an Ω-shaped loop focuses the current and the mw magnetic field. It generates a relatively homogeneous magnetic field over a volume of 0.07 × 0.1 mm3. It can be operated at 2.9 GHz in both transmission and reflection modes with bandwidths of 1000 and 400 MHz, respectively. The high power-to-magnetic field conversion efficiency allows us to produce π-pulses with a duration of 50 ns with only about 200 and 50 mW microwave power in transmission and reflection, respectively. The transmission mode also offers capability for efficient radio frequency excitation. The resonance frequency can be tuned between 1.3 and 6 GHz by adjusting the length of the resonator. This will be useful for experiments on NV-centers at higher external magnetic fields and on different types of optically active spin centers.