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arXiv:2406.04114 · Physical review. B./Physical review. B

Harmonic generation with topological edge states and electron-electron interaction

Siamak Pooyan, D. Bauer

Published Jan 14, 2025• 2 citations
arXivHTMLPDF

Abstract

It has been found previously that the presence or absence of topological edge states in the Su-Schrieffer-Heeger (SSH) model has a huge impact on harmonic generation spectra. More specifically, the yield of harmonics for harmonic orders that correspond to photon energies below the band gap is many orders of magnitude different in the trivial and topological phases. It is shown in this work that this effect is still present if electron-electron interaction is taken into account, i.e., if a Hubbard term is added to the SSH Hamiltonian. To that end, finite SSH-Hubbard chains at half filling are considered that are short enough to be accessible to exact diagonalization but already show edge states in the topological phase. We show that the huge difference in the harmonic yield between the trivial and topological phases can be reproduced with few-level models employing only the many-body ground state and a few excited many-body states.

DOI
10.1103/physrevb.111.014308

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It has been found previously that the presence or absence of topological edge states in the Su-Schrieffer-Heeger (SSH) model has a huge impact on harmonic generation spectra. More specifically, the yield of harmonics for harmonic orders that correspond to photon energies below the band gap is many orders of magnitude different in the trivial and topological phases. It is shown in this work that this effect is still present if electron-electron interaction is taken into account, i.e., if a Hubbard term is added to the SSH Hamiltonian. To that end, finite SSH-Hubbard chains at half filling are considered that are short enough to be accessible to exact diagonalization but already show edge states in the topological phase. We show that the huge difference in the harmonic yield between the trivial and topological phases can be reproduced with few-level models employing only the many-body ground state and a few excited many-body states.
We study two-particle states in a Su-Schrieffer-Heeger (SSH) chain with periodic boundary conditions and nearest-neighbor (NN) interactions. The system is mapped into a problem of a single particle in a two-dimensional (2D) SSH lattice with potential walls along specific edges. The 2D SSH model has a trivial Chern number but a non-trivial Zak's phase, the one-dimensional (1D) topological invariant, along specific directions of the lattice, which allow for the presence of topological edge states. Using center-of-mass and relative coordinates, we calculate the energy spectrum of these two-body states for strong interactions and find that, aside from the expected appearance of doublon bands, two extra in-gap bands are present. These are identified as bands of topological states localized at the edges of the internal coordinate, the relative distance between the two particles. As such, the topological states reported here are intrinsically many-body in what concerns their real space manifestation, having no counterpart in single-particle states derived from effective models. Finally, we compare the effect of Hubbard interactions with that of NN interactions to show how the presence of the topological bound states is specific to the latter case.
The interplay and competition of topology and electron--electron interactions have fascinated researchers since the discovery of topological insulators. The Su--Schrieffer--Heeger--Hubbard (SSH-Hubbard) model is a prototypical model which includes both nontrivial topology and interactions. Due to its simplicity, there are several artificial quantum systems which can realize such a model to a good approximation. Here we focus on the quarter-filled case, where interactions and dimerization open a charge gap. In particular, we study the single-particle spectral function for the extended SSH-Hubbard model with magnetic field and explore several parameter limits where effective model descriptions arise. In the strongly dimerized limit, we show that the low-energy excitations of the spectral function resemble a half-filled Hubbard model with effective dimer sites and renormalized couplings. For strong magnetic field and interactions, we find physics akin to the spinless Su--Schrieffer--Heeger model at half filling, featuring a noninteracting topological phase transition. Moreover, in light of the recent realization of this model in quantum dot simulation, we provide evidence for the stability of the topological phase towards moderate nonlocal interactions in the experimentally expected parameter range.
The strong-field process of high-harmonic generation (HHG) has, in recent years, been treated from a quantum optical perspective in the emerging research area of strong-field quantum optics. These investigations show that HHG radiation is, in general, in a nonclassical state of light. However, the quantum optical treatment of HHG from topological nontrivial materials is missing. Here, we aim to address this gap in current knowledge and consider the quantum optical HHG response from the Su-Schrieffer-Heeger model, a finite chain of atoms with both a topologically trivial and nontrivial insulating phase, the latter supporting edge states. We find that HHG from both topological phases is squeezed at the band-gap frequency. Interestingly, while the harmonic spectrum discriminates the two topological phases of the system, the degree of squeezing only discriminates the phases for smaller chain lengths. We attribute this difference to a relative increase in overlap between bulk and edge states in the topological nontrivial phase for smaller systems. Our findings reveal how the strength of dipole couplings governs the nonclassical HHG response and define new research questions on topologically protected generation of quantum light in strong-field physics.
We address the effect of nearest-neighbor (NN) interactions on the topological properties of the Su-Schrieffer-Heeger (SSH) chain, with alternating hopping amplitudes t1{t}_{1}t1​ and t2{t}_{2}t2​. Both numerically and analytically, we show that the presence of interactions induces phase transitions between topologically different regimes. In the particular case of one-hole excitations in a half-filled SSH chain, the V/t2V/{t}_{2}V/t2​ versus t1/t2{t}_{1}/{t}_{2}t1​/t2​ phase diagram has topological phases at diagonal regions of the phase plane. The interaction acts in this case as a passivation potential. For general filling of the SSH chain, different eigensubspaces of the SSH Hamiltonian may be classified as topologically trivial and nontrivial. The two-hole case is studied in detail in the large interaction limit, and we show that a mapping can be constructed of the two-hole SSH eigensubspaces into one-particle states of a noninteracting one-dimensional (1D) tight-binding model, with interfaces between regions with different hopping constants and local potentials. The presence of edge states of topological origin in the equivalent chain can be readily identified, as well as their correspondence to the original two-hole states. Of these states only some, identified by us, are protected and, therefore, truly topological. Furthermore, we found that the presence of the NN interaction generates a state where two holes occupy two consecutive edge states. Such many-body states should also occur for arbitrary filling leading to the possibility of a macroscopic hole gathering at the surface (at consecutive edge states).
We study the interplay of spontaneous symmetry breaking and topological properties in interacting one-dimensional models. We solve these models using bozonization and identify topologically non-trivial phases by counting the additional degeneracy (affiliated with the edge modes) of a finite-size system relative to the infinite one. We find even if the mean-field solution is topological, this may not be true when it arises from spontaneous symmetry breaking, including in the Su-Schrieffer-Heeger (SSH) model. This implies that the original SSH model, as presented by Su, Schrieffer, and Heeger, is topologically trivial, as opposed to its mean-field version. A spinful version, on the other hand, does exhibit a topologically non-trivial phase. In that state, both mean-field solutions are topologically non-trivial and correspond to non-interacting SSH chains in the opposite phases with the winding number ν=1ν=1ν=1. We show that this phase is protected by a chiral symmetry, similar to the non-interacting phases.
We study the effects of electron-electron interactions on the charge excitation spectrum of the spinful Su-Schrieffer-Heeger (SSH) model, a prototype of a one-dimensional bulk obstructed topological insulator. In view of recent progress in the fabrication of dopant-based quantum simulators we focus on experimentally detectable signatures of interacting topology in finite lattices. To this end we use Lanczos-based exact diagonalization to calculate the single-particle spectral function in real space which generalizes the local density of states to interacting systems. Its spatial and spectral resolution allows for the direct investigation and identification of edge states. By studying the noninteracting limit, we demonstrate that the topological in-gap states on the boundary are robust against both finite-size effects as well as random bond and onsite disorder which suggests the feasibility of simulating the SSH model in engineered dopant arrays in silicon. While edge excitations become zero-energy spinlike for any finite interaction strength, our analysis of the spectral function shows that the single-particle charge excitations are gapped out on the boundary. Despite the loss of topological protection, we find that these edge excitations are quasiparticlelike as long as they remain within the bulk gap. Above a critical interaction strength of ${U}_{c}\ensuremath{\approx}5t$ these quasiparticles on the boundary lose their coherence which is explained by the merging of edge and bulk states. This is in contrast to the many-body edge excitations which survive the limit of strong coupling, as established in the literature. Our findings show that for moderate repulsive interactions the nontrivial phase of the interacting SSH model can be detected through remnant signatures of topological single-particle states using single-particle local measurement techniques such as scanning tunneling spectroscopy.