The simulation of high-temperature superconducting materials by implementing strongly correlated fermionic models in optical lattices is one of the major objectives in the field of analog quantum simulation. Here we show that local control and optical bilayer capabilities combined with spatially resolved measurements create a versatile toolbox to study fundamental properties of both nickelate and cuprate high-temperature superconductors. On the one hand, we present a scheme to implement a mixed-dimensional (mixD) bilayer model that has been proposed to capture the essential pairing physics of pressurized bilayer nickelates. This allows for the long-sought realization of a state with long-range superconducting order in current lattice quantum simulation machines. In particular, we show how coherent pairing correlations can be accessed in a partially particle-hole transformed and rotated basis. On the other hand, we demonstrate that control of local gates enables the observation of d -wave pairing order in the two-dimensional (single-layer) repulsive Fermi-Hubbard model through the simulation of a system with attractive interactions. Lastly, we introduce a scheme to measure momentum-resolved dopant densities, providing access to observables complementary to solid-state experiments—which is of particular interest for future studies of the enigmatic pseudogap phase appearing in cuprates. Published by the American Physical Society 2024
The simulation of high-temperature superconducting materials by implementing strongly correlated fermionic models in optical lattices is one of the major objectives in the field of analog quantum simulation. Here we show that local control and optical bilayer capabilities combined with spatially resolved measurements create a versatile toolbox to study fundamental properties of both nickelate and cuprate high-temperature superconductors. On the one hand, we present a scheme to implement a mixed-dimensional (mixD) bilayer model that has been proposed to capture the essential pairing physics of pressurized bilayer nickelates. This allows for the long-sought realization of a state with long-range superconducting order in current lattice quantum simulation machines. In particular, we show how coherent pairing correlations can be accessed in a partially particle-hole transformed and rotated basis. On the other hand, we demonstrate that control of local gates enables the observation of d -wave pairing order in the two-dimensional (single-layer) repulsive Fermi-Hubbard model through the simulation of a system with attractive interactions. Lastly, we introduce a scheme to measure momentum-resolved dopant densities, providing access to observables complementary to solid-state experiments—which is of particular interest for future studies of the enigmatic pseudogap phase appearing in cuprates. Published by the American Physical Society 2024
Studying the low-temperature phases of doped Hubbard models, including the emergence of collective order and exotic normal phases, is at the heart of strongly correlated physics. This thesis offers new theoretical insights into the low-energy physics of doped Hubbard models, with a particular emphasis on leveraging quantum simulation as a powerful investigative tool. We explore the emergence of collective order driven by many-body interactions, by predicting and observing stripe-like structures in quantum gas microscopes of engineered Hamiltonians. These fluctuating stripe patterns are developed into a theoretical framework for the pseudogap— a highly enigmatic phase in hole-doped cuprates—where we show how fluctuating domain walls yield effective toric code descriptions. Ultracold atoms in optical lattices provide a unique platform for directly probing and testing this theory. We further investigate unconventional bilayer nickelate superconductors, predicting an exceptionally stable superfluid state in a single-band Hubbard model at experimentally accessible temperatures. By proposing schemes to observe coherent pair-pair correlations, this advances the long-standing goal of realizing and observing long-range superconducting order in ultracold atomic systems in optical lattices. On non-bipartite lattices, we examine kinetic magnetism in Hubbard models and moiré heterostructures. Additionally, the low-temperature regime of doped Hubbard models with enhanced symmetries is analyzed, revealing exotic phenomena such as sub-dimensional polaronic particles. We develop machine learning techniques to extract key physical insights from many-body snapshots, offering a new avenue for understanding intricate quantum phases. Finally, we go beyond the Fermi-Hubbard paradigm and show how non-local strongly correlated models can be leveraged to address classical optimization problems through quantum annealing.
The microscopic origin of high-temperature superconductivity in cuprates remains one of the central open questions in condensed matter physics. Growing experimental and theoretical evidence suggests that the bare single-band Fermi-Hubbard model may not fully capture properties of cuprates such as superconductivity, motivating us to revisit the canonical three-band model of the copper-oxide planes - the Emery model - from which the single-band counterpart was originally derived. Here, we propose and analyze a quantum simulation scheme for realizing the Emery model in regimes relevant to cuprates and infinite-layer nickelates with today's ultracold atom quantum simulation platforms, enabling the exploration of the three-band physics on system sizes that are challenging for current numerical methods. Specifically, we show that a two-dimensional optical lattice with a superimposed pattern of repulsive potentials can be designed to study low-temperature properties for variable parameter regimes of the Emery model relevant to cuprates as well as infinite-layer nickelates. Our results pave the way for real material simulations with ultracold atom quantum simulators and a better understanding of the physics of unconventional superconductors.
Connecting single-layer t-J to Kondo lattice models: Exploration with cold atoms
The Kondo effect, a hallmark of many-body physics, emerges from the antiferromagnetic coupling between localized spins and conduction fermions, leading to a correlated many-body singlet state. Here we propose to use the mixed-dimensional (mixD) bilayer Hubbard geometry as a platform to study Kondo lattice physics with current ultracold atom experiments. At experimentally feasible temperatures, we predict that key features of the Kondo effect can be observed, including formation of the Kondo cloud around a single impurity and the competition of singlet formation with Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions for multiple impurities, summarized in the Doniach phase diagram. Moreover, we show that the mixD platform provides a natural bridge between the Doniach phase diagram of the Kondo lattice model, relevant to heavy-fermion materials, and the phase diagram of cuprate superconductors as described by a single-layer Zhang-Rice type t-J model: It is possible to continuously tune between the two regimes by changing the interlayer Kondo coupling. Our findings demonstrate that the direct connection between high-temperature superconductivity and heavy-fermion physics can be experimentally studied using currently available quantum simulation platforms.
Among the most compelling targets for quantum simulation are strongly correlated phases and electronic-structure problems, where interactions organize electrons into collective states and produce intricate low-temperature phase diagrams. Cuprate superconductors are a canonical example: at low doping, superconductivity emerges from a metallic regime that exhibits a pseudogap above the critical temperature. Ultracold atoms in optical lattices provide a well-controlled, tunable setting to probe the microscopic mechanisms behind this behavior and, in fermion-native architectures, to implement electronic structure dynamics directly. This thesis demonstrates both large scale systematic analog quantum simulations in the most interesting regime of doped antiferromagnets and elementary high-fidelity gates as the basis for a digital or hybrid fermionic quantum processors in an optical lattice. Working with ultracold Lithium-6 in a two–dimensional optical superlattice, we first map the parameter space of the Fermi–Hubbard model over a wide range of temperatures and dopings. More than 40000 single-site spin- and density-resolved snapshots, spanning over a dense grid of doping levels and temperatures in a numerically challenging parameter space, reveal antiferromagnetic correlations extending across the system size and into the pseudogap regime. Temperatures down to T/t=0.2 are realized, determined by benchmarking the data to state-of-the-art numerical methods. By evaluating spin–charge correlators up to fifth order, we experimentally uncover a universal scaling behavior across the pseudogap crossover, governed by a single, doping-dependent temperature scale. These findings provide the first microscopic evidence of universal scaling in multi-point correlators and establish stringent benchmarks for future theoretical developments. On the same apparatus, we demonstrate that the controlled motion of fermions in double wells enables high-fidelity entanglement. Double-well potentials are used to engineer coherent pair-tunnelling and spin-exchange interactions that act as native SWAP^α operations. We demonstrate the collisional gate fidelities up to 99.8% and Bell-state lifetimes exceeding ten seconds, limited mainly by residual inhomogeneities in the optical potential. A composite pulse sequence isolates the pair-exchange channel, realizing the elementary building block required for fermionic quantum-chemistry algorithms. With the addition of site-selective addressing, our results mark a key step towards a fully digital, scalable fermionic quantum computer based on the controlled motion and entanglement of fermionic neutral atoms. The work establishes a hybrid analog-digital architecture: analog evolution under the Hubbard Hamiltonian yields thermodynamic states whose magnetic properties match and extend theoretical benchmarks, while digital collisional gates provide building blocks for error-corrected quantum computation and complex state preparation.
The Fermi-Hubbard model is the starting point for the simulation of many strongly correlated materials, including high-temperature superconductors, whose modelling is a key motivation for the construction of quantum simulation and computing devices. However, the detection of superconducting pairing correlations has so far remained out of reach, both because of their off-diagonal character - which makes them inaccessible to local density measurements - and because of the difficulty of preparing superconducting states. Here, we report measurement of significant pairing correlations in three different regimes of Fermi-Hubbard models simulated on Quantinuum's Helios trapped-ion quantum computer. Specifically, we measure non-equilibrium pairing induced by an electromagnetic field in the half-filled square lattice model, d-wave pairing in an approximate ground state of the checkerboard Hubbard model at 1/6-doping, and s-wave pairing in a bilayer model relevant to nickelate superconductors. These results show that a quantum computer can reliably create and probe physically relevant states with superconducting pairing correlations, opening a path to the exploration of superconductivity with quantum computers.
In this thesis, I present the experimental realisation of the two-dimensional Hubbard model with ultracold fermionic Potassium-40 atoms in optical lattices. By tuning the dimensionality, kinetic and interaction in the optical lattices, we perform an analogue quantum simulation to explore the phase diagram of the Hubbard model. \n \nThe first key result is the experimental observation of particle-hole symmetry, namely a phase mapping between repulsive and attractive interactions. We compare a density-ordered, Mott-insulating phase with repulsive interaction to a spin-ordered, preformed pair phase and found excellent agreement with the theoretical prediction. The precise control and excellent detection capability of our quantum gas apparatus allow us to validate the particle-hole symmetry, and utilise it to explore quantum phases with a novel approach. \n \nNext, we investigate the spin-ordering on the repulsive side. By implementing a novel scheme based on coherent manipulation of spin correlations, we probe the anti-ferromagnetic ordering in the low-temperature phase diagram. The momentum-resolved spin correlations permit the reconstruction of spatial correlators without site-resolved imaging fidelity. \n \nFinally, we probe the attractive side of the phase diagram with a focus in pairing phenomenon, in which we draw a close analogy with BCS-BEC crossovers present in high-temperature superconducting cuprates and trapped ultracold Fermi gases. From the pair correlation function derived from thermodynamics observables, we observe the competition between the effective Pauli repulsion in fermionic systems and the on-site attraction we implemented.