Programmable optical tweezer arrays of molecules are an emerging platform for quantum simulation and quantum information science. For these applications, the reduction and mitigation of errors remain major challenges. In this work, we leverage the rich internal structure of molecules to mitigate two types of errors—internal state preparation and qubit leakage errors. First, we demonstrate robust measurement-enhanced tweezer preparation at a record fidelity using site-resolved error detection followed by tweezer movement. Second, using a new hyperfine qubit encoding well suited for use as a quantum memory, we demonstrate site-resolved detection of qubit leakage errors (erasures) induced by blackbody radiation. This approach constitutes the first demonstration of erasure conversion in molecules, a capability that has found recent interest in quantum error correction. Our work opens the door to new possibilities with molecular tweezer arrays: Measurement-enhanced preparation opens access to mesoscopic defect-free molecular arrays that are important for quantum simulation of interacting many-body systems; erasure conversion in molecular arrays lays the technical groundwork for midcircuit detection, an important capability for explorations in quantum information processing.
Programmable optical tweezer arrays of molecules are an emerging platform for quantum simulation and quantum information science. For these applications, the reduction and mitigation of errors remain major challenges. In this work, we leverage the rich internal structure of molecules to mitigate two types of errors—internal state preparation and qubit leakage errors. First, we demonstrate robust measurement-enhanced tweezer preparation at a record fidelity using site-resolved error detection followed by tweezer movement. Second, using a new hyperfine qubit encoding well suited for use as a quantum memory, we demonstrate site-resolved detection of qubit leakage errors (erasures) induced by blackbody radiation. This approach constitutes the first demonstration of erasure conversion in molecules, a capability that has found recent interest in quantum error correction. Our work opens the door to new possibilities with molecular tweezer arrays: Measurement-enhanced preparation opens access to mesoscopic defect-free molecular arrays that are important for quantum simulation of interacting many-body systems; erasure conversion in molecular arrays lays the technical groundwork for midcircuit detection, an important capability for explorations in quantum information processing.
Polar molecules are a quantum resource with rich internal structure that can be coherently controlled. The structure, however, also makes the state preparation and measurement (SPAM) of molecules challenging. We advance the SPAM of individual molecules assembled from constituent atoms trapped in optical-tweezer arrays. Sites without Na Cs molecules are eliminated using high-fidelity Cs atom detection, increasing the peak molecule filling fraction of the array threefold. We site-selectively initialize the array in a rotational qubit subspace that is insensitive to differential ac Stark shifts from the optical tweezer. Lastly, we detect multiple rotational states per experimental cycle by imaging atoms after sequential state-selective dissociations. These demonstrations extend the SPAM capabilities of molecules for quantum information, simulation, and metrology. Published by the American Physical Society 2024
Polar molecules trapped in optical tweezer arrays offer a promising platform for quantum information processing, providing precise control and long-range interactions that enable high-fidelity gate operations. We investigate quantum error correction in this system and show the influence of underlying physical noise. A mapping is constructed from a molecular tweezer array onto a rotated surface code in which a single specification of the array, namely, which code qubits share a molecule and where those molecules are located, determines both the correlated erasure structure and the dipolar exchange graph. We compare molecular encodings with rotational qudit dimensions (D), two and four under heralded molecular loss, coherent dipolar exchange, and imperfect heralding. It is found that a D= 4 encoding with spatially dispersed pairing exhibits a finite distance crossing at approximately the same per molecule loss rate as D= 2, while using 48-49 % fewer molecules, at the cost of a 6-10 % increase in sub-threshold logical error. Fixing the encoding and varying only the spatial embedding produces substantially larger effects: pairing the two co-located qubits along a lattice direction yields a logical-sector asymmetry of approximately fifty times. Over the simulated distances (d = 5, 7, 9), the disfavoured sector shows little or no suppression of logical error with increasing code distance, whereas the favoured sector improves by a factor of 1.5-2.3. We also find that Pauli twirl of the exchange interaction overestimates the logical error rate, which we attribute to the excitation-conserving structure of the interaction. These results reveal that the spatial embedding of correlated loss units is an important design parameter for molecular architectures and that single-sector benchmarks may be insufficient when correlated loss has directional structure.
Control over the quantum states of individual molecules is crucial in the quest to harness their rich internal structure and dipolar interactions for applications in quantum science. In this paper, we develop a toolbox of techniques for the control and readout of individually trapped polar molecules in an array of optical tweezers. Starting with arrays of up to eight Rb and eight Cs atoms, we assemble arrays of RbCs molecules in their rovibrational and hyperfine ground state with an overall efficiency of 48(2)%. We demonstrate global microwave control of multiple rotational states of the molecules and use an auxiliary tweezer array to implement site-resolved addressing and state control. We show how the rotational state of the molecule can be mapped onto the position of Rb atoms and use this capability to readout multiple rotational states in a single experimental run. Further, using a scheme for the midsequence detection of molecule formation errors, we perform rearrangement of assembled molecules to prepare small defect-free arrays. Finally, we discuss a feasible route to scaling to larger arrays of molecules. Published by the American Physical Society 2024
Abstract Minimizing and understanding errors is critical for quantum science, both in noisy intermediate scale quantum (NISQ) devices 1 and for the quest towards fault-tolerant quantum computation 2,3 . Rydberg arrays have emerged as a prominent platform in this context 4 with impressive system sizes 5,6 and proposals suggesting how error-correction thresholds could be significantly improved by detecting leakage errors with single-atom resolution 7,8 , a form of erasure error conversion 9–12 . However, two-qubit entanglement fidelities in Rydberg atom arrays 13,14 have lagged behind competitors 15,16 and this type of erasure conversion is yet to be realized for matter-based qubits in general. Here we demonstrate both erasure conversion and high-fidelity Bell state generation using a Rydberg quantum simulator 5,6,17,18 . When excising data with erasure errors observed via fast imaging of alkaline-earth atoms 19–22 , we achieve a Bell state fidelity of ≥0.9971−13+10 ≥ 0.997 1 − 13 + 10 , which improves to ≥0.9985−12+7 ≥ 0.998 5 − 12 + 7 when correcting for remaining state-preparation errors. We further apply erasure conversion in a quantum simulation experiment for quasi-adiabatic preparation of long-range order across a quantum phase transition, and reveal the otherwise hidden impact of these errors on the simulation outcome. Our work demonstrates the capability for Rydberg-based entanglement to reach fidelities in the 0.999 regime, with higher fidelities a question of technical improvements, and shows how erasure conversion can be utilized in NISQ devices. These techniques could be translated directly to quantum-error-correction codes with the addition of long-lived qubits 7,22–24 .
Optical tweezer arrays 1,2 have transformed atomic and molecular physics, now forming the backbone for a range of leading experiments in quantum computing 3–8 , simulation 1,9–12 , and metrology 13–15 . Typical experiments trap tens to hundreds of atomic qubits, and recently systems with around one thousand atoms were realized without defining qubits or demonstrating coherent control 16–18 . However, scaling to thousands of atomic qubits with long coherence times, low-loss, and high-fidelity imaging is an outstanding challenge and critical for progress in quantum science, particularly towards quantum error correction 19,20 . Here, we experimentally realize an array of optical tweezers trapping over 6,100 neutral atoms in around 12,000 sites, simultaneously surpassing state-of-the-art performance for several metrics that underpin the success of the platform. Specifically, while scaling to such a large number of atoms, we demonstrate a coherence time of 12.6(1) seconds, a record for hyperfine qubits in an optical tweezer array. We show room-temperature trapping lifetimes of ~ 23 minutes, enabling record-high imaging survival of 99.98952(1)% with an imaging fidelity of over 99.99%. We present a plan for zone-based quantum computing 5,21 and demonstrate necessary coherence-preserving qubit transport and pick-up/drop-off operations on large spatial scales, characterized through interleaved randomized benchmarking. Our results, along with recent developments 8,22–24 , indicate that universal quantum computing and quantum error correction with thousands to tens of thousands of physical qubits could be a near-term prospect.
Over the past decade, quantum information science has progressed from few-qubit demonstrations to experiments with hundreds of qubits. Neutral atom processors based on individual atoms trapped in arrays of optical tweezers have emerged as a leading candidate due to their inherent scalability and flexible connectivity. Advanced protocols like measurement-based state preparation and quantum error correction, however, require efficient crosstalk-free mid-circuit operations for the readout, reset, and replenishment of a subset of qubits. In typical single-species atom arrays, where all atoms are identical and on-resonance, such operations necessitate complex overheads from single-site addressing, coherent transport, or shielding techniques, to mitigate the qubit decoherence induced from photons scattered by neighboring atoms. To address this challenge of engineering scalable quantum architectures compatible with efficient control techniques, we introduce and implement the first dual-species atom array platform, and explore new dynamics inaccessible in single-species arrays. In this approach, two atomic species are addressed independently due to the spectral separation between their control wavelengths. We engineer two-dimensional arrays from individual rubidium (Rb) and cesium (Cs) atoms in up to 512 optical tweezers, and show that the two species can be independently trapped, cooled, and imaged with state-of-the-art performance metrics. Harnessing this intrinsic crosstalk-free control, we establish the key primitives of mid-circuit readout, real-time processing and feed-forward, and coherent mid-circuit reloading. By integrating these capabilities, we realize in-sequence, real-time correction of correlated phase errors via a spectator qubit protocol. Next, we excite atoms to Rydberg states in the Förster regime, accessing hitherto unobserved enhanced interspecies Rydberg interactions, and program them to implement the first interspecies CNOT gate. We combine this multispecies entanglement with mid-circuit readout to achieve quantum non-demolition measurement of a Rb-qubit using an auxiliary Cs-qubit, circumventing physical qubit transport. Finally, leveraging the two qubit modalities, we present the first experimental demonstration of quantum cellular automata in atom arrays using only global addressing, and prepare a 17-qubit Cs cluster state with Rb-mediated interactions. The dual-species platform and techniques established in this thesis pave the way toward measurement-based algorithms and real-time feedback control in large-scale quantum systems.