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arXiv:2405.18109

Differential polarizability at 1064 nm of the strontium intercombination transition

Romaric Journet, F. Faisant, Sanghyeop Lee, Marc Cheneau

Published May 28, 2024• 0 citations
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Abstract

We measure the scalar, vector and tensor components of the differential dynamic polarizability of the strontium intercombination transition at 1064 nm. We compare the experimental values with the theoretical prediction based on the most recently published spectroscopic data, and find a very good agreement. We also identify a close-to-circular `magic' polarization where the differential polarizability strictly vanishes, and precisely determine its ellipticity. Our work opens new perspectives for laser cooling optically trapped strontium atoms, and provides a new benchmark for atomic models in the near infrared spectral range.

DOI
10.48550/arxiv.2405.18109

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We measure the scalar, vector and tensor components of the differential dynamic polarizability of the strontium intercombination transition at 1064 nm. We compare the experimental values with the theoretical prediction based on the most recently published spectroscopic data, and find a very good agreement. We also identify a close-to-circular `magic' polarization where the differential polarizability strictly vanishes, and precisely determine its ellipticity. Our work opens new perspectives for laser cooling optically trapped strontium atoms, and provides a new benchmark for atomic models in the near infrared spectral range.
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We characterize the anisotropic differential ac-Stark shift for the Dy 626nm626\phantom{\rule{3.33333pt}{0ex}}\mathrm{nm}626nm intercombination transition, induced in a far-detuned 1070nm1070\phantom{\rule{3.33333pt}{0ex}}\mathrm{nm}1070nm optical dipole trap, and observe the existence of a ``magic polarization'' for which the polarizabilities of the ground and excited states are equal. From our measurements we extract both the scalar and tensorial components of the dynamic dipole polarizability for the excited state, ${\ensuremath{\alpha}}_{E}^{\text{s}}=188(12){\ensuremath{\alpha}}_{\text{0}}$ and ${\ensuremath{\alpha}}_{E}^{\text{t}}=34(12){\ensuremath{\alpha}}_{\text{0}}$, respectively, where ${\ensuremath{\alpha}}_{\text{0}}$ is the atomic unit for the electric polarizability. We also provide a theoretical model allowing us to predict the excited state polarizability and find qualitative agreement with our observations. Furthermore, we utilize our findings to optimize the efficiency of Doppler cooling of a trapped gas, by controlling the sign and magnitude of the inhomogeneous broadening of the optical transition. The resulting initial gain of the collisional rate allows us, after forced evaporation cooling, to produce a quasipure Bose-Einstein condensate of 162Dy^{162}\mathrm{Dy}162Dy with $3\ifmmode\times\else\texttimes\fi{}{10}^{4}$ atoms.
We report experimental measurements of the dynamical polarizability of dysprosium, at a wavelength of 532 nm. We measure all three components (scalar, vector, and tensor) of the anisotropic polarizability for the ground and the excited manifolds of the intercombination transition of Dy at 626 nm. The apparatus on which the measurements are performed is presented. We obtain with this setup imaging of single Dy atoms with fidelity above 99% and losses below 2.5% induced by imaging. We then describe the methods used to extract the polarizability. In particular, we combine a measurement of trap frequency and trap depth on single atoms in optical tweezers, allowing us to obtain a measurement of the ground-state polarizability free of errors in trap waist calibration. The obtained values give a magic condition between two Zeeman states in the ground and excited manifolds, which is used to image single atoms in optical tweezer arrays. The scalar polarizability of the ground state is in disagreement with theoretical expectations, calling for future investigations to resolve the discrepancy.
Open-shell lanthanide atoms, and dysprosium in particular, combine a large ground-state angular momentum with dense electronic spectra, making their dynamical polarizability strongly dependent on wavelength and internal state, and therefore challenging to calculate and characterize experimentally. This issue has become especially relevant with the recent development of single-atom trapping of dysprosium in optical-tweezer arrays, where precise knowledge of the polarizability is needed to design optimized trapping architectures. Here, we exploit the strong spin-dependent light shift near the J′=J−1J'=J-1J′=J−1 intercombination line at 530.306 nm to determine the background scalar and vector polarizabilities of 162^{162}162Dy in its ground state near this wavelength. Our measurements quantitatively agree with atomic-structure calculations and provide new insight into the contributions of nearby transitions in a spectral region relevant to emerging dysprosium tweezer platforms.
We calculate and measure the magic wavelengths for the $6{s}^{2}^{1}S_{0}\ensuremath{-}6s6p\phantom{\rule{0.16em}{0ex}}^{3}P_{1}$ intercombination transition of the neutral ytterbium atom. The calculation is performed with the ab initio configuration interaction +++ all-order method. The measurement is done with laser spectroscopy on cold atoms in an optical dipole trap. The magic wavelengths are determined to be 1035.68(4) nm for the $\ensuremath{\pi}$ transition $(\mathrm{\ensuremath{\Delta}}m=0)$ and 1036.12(3) nm for the $\ensuremath{\sigma}$ transitions $(|\mathrm{\ensuremath{\Delta}}m|=1)$ in agreement with the calculated values. Laser cooling on the narrow intercombination transition could achieve better results for atoms in an optical dipole trap when the trap wavelength is tuned to near the magic wavelength.