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arXiv:2405.14218 · Physical review. B./Physical review. B

Collective modes in Fulde-Ferrell-Larkin-Ovchinnikov superconductors: Role of long-range Coulomb interaction and signatures in density response

Ryoga Miwa, Ryoi Ohashi, Satoshi Fujimoto, Takeshi Mizushima

Published Feb 18, 2025• 2 citations
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Abstract

We theoretically investigate collective excitations in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) states of Pauli-limited superconducting films. When the long-range Coulomb interaction is absent, excitation spectra consist of two gapless and three gapped modes. The gapless modes are the Nambu-Goldstone modes associated with the spontaneous breaking of the $\mathrm{U}(1)$ symmetry and the translational symmetry. The gapped modes include the Higgs mode and the twofold degenerate modes that cause the oscillation of the domain width and grayness of FFLO nodal planes. We find that the long-range Coulomb interaction only gaps out the gapless phase mode through the Anderson-Higgs mechanism, while the other modes remain unaffected. Furthermore, the field evolution of the dispersion of the gapless elastic mode, the Nambu-Goldstone mode associated with the translational symmetry breaking, is associated with that of the bandwidth of the mid-gap Andreev bound states. We demonstrate that the signature of the elastic mode can be detected by measuring the density-density response function.

DOI
10.1103/physrevb.111.054516

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We theoretically investigate collective excitations in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) states of Pauli-limited superconducting films. When the long-range Coulomb interaction is absent, excitation spectra consist of two gapless and three gapped modes. The gapless modes are the Nambu-Goldstone modes associated with the spontaneous breaking of the U(1)\mathrm{U}(1)U(1) symmetry and the translational symmetry. The gapped modes include the Higgs mode and the twofold degenerate modes that cause the oscillation of the domain width and grayness of FFLO nodal planes. We find that the long-range Coulomb interaction only gaps out the gapless phase mode through the Anderson-Higgs mechanism, while the other modes remain unaffected. Furthermore, the field evolution of the dispersion of the gapless elastic mode, the Nambu-Goldstone mode associated with the translational symmetry breaking, is associated with that of the bandwidth of the mid-gap Andreev bound states. We demonstrate that the signature of the elastic mode can be detected by measuring the density-density response function.
In nonuniform Larkin-Ovchinnikov-Fulde-Ferrell (LOFF) superconductors, both the gauge symmetry and the continuous translational symmetry of the normal state are spontaneously broken. This leads to additional bosonic excitations, or Goldstone modes, corresponding to the deformations of the order parameter amplitude modulation in real space. We derive general expressions for the energy of the phase and elastic Goldstone modes. As an example, the superfluid density and the elastic modulus of a one-dimensional LOFF superconductor are calculated at low temperatures.
The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase is an unconventional superconducting state found under the influence of a strong Zeeman field. This phase is identified by finite center-of-mass momenta in the Cooper pairs, causing the pairing amplitude to oscillate in real space. Repulsive correlations, on the other hand, smear out spatial inhomogeneities in ddd-wave superconductors. We investigate the FFLO state in a strongly correlated ddd-wave superconductor within a consolidated framework of Hartree-Fock-Bogoliubov theory and the Gutzwiller approximation. We find that the crucial effects of strong correlations lie in shifting the BCS-FFLO phase boundary towards a lower Zeeman field and thereby enlarging the window of the FFLO phase. In the FFLO state, our calculation features a sharp midgap peak in the density of states, indicating the formation of strongly localized Andreev bound states. We also find that the signatures of the FFLO phase survive even in the presence of an additional translational-symmetry-breaking competing order in the ground state. This is demonstrated by considering a broken-symmetry ground state with a simultaneous presence of the ddd-wave superconducting order and a spin-density wave order, often found in unconventional superconductors.
We characterize the collective modes of a soliton train in a quasi-one-dimensional Fermi superfluid, using a mean-field formalism. In addition to the expected Goldstone and Higgs modes, we find novel long-lived gapped modes associated with oscillations of the soliton cores. The soliton train has an instability that depends strongly on the interaction strength and the spacing of solitons. It can be stabilized by filling each soliton with an unpaired fermion, thus forming a commensurate Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. We find that such a state is always dynamically stable, which paves the way for realizing long-lived FFLO states in experiments via phase imprinting.
Fulde-Ferrell-Larkin-Ovchinnikov Superfluids with PPP-wave Symmetry in Spinless Fermionic Optical Lattices
The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state, whose Cooper pairing hosts a non-zero center-of-mass momentum, is predicted and well studied in spin-singlet superfluids in past decades. Different from previous works that engineer FFLO superfluids in spinful cold atoms, we show that the FFLO superfluids, with ppp-wave symmetry, can emerge in a spinless environment associated with nearest-neighbor-site interactions. The novel mechanism of the FFLO superfluids lies on the split Fermi surfaces at low filling factor, which naturally gives rise to Cooper pairings with finite momentum. The phase transition is accompanied by changed Chern numbers, in which, different from the conventional picture, the band gap does not close. The exotic topological transition can be explained by the spontaneously-broken translational invariance of order parameters. Finally, we investigate the Berezinskii-Kosterlitz-Thouless (BKT) transition temperature of the FFLO state, and show its possibility to be observed at finite temperature.
We show that the gauge-invariant kinetic equation of superconductivity provides an efficient approach to study the electromagnetic response of the gapless Nambu-Goldstone and gapful Higgs modes on an equal footing. We prove that the Fock energy in the kinetic equation is equivalent to the generalized Ward's identity. Hence, the gauge invariance directly leads to the charge conservation. Both linear and second-order optical responses are analytically investigated. The linear response of the Higgs mode vanishes in the long-wave limit, whereas the linear response of the Nambu-Goldstone mode interacts with the long-range Coulomb interaction, causing the original gapless energy spectrum effectively lifted up to the plasma frequency as a result of the Anderson-Higgs mechanism, consistent with previous work. The second-order response exhibits interesting physics. On the one hand, a finite second-order optical response of the Higgs mode is obtained in the long-wave limit. We reveal that this response, which has been experimentally observed, is attributed solely to the drive effect rather than the widely considered Anderson-pump effect. On the other hand, the second-order optical response of the Nambu-Goldstone mode, free from the influence of the long-range Coulomb interaction and hence the Anderson-Higgs mechanism, is predicted. We find that both Anderson-pump and drive effects play important role in this response. A tentative scheme to detect this second-order response is proposed.