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arXiv:2405.03149 · Few-Body Systems

Observing S-Matrix Pole Flow in Resonance Interplay

Matthew Chilcott, Samyajit Gayen, James F. E. Croft, Ryan Thomas, Niels Kjærgaard

Published May 25, 2024• 2 citations
arXivHTMLPDF

Abstract

Abstract We provide an overview of experiments exploring resonances in the collision of ultracold clouds of atoms. Using a laser-based accelerator that capitalises on the energy resolution provided by the ultracold atomic setting, we unveil resonance phenomena such as Feshbach and shape resonances in their quintessential form by literally photographing the halo of outgoing scattered atoms. We exploit the tunability of magnetic Feshbach resonances to instigate an interplay between scattering resonances. By experimentally recording the scattering in a parameter space spanned by collision energy and magnetic field, we capture the imprint of the S -matrix pole flow in the complex energy plane. After revisiting experiments that place a Feshbach resonance in the proximity of a shape resonance and an anti-bound state, respectively, we discuss the possibility of using S -matrix pole interplay between two Feshbach resonances to create a bound-state-in-the-continuum.

DOI
10.1007/s00601-024-01930-4

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Abstract We provide an overview of experiments exploring resonances in the collision of ultracold clouds of atoms. Using a laser-based accelerator that capitalises on the energy resolution provided by the ultracold atomic setting, we unveil resonance phenomena such as Feshbach and shape resonances in their quintessential form by literally photographing the halo of outgoing scattered atoms. We exploit the tunability of magnetic Feshbach resonances to instigate an interplay between scattering resonances. By experimentally recording the scattering in a parameter space spanned by collision energy and magnetic field, we capture the imprint of the S -matrix pole flow in the complex energy plane. After revisiting experiments that place a Feshbach resonance in the proximity of a shape resonance and an anti-bound state, respectively, we discuss the possibility of using S -matrix pole interplay between two Feshbach resonances to create a bound-state-in-the-continuum.
In quantum mechanics, collisions between two particles are captured by a scattering matrix which describes the transfer from an initial entrance state to an outgoing final state. Analyticity of the elements of this SSS matrix enables their continuation onto the complex energy plane and opens up a powerful and widely used framework in scattering theory, where bound states and scattering resonances for a physical system are ascribed to SSS-matrix poles. In the Gedankenexperiment of gradually changing the potential parameters of the system, the complex energy poles will begin to move, and in their ensuing flow, two poles approaching will interact. An actual observation of this intriguing interaction between scattering poles in a collision experiment has, however, been elusive. Here, we expose the interplay between two scattering poles relating to a shape resonance and a magnetically tunable Feshbach resonance by studying ultracold atoms with a laser-based collider. We exploit the tunability of the Feshbach resonance to observe a compelling avoided crossing of the poles in their energies which is the hallmark of a strongly coupled system.
Ultracold atomic gases have realized numerous paradigms of condensed matter physics, where control over interactions has crucially been afforded by tunable Feshbach resonances. So far, the characterization of these Feshbach resonances has almost exclusively relied on experiments in the threshold regime near zero energy. Here, we use a laser-based collider to probe a narrow magnetic Feshbach resonance of rubidium above threshold. By measuring the overall atomic loss from colliding clouds as a function of magnetic field, we track the energy-dependent resonance position. At higher energy, our collider scheme broadens the loss feature, making the identification of the narrow resonance challenging. However, we observe that the collisions give rise to shifts in the center-of-mass positions of outgoing clouds. The shifts cross zero at the resonance and this allows us to accurately determine its location well above threshold. Our inferred resonance positions are in excellent agreement with theory.Studies on energy-dependent scattering of ultracold atoms were previously carried out near zero collision energies. Here, the authors observe a magnetic Feshbach resonance in ultracold Rb collisions for above-threshold energies and their method can also be used to detect higher partial wave resonances.
Abstract Ultracold atomic gases have realized numerous paradigms of condensed matter physics, where control over interactions has crucially been afforded by tunable Feshbach resonances. So far, the characterization of these Feshbach resonances has almost exclusively relied on experiments in the threshold regime near zero energy. Here, we use a laser-based collider to probe a narrow magnetic Feshbach resonance of rubidium above threshold. By measuring the overall atomic loss from colliding clouds as a function of magnetic field, we track the energy-dependent resonance position. At higher energy, our collider scheme broadens the loss feature, making the identification of the narrow resonance challenging. However, we observe that the collisions give rise to shifts in the center-of-mass positions of outgoing clouds. The shifts cross zero at the resonance and this allows us to accurately determine its location well above threshold. Our inferred resonance positions are in excellent agreement with theory.
Due to atomic interactions, a dilute gas Bose-Einstein condensate acquires a self- energy proportional to the two-body scattering length a. This self-energy strongly influences the stability, formation rate, size and shape, collective excitations, and other properties of a condensate. For a given atomic species at zero magnetic field, the scattering length is fixed, and this had led to a rather limited range of interaction strengths in experiments. However, it has been predicted that a magnetically tunable Feshbach resonance could be used to strongly modify scattering lengths [1]. We have observed such a Feshbach resonance in collisions of ultracold 85Rb(f =2, mf=−2) atoms in a magnetic field B. From our measured resonance position and width, we infer that the scattering length a2,−2 for collisions of these atoms has the dispersive resonance form.
We employ a quantum defect theory framework to provide a detailed analysis of the interplay between a magnetic Feshbach resonance and a shape resonance in cold collisions of ultracold 87Rb^{87}\mathrm{Rb}87Rb atoms as captured in recent experiments using a laser-based collider [M. Chilcott et al., Phys. Rev. Research 3, 033209 (2021)]. By exerting control over a parameter space spanned by both collision energy and magnetic field, the width of a Feshbach resonance can be tuned over several orders of magnitude. We apply a quantum defect theory specialized for ultracold atomic collisions to fully describe of the experimental observations. While the width of a Feshbach resonance generally increases with collision energy, its coincidence with a shape resonance leads to a significant additional boost. By conducting experiments at a collision energy matching the shape resonance and using the shape resonance as a magnifying lens, we demonstrate a feature broadening to a magnetic width of 8 G compared to a predicted Feshbach resonance width much less than 0.10.10.1 mG.
We observe magnetically tuned collision resonances for ultracold Cs2 molecules stored in a CO2-laser trap. By magnetically levitating the molecules against gravity, we precisely measure their magnetic moment. We find an avoided level crossing which allows us to transfer the molecules into another state. In the new state, two Feshbach-like collision resonances show up as strong inelastic loss features. We interpret these resonances as being induced by Cs4 bound states near the molecular scattering continuum. The tunability of the interactions between molecules opens up novel applications such as controlled chemical reactions and synthesis of ultracold complex molecules.