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arXiv:2405.02453 · Physical Review Research

N -way parametric frequency beamsplitter for quantum photonics

Richard C. Oliver, Miri Blau, Chaitali Joshi, Xingchen Ji, R. Gutiérrez-Jáuregui, Ana Asenjo-Garcı́a, Michal F. Lipson, Alexander L. Gaeta

Published May 1, 2025• 9 citations

Abstract

Optical networks are the leading platform for the transfer of information due to their low loss and ability to scale to many information channels using optical frequency modes. To fully leverage the quantum properties of light in this platform, it is desired to manipulate higher-dimensional superpositions by orchestrating linear, beamsplitter-type interactions between several channels simultaneously. We propose a method of achieving simultaneous, all-to-all coupling between N optical frequency modes via N -way Bragg-scattering four-wave mixing. By exploiting the frequency degree of freedom, additional modes can be multiplexed in an interaction medium of fixed volume and loss while avoiding the introduction of excess noise. We generalize the theory of the frequency-encoded two-mode interaction to N modes under this four-wave-mixing approach, finding that arbitrary unitary transformations are possible through successive four-wave-mixing pump configurations. We experimentally verify the quantum nature of this scheme by demonstrating three-way multiphoton interference. Two input photons are shared among three frequency modes and display interference differing from that of two classical (coherent-state) inputs. These results show the potential of our approach for the scalability of photonic quantum information processing to general N -mode systems in the frequency domain.

DOI: 10.1103/physrevresearch.7.023108

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Quantum information is the next frontier in information science, promising unconditionally secure communications, enhanced channel capacities, and computing capabilities far beyond their classical counterparts. And as quantum information processing devices continue to transition from the lab to the field, the demand for the foundational infrastructure connecting them with each other and their users---the quantum internet---will only increase. Due to the remarkable success of frequency multiplexing and control in the classical internet, quantum information encoding in optical frequency offers an intriguing synergy with state-of-the-art fiber-optic networks. Yet coherent quantum frequency operations prove extremely challenging, due to the difficulties in mixing frequencies efficiently, arbitrarily, in parallel, and with low noise. Here we implement an original approach based on a reconfigurable quantum frequency processor, designed to perform arbitrary manipulations of spectrally encoded qubits. This processor's unique tunability allows us to demonstrate frequency-bin Hong-Ou-Mandel interference with record-high 94% visibility. Furthermore, by incorporating such tunability with our method's natural parallelizability, we synthesize independent quantum frequency gates in the same device, realizing the first high-fidelity flip of spectral correlations on two entangled photons. Compared to quantum frequency mixing approaches based on nonlinear optics, our linear method removes the need for additional pump fields and significantly reduces background noise. Our results demonstrate multiple functionalities in parallel in a single platform, representing a huge step forward for the frequency-multiplexed quantum internet.

Frequency-bin encoding has recently emerged as a powerful approach for photonic quantum information processing, offering high dimensionality, gate-parallelization, and compatibility with existing telecommunication infrastructure. However, its scalable deployment has so far been hindered by the lack of an integrated platform capable of unifying quantum state generation, coherent frequency mixing, and programmable spectral control.\\ Here, we report the first fully integrated quantum frequency processor, monolithically integrating on the same silicon photonic chip a microresonator-based biphoton quantum frequency comb source, a pump-rejection filter, high-speed phase modulators, and a four-channel, line-by-line pulse shaper. We demonstrate key functionalities, such as tunable frequency beamsplitters with success probabilities exceeding

94\%

and fidelities above

99.9\%

, as well as the ability to synthesize more general single-qubit gates. Finally, we generate and coherently manipulate high-dimensional frequency-bin entangled states entirely on chip, showcasing control over two-photon quantum walks and performing the first on-chip frequency-bin quantum state tomography of a Bell-state with a fidelity of

95.7(3)\%

. By integrating all key functional elements on the same

4\times7\,\textrm{mm}^2

chip, with the possibility of scaling to a larger number of modes, our work marks an important step toward large-scale frequency-domain photonic processors for both classical and quantum applications.

In this paper, we propose a novel method for interfering frequency-multiplexed photonic quantum states without the use of optical nonlinear effects, and experimentally demonstrate this technique via frequency-domain Hong-Ou-Mandel (HOM) interference. By cascading the generation of quantum states onto arbitrary orthogonal modes, we can induce interference across any desired frequency mode. Following the generation of quantum states onto the frequency modes, performing measurements in independent frequency bands enables the realisation of a frequency-domain linear optical circuit analogous to linear interference in the spatial domain. We successfully demonstrated programmable quantum interference by controlling the spectral mode functions and measurement bases. Our method offers a new approach to harness the full potential of light's temporal-frequency degrees of freedom, providing a path towards scalable and programmable photonic quantum computing architectures without the need for optical nonlinearities or spatial-mode beam splitters.

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