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arXiv:2003.06533 · Physical Review Letters

Frequency-Domain Quantum Interference with Correlated Photons from an Integrated Microresonator

Chaitali Joshi, Alessandro Farsi, Avik Dutt, Bok Young Kim, Xingchen Ji, Yun Zhao, Andrew M. Bishop, Michal F. Lipson, Alexander L. Gaeta

Published Apr 6, 2020• 74 citations
arXivHTMLPDF

Abstract

Frequency encoding of quantum information together with fiber and integrated photonic technologies can significantly reduce the complexity and resource requirements for realizing all-photonic quantum networks. The key challenge for such frequency domain processing of single photons is to realize coherent and selective interactions between quantum optical fields of different frequencies over a range of bandwidths. Here, we report frequency-domain Hong-Ou-Mandel interference with spectrally distinct photons generated from a chip-based microresonator. We use four-wave mixing to implement an active "frequency beam splitter" and achieve interference visibilities of 0.95±0.02. Our work establishes four-wave mixing as a tool for selective high-fidelity two-photon operations in the frequency domain which, combined with integrated single-photon sources, provides a building block for frequency-multiplexed photonic quantum networks.

DOI
10.1103/physrevlett.124.143601

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Frequency encoding of quantum information together with fiber and integrated photonic technologies can significantly reduce the complexity and resource requirements for realizing all-photonic quantum networks. The key challenge for such frequency domain processing of single photons is to realize coherent and selective interactions between quantum optical fields of different frequencies over a range of bandwidths. Here, we report frequency-domain Hong-Ou-Mandel interference with spectrally distinct photons generated from a chip-based microresonator. We use four-wave mixing to implement an active "frequency beam splitter" and achieve interference visibilities of 0.95±0.02. Our work establishes four-wave mixing as a tool for selective high-fidelity two-photon operations in the frequency domain which, combined with integrated single-photon sources, provides a building block for frequency-multiplexed photonic quantum networks.
Abstract The photon's frequency degree of freedom, being compatible with mature telecom infrastructure, offers large potential for the stable and controllable realization of photonic quantum processing applications such as the quantum internet. The Hong–Ou–Mandel effect, as a two‐photon interference phenomenon, serves as a central building block for such frameworks. A key element yet missing to enable meaningful frequency‐based implementations as well as scalability in the number of processed photons, is the demonstration of the Hong–Ou–Mandel effect between independently created photons of different frequencies. The experimental implementation of bosonic and fermionic frequency domain Hong–Ou–Mandel interference between independently generated single photons is reported here, with measured visibilities of 74.31% ± 3.56% and 86.44% ± 8.27%, respectively. This is achieved through a scalable photonic frequency circuit that creates two post‐selected pure single photons, which undergo frequency mixing at an electro‐optic phase modulator. The system is on‐the‐fly reconfigurable allowing to probe bosonic and fermionic Hong–Ou–Mandel interference in the same experimental setup. The work demonstrates the versatility of frequency domain processing and its scalability toward higher photon numbers, which enables new quantum gate concepts as well as the establishment of frequency‐based large‐scale quantum networks.
Quantum information is the next frontier in information science, promising unconditionally secure communications, enhanced channel capacities, and computing capabilities far beyond their classical counterparts. And as quantum information processing devices continue to transition from the lab to the field, the demand for the foundational infrastructure connecting them with each other and their users---the quantum internet---will only increase. Due to the remarkable success of frequency multiplexing and control in the classical internet, quantum information encoding in optical frequency offers an intriguing synergy with state-of-the-art fiber-optic networks. Yet coherent quantum frequency operations prove extremely challenging, due to the difficulties in mixing frequencies efficiently, arbitrarily, in parallel, and with low noise. Here we implement an original approach based on a reconfigurable quantum frequency processor, designed to perform arbitrary manipulations of spectrally encoded qubits. This processor's unique tunability allows us to demonstrate frequency-bin Hong-Ou-Mandel interference with record-high 94% visibility. Furthermore, by incorporating such tunability with our method's natural parallelizability, we synthesize independent quantum frequency gates in the same device, realizing the first high-fidelity flip of spectral correlations on two entangled photons. Compared to quantum frequency mixing approaches based on nonlinear optics, our linear method removes the need for additional pump fields and significantly reduces background noise. Our results demonstrate multiple functionalities in parallel in a single platform, representing a huge step forward for the frequency-multiplexed quantum internet.
Hong-Ou-Mandel (HOM) interference is a compelling quantum phenomenon that demonstrates the nonclassical nature of single photons. In this study, we investigate an electromagnetically induced transparency-based double-$\mathrm{\ensuremath{\Lambda}}$ four-wave mixing system from the perspective of quantized light fields. The system can be used to realize efficient HOM interference in the frequency domain. By using the reduced density operator theory, we demonstrate that although the double-$\mathrm{\ensuremath{\Lambda}}$ medium does not exhibit phase-dependent properties for the closed-loop case of two incident single photons, frequency-domain HOM two-photon interference occurs. For experimentally achievable optical depth conditions, our theory indicates that this double-$\mathrm{\ensuremath{\Lambda}}$ scheme can perform high-fidelity Hadamard gate operations on frequency-encoded single-photon qubits, and thereby generate HOM two-photon NOON states with a fidelity greater than 0.99. Furthermore, we demonstrate that this scheme can be used to realize arbitrary single-qubit gates and two-qubit SWAP gates by simply controlling the laser detuning and phase, exhibiting its multifunctional properties and providing a different route to scalable optical quantum computing.
The exploration of photonic systems for quantum information processing has generated widespread interest in multiple cutting-edge research fields. Photonic frequency encoding stands out as an especially viable approach, given its natural alignment with established optical communication technologies, including fiber networks and wavelength-division multiplexing systems. Substantial reductions in hardware resources and improvements in quantum performance can be expected by utilizing multiple frequency modes. The integration of nonlinear photonics with microresonators provides a compelling way for generating frequency-correlated photon pairs across discrete spectral modes. Here, by leveraging the high material nonlinearity and low nonlinear loss, we demonstrate an efficient chip-scale multi-wavelength quantum light source based on AlGaAs-on-insulator, featuring a free spectral range of approximately 200 GHz at telecom wavelengths. The optimized submicron waveguide geometry provides both high effective nonlinearity (~550 m−1^{-1}−1W−1^{-1}−1) and broad generation bandwidth, producing eleven distinct wavelength pairs across a 35.2 nm bandwidth with an average spectral brightness of 2.64 GHz mW−2^{-2}−2nm−1^{-1}−1. The generation of energy-time entanglement for each pair of frequency modes is verified through Franson interferometry, yielding an average net visibility of 93.1%. With its exceptional optical gain and lasing capabilities, the AlGaAs-on-insulator platform developed here shows outstanding potential for realizing fully integrated, ready-to-deploy quantum photonic systems on chip.