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arXiv:2404.19551 · Physical Review Research

Formation of Rydberg crystals induced by quantum melting in one dimension

Zeki Zeybek, Peter Schmelcher, Rick Mukherjee

Published Jan 13, 2025• 4 citations
arXivHTMLPDF

Abstract

Quantum fluctuations in frustrated systems can lead to the emergence of complex many-body phases. However, the role of quantum fluctuations in frustration-free lattices is less explored and could provide an interesting avenue for exploring new physics, and perhaps is easier to realize compared to frustrated lattice systems. Using Rydberg atoms with tunable interactions as a platform, we leverage strong van der Waals interactions and obtain a constrained model in one dimension with nonlocal fluctuations given by dipolar interactions alongside local fluctuations. The combined effect of such processes leads to intrinsically quantum-ordered Rydberg crystals through the order-by-disorder mechanism. Finite-size analyses indicate that combined fluctuations drive the transition from disordered to ordered phases, contrary to the expected direction. We provide a theoretical description to understand the physics of order-by-disorder in one-dimensional systems, which are typically seen only in higher dimensions.

DOI
10.1103/physrevresearch.7.l012009

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Quantum fluctuations in frustrated systems can lead to the emergence of complex many-body phases. However, the role of quantum fluctuations in frustration-free lattices is less explored and could provide an interesting avenue for exploring new physics, and perhaps is easier to realize compared to frustrated lattice systems. Using Rydberg atoms with tunable interactions as a platform, we leverage strong van der Waals interactions and obtain a constrained model in one dimension with nonlocal fluctuations given by dipolar interactions alongside local fluctuations. The combined effect of such processes leads to intrinsically quantum-ordered Rydberg crystals through the order-by-disorder mechanism. Finite-size analyses indicate that combined fluctuations drive the transition from disordered to ordered phases, contrary to the expected direction. We provide a theoretical description to understand the physics of order-by-disorder in one-dimensional systems, which are typically seen only in higher dimensions.
We describe the zero-temperature phase diagram of a model of a two-dimensional square-lattice array of neutral atoms, excited into Rydberg states and interacting via strong van der Waals interactions. Using the density-matrix renormalization group algorithm, we map out the phase diagram and obtain a rich variety of phases featuring complex density wave orderings, upon varying lattice spacing and laser detuning. While some of these phases result from the classical optimization of the van der Waals energy, we also find intrinsically quantum-ordered phases stabilized by quantum fluctuations. These phases are surrounded by novel quantum phase transitions, which we analyze by finite-size scaling numerics and Landau theories. Our work highlights Rydberg quantum simulators in higher dimensions as promising platforms to realize exotic many-body phenomena.
Competing short- and long-range interactions represent distinguished ingredients for the formation of complex quantum many-body phases. Their study is hard to realize with conventional quantum simulators. In this regard, Rydberg atoms provide an exception as their excited manifold of states have both density-density and exchange interactions whose strength and range can vary considerably. Focusing on one-dimensional systems, we leverage the Van der Waals and dipole-dipole interactions of the Rydberg atoms to obtain the zero-temperature phase diagram for a uniform chain and a dimer model. For the uniform chain, we can influence the boundaries between ordered phases and a Luttinger liquid phase. For the dimerized case, a new type of bond-order-density-wave phase is identified. This demonstrates the versatility of the Rydberg platform in studying physics involving short- and long-ranged interactions simultaneously.
Abstract. We discuss the many-body physics of an ensemble of Rydberg dressed atoms with van der Waals dipole-dipole interactions in a one-dimensional lattice. Using a strong coupling expansion and numerical density-matrix renormalisation group simulations, we calculate the many-body phase diagram. A devil’s staircase structure emerges with Mott-insulating phases at any rational filling fraction. Closed analytic expressions are given for the phase boundaries in second order of the tunnelling amplitude and shown to agree very well with the numerical results. The transition point where the incompressible phases melt due to the kinetic energy term depends strongly on the denominator of the filling fraction and varies over many orders of magnitude between different phases.
We discuss the many-body physics of an ensemble of Rydberg dressed atoms with van der Waals dipole–dipole interactions in a one-dimensional lattice. Using a strong coupling expansion and numerical density-matrix renormalization group simulations, we calculate the many-body phase diagram. A devil's staircase structure emerges with Mott-insulating phases at any rational filling fraction. Closed analytic expressions are given for the phase boundaries in second order of the tunneling amplitude and are shown to agree very well with the numerical results. The transition point where the incompressible phases melt due to the kinetic energy term depends strongly on the denominator of the filling fraction and varies over many orders of magnitude between different phases.
We investigate the zero-temperature phase diagram of a one-dimensional constrained quantum spin chain realized in coherently driven Rydberg-atom arrays with competing local Rabi driving and dipole-dipole exchange interactions. Projecting onto the blockade-constrained Hilbert space yields an effective model in which local and nonlocal quantum fluctuations compete on equal footing. Combining exact diagonalization, the density-matrix renormalization group, and variational uniform matrix-product-state calculations, we establish a complete phase diagram comprising a Luttinger liquid, an antiferromagnetic ordered phase, and a polarized paramagnet. We identify two distinct mechanisms for the destruction of antiferromagnetic order: a conventional Ising transition at strong driving and a continuous quantum melting into the Luttinger liquid at weak driving, characterized using entanglement-based diagnostics and finite-entanglement scaling. In addition, we uncover an exact ground-state factorization line embedded within the ordered phase, providing an analytically tractable zero-entanglement reference point for experiments with programmable Rydberg quantum simulators.
We consider cold Rydberg atoms in a one-dimensional optical lattice in the Mott regime with a single atom per site at zero temperature. An external laser drive with Rabi frequency $\ensuremath{\Omega}$ and laser detuning $\ensuremath{\Delta}$ creates Rydberg excitations whose dynamics is governed by an effective spin-chain model with (quasi) long-range interactions. This system possesses intrinsically a large degree of frustration resulting in a ground-state phase diagram in the $(\ensuremath{\Delta},\ensuremath{\Omega})$ plane with a rich topology. As a function of $\ensuremath{\Delta}$, the Rydberg blockade effect gives rise to a series of crystalline phases commensurate with the optical lattice that form a so-called devil's staircase. The Rabi frequency $\ensuremath{\Omega}$, on the other hand, creates quantum fluctuations that eventually lead to a quantum melting of the crystalline states. Upon increasing $\ensuremath{\Omega}$, we find that generically a commensurate-incommensurate transition to a floating Rydberg crystal that supports gapless phonon excitations occurs first. For even larger $\ensuremath{\Omega}$, dislocations within the floating Rydberg crystal start to proliferate and a second, Kosterlitz-Thouless-Nelson-Halperin-Young dislocation-mediated melting transition finally destroys the crystalline arrangement of Rydberg excitations. This latter melting transition is generic for one-dimensional Rydberg crystals and persists even in the absence of an optical lattice. The floating phase and the concomitant transitions can, in principle, be detected by Bragg scattering of light.