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arXiv:1104.2603 · Physical Review B

Dislocation-mediated melting of one-dimensional Rydberg crystals

Eran Sela, Matthias Punk, Markus Garst

Published Aug 29, 2011• 61 citations
arXivHTMLPDF

Abstract

We consider cold Rydberg atoms in a one-dimensional optical lattice in the Mott regime with a single atom per site at zero temperature. An external laser drive with Rabi frequency $\ensuremath{\Omega}$ and laser detuning $\ensuremath{\Delta}$ creates Rydberg excitations whose dynamics is governed by an effective spin-chain model with (quasi) long-range interactions. This system possesses intrinsically a large degree of frustration resulting in a ground-state phase diagram in the $(\ensuremath{\Delta},\ensuremath{\Omega})$ plane with a rich topology. As a function of $\ensuremath{\Delta}$, the Rydberg blockade effect gives rise to a series of crystalline phases commensurate with the optical lattice that form a so-called devil's staircase. The Rabi frequency $\ensuremath{\Omega}$, on the other hand, creates quantum fluctuations that eventually lead to a quantum melting of the crystalline states. Upon increasing $\ensuremath{\Omega}$, we find that generically a commensurate-incommensurate transition to a floating Rydberg crystal that supports gapless phonon excitations occurs first. For even larger $\ensuremath{\Omega}$, dislocations within the floating Rydberg crystal start to proliferate and a second, Kosterlitz-Thouless-Nelson-Halperin-Young dislocation-mediated melting transition finally destroys the crystalline arrangement of Rydberg excitations. This latter melting transition is generic for one-dimensional Rydberg crystals and persists even in the absence of an optical lattice. The floating phase and the concomitant transitions can, in principle, be detected by Bragg scattering of light.

DOI
10.1103/physrevb.84.085434

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We consider cold Rydberg atoms in a one-dimensional optical lattice in the Mott regime with a single atom per site at zero temperature. An external laser drive with Rabi frequency \ensuremathΩ\ensuremath{\Omega}\ensuremathΩ and laser detuning \ensuremathΔ\ensuremath{\Delta}\ensuremathΔ creates Rydberg excitations whose dynamics is governed by an effective spin-chain model with (quasi) long-range interactions. This system possesses intrinsically a large degree of frustration resulting in a ground-state phase diagram in the (\ensuremathΔ,\ensuremathΩ)(\ensuremath{\Delta},\ensuremath{\Omega})(\ensuremathΔ,\ensuremathΩ) plane with a rich topology. As a function of \ensuremathΔ\ensuremath{\Delta}\ensuremathΔ, the Rydberg blockade effect gives rise to a series of crystalline phases commensurate with the optical lattice that form a so-called devil's staircase. The Rabi frequency \ensuremathΩ\ensuremath{\Omega}\ensuremathΩ, on the other hand, creates quantum fluctuations that eventually lead to a quantum melting of the crystalline states. Upon increasing \ensuremathΩ\ensuremath{\Omega}\ensuremathΩ, we find that generically a commensurate-incommensurate transition to a floating Rydberg crystal that supports gapless phonon excitations occurs first. For even larger \ensuremathΩ\ensuremath{\Omega}\ensuremathΩ, dislocations within the floating Rydberg crystal start to proliferate and a second, Kosterlitz-Thouless-Nelson-Halperin-Young dislocation-mediated melting transition finally destroys the crystalline arrangement of Rydberg excitations. This latter melting transition is generic for one-dimensional Rydberg crystals and persists even in the absence of an optical lattice. The floating phase and the concomitant transitions can, in principle, be detected by Bragg scattering of light.
We investigate the quantum melting of one-dimensional crystals that are realized in an atomic lattice in which ground state atoms are laser excited to two Rydberg states. We focus on a regime where both, intra- and interstate density-density interactions as well as coherent exchange interactions contribute. We determine stable crystalline phases in the classical limit and explore their melting under quantum fluctuations introduced by the excitation laser as well as two-body exchange. We find that within a specific parameter range quantum fluctuations introduced by the laser can give rise to a devil's staircase structure which one might associate with transitions in the classical limit. The melting through exchange interactions is shown to also proceed in a steplike fashion, in the case of small crystals, due to the proliferation of Rydberg spin waves.
We analyze the ground state properties of a one-dimensional cold atomic system in a lattice, where Rydberg excitations are created by an external laser drive. In the classical limit, the ground state is characterized by a complete devil's staircase for the commensurate solid structures of Rydberg excitations. Using perturbation theory and a mapping onto an effective low-energy Hamiltonian, we find a transition of these commensurate solids into a floating solid with algebraic correlations. For stronger quantum fluctuations the floating solid eventually melts within a second quantum phase transition and the ground state becomes paramagnetic.
We study the ground-state phase diagram of Rydberg atoms in a triangular-prism optical tweezer array using the density matrix renormalization group. By tuning the detuning-to-Rabi-frequency ratio and the Rydberg blockade radius, the system realizes several density-wave phases with spontaneous breaking of translational and leg-exchange symmetries. Unlike two-leg Rydberg ladders with Z2\mathbb{Z}_2Z2​ leg-exchange symmetry, the triangular prism has D3\mathbb{D}_3D3​ symmetry, leading to a richer set of ordered phases and transitions. For blockade radius moderately larger than the lattice spacing, a phase with alternating double and single Rydberg occupancy appears at large detuning. It breaks Z2\mathbb{Z}_2Z2​ translational and Z3\mathbb{Z}_3Z3​ rotational symmetry while preserving a rung reflection symmetry. Upon decreasing detuning, it melts through two Berezinskii-Kosterlitz-Thouless transitions with an intermediate critical phase described by a Z6\mathbb{Z}_6Z6​ clock model. At larger blockade radius, a phase with one Rydberg excitation per triangle and broken D3\mathbb{D}_3D3​ symmetry appears through a first-order transition. When double occupation of neighboring triangles is suppressed, rung-trimerized density waves develop as detuning increases from the disordered phase. Their melting follows the same structure as in Rydberg chains and two-leg ladders: the Z2\mathbb{Z}_2Z2​ case has Ising critical lines, while the Z3\mathbb{Z}_3Z3​ and Z4\mathbb{Z}_4Z4​ cases have chiral critical lines, with Potts and Ashkin-Teller points only on the corresponding commensurate lines. Inside the Z2\mathbb{Z}_2Z2​ rung-trimerized phase, an entanglement-entropy peak signals a crossover regime with enhanced period-2 density modulation before a first-order transition into a Z2×D3\mathbb{Z}_2\times\mathbb{D}_3Z2​×D3​ phase. Floating phases with incommensurate quasi-long-range order appear between trimerized states of different periods.
Rydberg atoms have experimentally interestingproperties such as strong long-range Van der Waals interactions and the dipole blockade effect. In optical lattices the blockade effect ensures that only one Rydberg excitation per site is allowed, effectively creating a Rydberg crystal. We theoretically show that it is also possible for a one-dimensional Rydberg crystal to spontaneously form in a random ensemble of atoms, e.g. a magneto-optical trap. This is done using an existing Monte Carlo model [1] to simulate the excitation dynamics inside the intersection of two lasers for a two-step excitation scheme. With a blue-detuned laser for the upper transition, the first Rydberg excitation will occur after a relatively long time. That first Rydberg atom will then seed further Rydberg excitations, as the blockade effect shifts atoms at a certain distance into resonance. If two dimensions of the laser intersection are smaller than the blockade radius, a one-dimensional Rydberg crystal will form.
The floating phase, a critical incommensurate phase, has been theoretically predicted as a potential intermediate phase between crystalline ordered and disordered phases. In this study, we investigate the different quantum phases that arise in ladder arrays comprising up to 92 neutral-atom qubits and experimentally observe the emergence of the quantum floating phase. We analyze the site-resolved Rydberg state densities and the distribution of state occurrences. The site-resolved measurement reveals the formation of domain walls within the commensurate ordered phase, which subsequently proliferate and give rise to the floating phase with incommensurate quasi-long-range order. By analyzing the Fourier spectra of the Rydberg density-density correlations, we observe clear signatures of the incommensurate wave order of the floating phase. Furthermore, as the experimental system sizes increase, we show that the wave vectors approach a continuum of values incommensurate with the lattice. Our work motivates future studies to further explore the nature of commensurate-incommensurate phase transitions and their non-equilibrium physics. The critical floating phase can bridge crystalline orders and the disordered phase. Here, the authors experimentally observe the quantum floating phase in neutral atom qubit arrays, revealing domain walls and incommensurate quasi long-range order, and analyse its emergence via Fourier spectroscopy.
Abstract We examine the adiabatic preparation of crystalline phases of Rydberg excitations in a one-dimensional lattice gas by frequency sweep of the excitation laser, as proposed by Pohl et al (2010 Phys. Rev. Lett. 104 043002 ) and recently realized experimentally by Schauß et al (2015 Science 347 1455 ). We find that the preparation of crystals of a few Rydberg excitations in a unitary system of several tens of atoms requires exceedingly long times for the adiabatic following of the ground state of the system Hamiltonian. Using quantum stochastic (Monte Carlo) wavefunction simulations, we show that realistic decay and dephasing processes affecting the atoms during the preparation lead to a final state of the system that has only a small overlap with the target crystalline state. Yet, the final number and highly sub-Poissonian statistics of Rydberg excitations and their spatial order are little affected by the relaxations.