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arXiv:1511.09214 · Journal of Physics B Atomic Molecular and Optical Physics

On the adiabatic preparation of spatially-ordered Rydberg excitations of atoms in a one-dimensional optical lattice by laser frequency sweeps

David Petrosyan, Klaus Mølmer, Michael Fleischhauer

Published Apr 5, 2016• 11 citations
arXivHTMLPDF

Abstract

Abstract We examine the adiabatic preparation of crystalline phases of Rydberg excitations in a one-dimensional lattice gas by frequency sweep of the excitation laser, as proposed by Pohl et al (2010 Phys. Rev. Lett. 104 043002 ) and recently realized experimentally by Schauß et al (2015 Science 347 1455 ). We find that the preparation of crystals of a few Rydberg excitations in a unitary system of several tens of atoms requires exceedingly long times for the adiabatic following of the ground state of the system Hamiltonian. Using quantum stochastic (Monte Carlo) wavefunction simulations, we show that realistic decay and dephasing processes affecting the atoms during the preparation lead to a final state of the system that has only a small overlap with the target crystalline state. Yet, the final number and highly sub-Poissonian statistics of Rydberg excitations and their spatial order are little affected by the relaxations.

DOI
10.1088/0953-4075/49/8/084003

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Abstract We examine the adiabatic preparation of crystalline phases of Rydberg excitations in a one-dimensional lattice gas by frequency sweep of the excitation laser, as proposed by Pohl et al (2010 Phys. Rev. Lett. 104 043002 ) and recently realized experimentally by Schauß et al (2015 Science 347 1455 ). We find that the preparation of crystals of a few Rydberg excitations in a unitary system of several tens of atoms requires exceedingly long times for the adiabatic following of the ground state of the system Hamiltonian. Using quantum stochastic (Monte Carlo) wavefunction simulations, we show that realistic decay and dephasing processes affecting the atoms during the preparation lead to a final state of the system that has only a small overlap with the target crystalline state. Yet, the final number and highly sub-Poissonian statistics of Rydberg excitations and their spatial order are little affected by the relaxations.
We examine the adiabatic preparation of spatially-ordered Rydberg excitations of atoms in finite one-dimensional lattices by frequency-chirped laser pulses, as realized in a number of recent experiments simulating quantum Ising model. Our aims are to unravel the microscopic mechanism of the phase transition from the unexcited state of atoms to the antiferromagnetic-like state of Rydberg excitations by traversing an extended gapless phase, and to estimate the preparation fidelity of the target state in a moderately sized system amenable to detailed numerical analysis. We find that, in the basis of the bare atomic states, the system climbs the ladder of Rydberg excitations predominantly along the strongest-amplitude paths towards the final ordered state. We show that, despite its complexity, the interacting many-body system can be described as an effective two-level system involving a pair of lowest-energy instantaneous collective eigenstates of the time-dependent Hamiltonian. The final preparation fidelity of the target state can then be well approximated by the Landau-Zener formula, while the nonadiabatic population leakage during the passage can be estimated using a perturbative approach applied to the instantaneous collective eigenstates.
The competition between resonant optical excitation of Rydberg states of atoms and their strong, long-range van der Waals interaction results in spatial ordering of Rydberg excitations in a two-dimensional lattice gas, as observed in a recent experiment of Schau\ss{} et al. [Nature (London) 491, 87 (2012)]. Here we use semiclassical Monte Carlo simulations to obtain stationary states for hundreds of atoms in finite-size lattices. We show the formation of regular spatial structures of Rydberg excitations in a system of increasing size, and find highly sub-Poissonian distribution of the number of Rydberg excitations characterized by a large negative value of the Mandel QQQ parameter which is nearly independent of the system size.
We examine the adiabatic preparation of spatially ordered Rydberg excitations of atoms in finite one-dimensional lattices by frequency-chirped laser pulses, as realized in a number of recent experiments simulating quantum Ising model. Our aims are to unravel the microscopic mechanism of the phase transition from the unexcited state of atoms to the antiferromagneticlike state of Rydberg excitations by traversing an extended gapless phase and to estimate the preparation fidelity of the target state in a moderately sized system amenable to detailed numerical analysis. We show that, despite its complexity, the interacting many-body system can be described as an effective two-level system involving a pair of lowest-energy instantaneous collective eigenstates of the time-dependent Hamiltonian. The final preparation fidelity of the target state can then be well approximated by the Landau-Zener formula, while the nonadiabatic population leakage during the passage can be estimated using a perturbative approach applied to the instantaneous collective eigenstates.
Ultracold atomic gases have been used extensively in recent years to realize textbook examples of condensed matter phenomena. Recently, phase transitions to ordered structures have been predicted for gases of highly excited, 'frozen' Rydberg atoms. Such Rydberg crystals are a model for dilute metallic solids with tunable lattice parameters, and provide access to a wide variety of fundamental phenomena. We investigate theoretically how such structures can be created in four distinct cold atomic systems, by using tailored laser-excitation in the presence of strong Rydberg-Rydberg interactions. We study in detail the experimental requirements and limitations for these systems, and characterize the basic properties of small crystalline Rydberg structures in one, two and three dimensions.
Abstract. We describe the dynamical preparation of anisotropic crystalline phases obtained by laser-exciting ultracold Alkali atoms to Rydberg p-states where they interact via anisotropic van der Waals interactions. We develop a time-dependent variational mean field ansatz to model large, but finite two-dimensional systems in experimentally accessible parameter regimes, and we present numerical simulations to illustrate the dynamical formation of anisotropic Rydberg crystals. PACS numbers: 32.80.Ee,34.20.Cf,64.70.Tg
We study resonant optical excitations of strongly interacting Rydberg states of atoms in the presence of relaxations. We employ the quantum stochastic (Monte Carlo) wavefunctions to simulate the dissipative dynamics of tens of atoms in two-dimensional lattices. We show that under typical experimental conditions involving the slow Rydberg state decay and sizable relaxation of atomic coherences, on the timescale of several μs the atomic ensemble approaches a stationary state in which much of the quantum correlations between the atoms have decayed away. The steady state, however, exhibits strong classical correlations of Rydberg excitation probabilities.