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arXiv:2404.18163 · Physical review. E

Thermodynamic uncertainty relation for quantum entropy production

Domingos S. P. Salazar

Published Jul 11, 2024• 4 citations
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Abstract

In quantum thermodynamics, entropy production is usually defined in terms of the quantum relative entropy between two states. We derive a lower bound for the quantum entropy production in terms of the mean and variance of quantum observables, which we refer to as a thermodynamic uncertainty relation (TUR) for the entropy production. In the absence of coherence between the states, our result reproduces classic TURs in stochastic thermodynamics. For the derivation of the TUR, we introduce a lower bound for a quantum generalization of the χ^{2} divergence between two states and discuss its implications for stochastic and quantum thermodynamics, as well as the limiting case where it reproduces the quantum Cramér-Rao inequality.

DOI
10.1103/physreve.110.014118

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In quantum thermodynamics, entropy production is usually defined in terms of the quantum relative entropy between two states. We derive a lower bound for the quantum entropy production in terms of the mean and variance of quantum observables, which we refer to as a thermodynamic uncertainty relation (TUR) for the entropy production. In the absence of coherence between the states, our result reproduces classic TURs in stochastic thermodynamics. For the derivation of the TUR, we introduce a lower bound for a quantum generalization of the χ^{2} divergence between two states and discuss its implications for stochastic and quantum thermodynamics, as well as the limiting case where it reproduces the quantum Cramér-Rao inequality.
For classic systems, the thermodynamic uncertainty relation (TUR) states that the fluctuations of a current have a lower bound in terms of the entropy production. Some TURs are rooted in information theory, particularly derived from relations between observations (mean and variance) and dissimilarities, such as the Kullback-Leibler divergence, which plays the role of entropy production in stochastic thermodynamics. We generalize this idea for quantum systems, where we find a lower bound for the uncertainty of quantum observables given in terms of the quantum relative entropy. We apply the result to obtain a quantum thermodynamic uncertainty relation in terms of the quantum entropy production, valid for arbitrary dynamics and nonthermal environments.
The thermodynamic uncertainty relation (TUR) imposes a fundamental constraint between current fluctuations and entropy production, providing a refined formulation of the second law for micro- and nanoscale systems. Quantum violations of the classical TUR reveal genuinely quantum thermodynamic effects, which are essential for improving performance and enabling optimization in quantum technologies. In this work, we analyze the TUR in a class of paradigmatic quantum thermal-machine models whose operation is enabled by coherent coupling between two energy levels forming a virtual qubit. Steady-state coherences are confined to this virtual-qubit subspace, while in the absence of coherent coupling the system satisfies detailed balance with the thermal reservoirs and supports no steady-state heat currents. We show that the steady-state currents and entropy production can be fully reproduced by an effective classical Markov process, whereas current fluctuations acquire an additional purely quantum correction originating from coherence. As a result, the thermodynamic uncertainty naturally decomposes into a classical (diagonal) contribution and a coherent contribution. The latter becomes negative under resonant conditions and reaches its minimum at the coupling strength that maximizes steady-state coherence. We further identify the conditions for minimizing the thermodynamic uncertainty, and the criteria for surpassing the classical TUR bound in the vicinity of the reversible limit.
Thermodynamic uncertainty relations (TURs) and kinetic uncertainty relations (KURs) provide tradeoff relations between measurement fluctuation and thermodynamic cost, such as entropy production and activity. Conventionally, these relations are derived using the Cramér-Rao inequality, which involves an auxiliary perturbation in deterministic differential equations governing the time evolution of the system’s probability distribution. In this study, without relying on the previous formulation based on a deterministic evolving equation, we demonstrate that the main previously discovered uncertainty relations can be derived solely through the stochastic representation of the same dynamics. For this purpose, we propose a unified method based on stochastic representations for general Markovian dynamics. Extending beyond classical systems, we apply this method to Markovian open quantum systems by unraveling their dynamics, deriving quantum uncertainty relations that are tighter than existing ones in regimes where quantum effects play a significant role. This fully establishes uncertainty relations for both classical and quantum systems as intrinsic properties of their stochastic nature. Thermodynamic and kinetic uncertainty relations describe trade-offs between measurement fluctuations and thermodynamic costs, such as entropy production and activity. In this work, the authors present a general framework for deriving uncertainty relations in classical and quantum systems, leveraging the intrinsic stochastic properties of these systems.
To reveal the role of the quantumness in the Otto cycle and to discuss the validity of the thermodynamic uncertainty relation (TUR) in the cycle, we study the quantum Otto cycle and its classical counterpart. In particular, we calculate exactly the mean values and relative error of thermodynamic quantities. In the quasistatic limit, quantumness reduces the productivity and precision of the Otto cycle compared to that in the absence of quantumness, whereas in the finite-time mode, it can increase the cycle's productivity and precision. Interestingly, as the strength (heat conductance) between the system and the bath increases, the precision of the quantum Otto cycle overtakes that of the classical one. Testing the conventional TUR of the Otto cycle, in the region where the entropy production is large enough, we find a tighter bound than that of the conventional TUR. However, in the finite-time mode, both quantum and classical Otto cycles violate the conventional TUR in the region where the entropy production is small. This implies that another modified TUR is required to cover the finite-time Otto cycle. Finally, we discuss the possible origin of this violation in terms of the uncertainty products of the thermodynamic quantities and the relative error near resonance conditions.
Symmetry breaking with respect to the time reversal characterizes entropy production. This viewpoint induces us to regard thermodynamic uncertainty relation (TUR), stating that higher precision can be achieved at the cost of higher entropy production, as a relation between precision and the extent of symmetry breaking. In this Letter, we formalize a TUR as symmetry breaking in quantum Markov processes, where the extent of symmetry breaking constitutes the thermodynamic cost. We derive a TUR for quantum continuous measurement, which holds for any conceivable continuous measurement. We demonstrate that counting- and current-type TURs can be obtained as particular cases of the obtained bound.
We derive a thermodynamic uncertainty relation (TUR) under quantum continuous measurement and feedback control. By incorporating the quantum-classical-transfer entropy, which quantifies the information gained by continuous measurement, we show that the precision of currents is constrained by information-thermodynamic costs such as the entropy production and information gain. Our result shows that information gain has the potential to enhance the precision of currents beyond the bounds set by the conventional TUR. We illustrate the bound with a driven two-level system under continuous measurement and feedback, demonstrating that feedback achieves higher precision of currents while suppressing the entropy production.