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arXiv:2404.16229 · Physical review. B./Physical review. B

Two-qubit gate with macroscopic singlet-triplet qubits in synthetic spin-one chains in InAsP quantum dot nanowires

Hassan Allami, Daniel Miravet, Marek Korkusiński, Paweł Hawrylak

Published Mar 5, 2025• 1 citation
arXivHTMLPDF

Abstract

We present a theory of a two-qubit gate with macroscopic singlet-triplet (ST) qubits in synthetic spin-one chains in InAsP quantum dot nanowires. The macroscopic topologically protected singlet-triplet qubits are built with two spin-half Haldane quasiparticles. The Haldane quasiparticles are hosted by a synthetic spin-one chain realized in chains of InAsP quantum dots embedded in an InP nanowire, with four electrons each. The quantum dot nanowire is described by a Hubbard-Kanamori (HK) Hamiltonian derived from an interacting atomistic model. Using exact diagonalization and matrix product states tools, we demonstrate that the low-energy behavior of the HK Hamiltonian is effectively captured by an antiferromagnetic spin-one chain Hamiltonian. Next, we consider two macroscopic qubits and present a method for creating a tunable coupling between the two macroscopic qubits by inserting an intermediate control dot between the two chains. Finally, we propose and demonstrate two approaches for generating highly accurate two-ST qubit gates: (1) by controlling the length of each qubit and (2) by employing different background magnetic fields for the two qubits.

DOI
10.1103/physrevb.111.115403

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We present a theory of a two-qubit gate with macroscopic singlet-triplet (ST) qubits in synthetic spin-one chains in InAsP quantum dot nanowires. The macroscopic topologically protected singlet-triplet qubits are built with two spin-half Haldane quasiparticles. The Haldane quasiparticles are hosted by a synthetic spin-one chain realized in chains of InAsP quantum dots embedded in an InP nanowire, with four electrons each. The quantum dot nanowire is described by a Hubbard-Kanamori (HK) Hamiltonian derived from an interacting atomistic model. Using exact diagonalization and matrix product states tools, we demonstrate that the low-energy behavior of the HK Hamiltonian is effectively captured by an antiferromagnetic spin-one chain Hamiltonian. Next, we consider two macroscopic qubits and present a method for creating a tunable coupling between the two macroscopic qubits by inserting an intermediate control dot between the two chains. Finally, we propose and demonstrate two approaches for generating highly accurate two-ST qubit gates: (1) by controlling the length of each qubit and (2) by employing different background magnetic fields for the two qubits.
In this thesis I present a theory of a macroscopic singlet-triplet qubit in quantum dots embedded in nanowires, each containing 4 electrons and together simulating an artficial Haldane gap material. A Haldane gap material exhibits a 4-fold degenerate ground state separated by an energy gap from excitations. The ground state is equivalent to a degenerate spin-singlet and -triplet state. The 4 degenerate states exhibit the characteristics of spins-1/2 localized on either end of the chain. These states may be used as a coded qubit for quantum information processing. Using the effective mass approximation, I calculate single-particle energy levels of one and two quantum dots in a quantum wire. Using these energy levels I compute the Coulomb matrix elements of the interacting Hamiltonian. Using configuration interaction I demonstrate that the ground state of a quantum dot with 4 electrons is a spin-1 state. I then show that the two dot system behaves approximately like two spin-1 objects interacting via an antiferromagnetic Heisenberg Hamiltonian. While the Heisenberg model is approximate, the two dots have a spin-0 ground-state, indicating antiferromagnetic coupling. I then present a simpler spin model to illustrate the physical parameters which control this interaction. Finally, I present a brief solution to the Heisenberg Hamiltonian for finite spin-chains, and show how one can manipulate the singlet-triplet combined ground state of the spin-chain via localized magnetic field, realizing a singlet-triplet qubit in a macroscopic semiconductor device.
We present here the steps enabling the microscopic design of a synthetic spin-1 chain in an InAsP quantum dot (QD) array embedded in an InP nanowire. The chain is described by a two-leg multiorbital Hubbard Kanamori (HK) model with parameters obtained from the microscopic calculations of up to eight electrons in a single and double QD. In this HK model describing long arrays of QDs, using both exact diagonalization and matrix product state (MPS) tools, we demonstrate a fourfold quasidegenerate ground state separated from excited states by a finite energy gap similar to a Heisenberg spin-1 chain in the Haldane phase. We demonstrate characteristic behavior of spin-12\frac{1}{2}21​ quasiparticles at the edges of the chain by observing the magnetic field dependence of the low-energy spectrum as a function of the applied magnetic field. The applied magnetic field isolates the singlet and Sz=0{S}^{z}=0Sz=0 triplet states from the other triplet components emulating a singlet-triplet qubit but with macroscopic quantum states. Most importantly, the regions in parameter space where the low-energy spectrum of the multiorbital Hubbard chain yields a Heisenberg spin-1 chain spectrum are mapped out.
We study controllable exchange coupling between two singlet-triplet qubits. We start from the original second quantized Hamiltonian of a quadruple quantum dot system and obtain the effective spin-spin interaction between the two qubits using the projection operator method. Under a strong uniform external magnetic field and an inhomogeneous local micromagnetic field, the effective interqubit coupling is of the Ising type, and the coupling strength can be expressed in terms of quantum dot parameters. Finally, we discuss how to generate various two-qubit operations using this controllable coupling, such as entanglement generation, and a controlled-not gate.
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
We describe high-fidelity entangling gates between singlet-triplet qubits (STQs) which are coupled via one quantum state (QS). The QS can be provided by a quantum dot itself or by another confined system. The orbital energies of the QS are tunable using an electric gate close to the QS, which changes the interactions between the STQs independent of their single-qubit parameters. Short gating sequences exist for controlled not (cnot) operations. We show that realistic quantum dot setups permit excellent entangling operations with gate infidelities below ${10}^{\ensuremath{-}3}$, which is lower than the quantum error correction threshold of the surface code. We consider limitations from fabrication errors, hyperfine interactions, spin-orbit interactions, and charge noise in GaAs and Si heterostructures.