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arXiv:2404.07261 · Physical Review Letters

Exact Deconfined Gauge Structures in the Higher-Spin Yao-Lee Model: A Quantum Spin-Orbital Liquid with Spin Fractionalization and Non-Abelian Anyons

Zhengzhi Wu, J. X. Zhang, Hong Yao

Published Dec 5, 2024• 5 citations
arXivHTMLPDF

Abstract

The nonintegrable higher spin Kitaev honeycomb model has an exact Z_{2} gauge structure, which exclusively identifies quantum spin liquid in the half-integer spin Kitaev model. But its constraints for the integer-spin Kitaev model are much limited, and even trivially gapped insulators cannot be excluded. The physical implications of exact Z_{2} gauge structure, especially Z_{2} fluxes, in integer-spin models remain largely unexplored. In this Letter, we theoretically show that a spin-S Yao-Lee model [a spin-orbital model with SU(2) spin-rotation symmetry] possesses a topologically nontrivial quantum spin-orbital liquid ground state for any spin (both integer and half-integer spin) by constructing exact deconfined fermionic Z_{2} gauge charges. We further show that the conserved Z_{2} flux can also demonstrate the intriguing spin fractionalization phenomena in the non-Abelian topological order phase of the spin-1 Yao-Lee model. Its deconfined Z_{2} vortex excitation carries fractionalized spin-1/2 quantum number in the low-energy subspace, which is also a non-Abelian anyon. Our exact manifestation of spin fractionalization in an integer-spin model is rather rare in previous studies, and is absent in the Kitaev honeycomb model.

DOI
10.1103/physrevlett.133.236504

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The nonintegrable higher spin Kitaev honeycomb model has an exact Z_{2} gauge structure, which exclusively identifies quantum spin liquid in the half-integer spin Kitaev model. But its constraints for the integer-spin Kitaev model are much limited, and even trivially gapped insulators cannot be excluded. The physical implications of exact Z_{2} gauge structure, especially Z_{2} fluxes, in integer-spin models remain largely unexplored. In this Letter, we theoretically show that a spin-S Yao-Lee model [a spin-orbital model with SU(2) spin-rotation symmetry] possesses a topologically nontrivial quantum spin-orbital liquid ground state for any spin (both integer and half-integer spin) by constructing exact deconfined fermionic Z_{2} gauge charges. We further show that the conserved Z_{2} flux can also demonstrate the intriguing spin fractionalization phenomena in the non-Abelian topological order phase of the spin-1 Yao-Lee model. Its deconfined Z_{2} vortex excitation carries fractionalized spin-1/2 quantum number in the low-energy subspace, which is also a non-Abelian anyon. Our exact manifestation of spin fractionalization in an integer-spin model is rather rare in previous studies, and is absent in the Kitaev honeycomb model.
The higher spin Kitaev model prominently features the extensive locally conserved quantities the same as the spin-1/2 Kitaev honeycomb model, although it is not exactly solvable. It remains an open question regarding the physical meaning of these conserved quantities in the higher spin model. In this Letter, by introducing a Majorana parton construction for a general spin-S we uncover that these conserved quantities are exactly the Z_{2} gauge fluxes in the general spin-S model, including the case of spin-1/2. Particularly, we find an even-odd effect that the Z_{2} gauge charges are fermions in the half integer spin model, but are bosons in the integer spin model. We further prove that the fermionic Z_{2} gauge charges are always deconfined; hence, the half integer spin Kitaev model would have nontrivial spin liquid ground states regardless of interaction strengths in the Hamiltonian. The bosonic Z_{2} gauge charges of the integer spin model, on the other hand, could condense, leading to a trivial product state, and this is indeed the case at the anisotropic limit of the model.
The exactly solvable spin-1/2 Kitaev model on a honeycomb lattice has drawn significant interest, as it offers a pathway to realizing the long-sought-after quantum spin liquid. Building upon the Kitaev model, Yao and Lee introduced another exactly solvable model on an unusual star lattice featuring non-abelian spinons. The additional pseudospin degrees of freedom in this model could provide greater stability against perturbations, making this model appealing. However, a mechanism to realize such an interaction in a standard honeycomb lattice remains unknown. Here, we provide a microscopic theory to obtain the Yao-Lee model, on a honeycomb lattice by utilizing strong spin-orbit coupling of anions edge-shared between two e g ions in the exchange processes. This mechanism leads to the desired bond-dependent interaction among spins rather than orbitals, unique to our model, implying that the orbitals fractionalize into gapless Majorana fermions and fermionic octupolar excitations emerge. Since the conventional Kugel-Khomskii interaction also appears, we examine the phase diagram, including these interactions, using classical Monte Carlo simulations and exact diagonalization techniques. Our findings reveal a broad region of disordered states that break rotational symmetry in the bond energy, suggesting intriguing behavior reminiscent of a spin-orbital liquid.
The formation of quantum spin liquids in frustrated magnets represents an exciting possibility due to the rather exotic features they harbor, including fractionalized excitations and emergent gauge fields. \nUnfortunately, they are notoriously difficult to study as there are often no good analytical methods available and quantum Monte Carlo simulations are hindered by the negative sign problem. \nThe Kitaev honeycomb model is a notable exception of a frustrated quantum model which is exactly solvable and which hosts a number of distinct quantum spin liquid ground states. \nAs such, it allows for a rare opportunity to study the physics of spin liquids with full analytical control. \n \nIn this thesis, we study the fractionalization of spin-1/2 moments into Majorana fermions and an emergent Z2 gauge field in a generalization of the Kitaev honeycomb model to a number of three-dimensional lattices. \nWhile the excitations of the gauge field are always gapped, the fermionic quasiparticles may exhibit a gapless dispersion, forming fully two-dimensional Fermi surfaces, symmetry protected nodal lines, or topological Weyl nodes. \nWe show that one can deduce rather general constraints on the possible gapless excitations by making use of an object called the projective symmetry group. \nIn doing so we provide a scheme for classifying the various gapless Kitaev spin liquids. \nA thorough analysis is carried out for a number of these spin liquids, primarily investigating the stability of the gapless modes and the novel features resulting from their sometimes non-trivial topology, as well as their effects on certain equal-time correlation functions.
We study a frustrated two-dimensional lattice spin model with Kitaev-type interaction. The lattice is obtained from the honeycomb lattice by replacing half of its sites with triangles. Using the SO(3) Majorana representation of spin, the model is exactly mapped into a Z2{Z}_{2}Z2​ lattice gauge theory of complex fermions with standard Gauss law constraint. We show that the ground state of the model is a chiral spin liquid, and it has gapless excitations. The Chern number of the ground state is $\ifmmode\pm\else\textpm\fi{}1$, implying the existence of a chiral edge mode. The vortex excitation of the model is bound with a Majorana zero mode, such mode behaves as non-Abelian anyons.
The Yao-Lee model is an example of exactly solvable spin-orbital models that are generalizations of the original Kitaev honeycomb model with extra local orbital degrees of freedom. Similarly to the Kitaev model, both spin and orbital degrees of freedom are effectively represented using sets of three-flavored Majorana fermions. The Yao-Lee model exhibits a quantum spin liquid ground state with gapped and immobile Z2{Z}_{2}Z2​ fluxes and threefold degenerate itinerant Majorana fermions. Our work demonstrated that by introducing different time-reversal-symmetry- (TRS) breaking fields one can split the degeneracy of Majorana fermions and close the gap for some of the bands, thus changing its topology. We calculated a comprehensive topological phase diagram for the Yao-Lee model by considering various combinations of TRS-breaking fields. This investigation revealed the emergence of distinct topological regions, each separated by nodal lines, signifying an evolution in the model's topological properties. We also investigated the impact of vacancies in the system. Our findings revealed that while vacancies modify the low-energy spectrum of the model, their presence has a limited impact on the topological properties of the model, at least for small-enough concentrations.
Abstract Elementary excitations in entangled states such as quantum spin liquids may exhibit exotic statistics different from those obeyed by fundamental bosons and fermions. Non-Abelian anyons exist in a Kitaev spin liquid—the ground state of an exactly solvable model. A smoking-gun signature of these excitations, namely a half-integer quantized thermal Hall conductivity, was recently reported in α-RuCl3. While fascinating, a microscopic theory for this phenomenon remains elusive because the pure Kitaev model cannot display this effect in an intermediate magnetic field. Here we present a microscopic theory of the Kitaev spin liquid emerging between the low- and high-field states. Essential to this result is an antiferromagnetic off-diagonal symmetric interaction which allows the Kitaev spin liquid to protrude from the ferromagnetic Kitaev limit under a magnetic field. This generic model displays a strong field anisotropy, and we predict a wide spin liquid regime when the field is perpendicular to the honeycomb plane.