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arXiv:2404.00871 · Physical Review A

Quantum metrology of absorption and gain parameters using two-mode bright squeezed light

Mrunal Kamble, Jiaxuan Wang, G. S. Agarwal

Published May 16, 2024• 14 citations
arXivHTMLPDF

Abstract

Absorption and gain processes are fundamental to any light-matter interaction and a precise measurement of these parameters is important for various scientific and technological applications. Quantum probes, specifically the squeezed states, have proved very successful, particularly in the applications that deal with phase shift and force measurements. In this paper, we focus on improving the sensitivity of the estimation of the photon-loss coefficient of a weakly absorbing medium as well as the estimation of the gain parameter using a two-mode bright squeezed state. The generation of this state combines the advantage of a coherent beam for its large photon number with the quantum properties of the two-mode squeezing operation in an optical parametric amplifier. We present two measurement schemes: balanced photodetection and time-reversed metrology, both utilizing two-mode bright squeezed light. The maximum quantum advantage we can achieve using two-mode bright squeezed light is 3.7 times for the absorption parameter $\ensuremath{\alpha}=0.05$ and 8.4 times for $\ensuremath{\alpha}=0.01$ as compared to using only the coherent state. Similarly, the maximum quantum advantage for the estimation of optical gain is found around 2.95 times for the gain coefficient $G=1.05$ and around 6.35 times for $G=1.01$. We discuss the significance of using one measurement scheme over the other under different squeezing conditions. We compare our results with the Cram\'er-Rao bound for a two-mode bright squeezed state to assess the quality of the proposed methodologies.

DOI
10.1103/physreva.109.053715

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Absorption and gain processes are fundamental to any light-matter interaction and a precise measurement of these parameters is important for various scientific and technological applications. Quantum probes, specifically the squeezed states, have proved very successful, particularly in the applications that deal with phase shift and force measurements. In this paper, we focus on improving the sensitivity of the estimation of the photon-loss coefficient of a weakly absorbing medium as well as the estimation of the gain parameter using a two-mode bright squeezed state. The generation of this state combines the advantage of a coherent beam for its large photon number with the quantum properties of the two-mode squeezing operation in an optical parametric amplifier. We present two measurement schemes: balanced photodetection and time-reversed metrology, both utilizing two-mode bright squeezed light. The maximum quantum advantage we can achieve using two-mode bright squeezed light is 3.7 times for the absorption parameter \ensuremathα=0.05\ensuremath{\alpha}=0.05\ensuremathα=0.05 and 8.4 times for \ensuremathα=0.01\ensuremath{\alpha}=0.01\ensuremathα=0.01 as compared to using only the coherent state. Similarly, the maximum quantum advantage for the estimation of optical gain is found around 2.95 times for the gain coefficient G=1.05G=1.05G=1.05 and around 6.35 times for G=1.01G=1.01G=1.01. We discuss the significance of using one measurement scheme over the other under different squeezing conditions. We compare our results with the Cram'er-Rao bound for a two-mode bright squeezed state to assess the quality of the proposed methodologies.
Enhancing the precision of a measurement requires maximizing the information that can be gained about the quantity of interest from probing a system. For optical-based measurements, such an enhancement can be achieved through two approaches, increasing the number of photons used to interrogate the system and using quantum states of light to increase the amount of quantum Fisher information gained per photon. Here we consider the use of quantum states of light with a large number of photons, namely the bright single-mode squeezed state and the bright two-mode squeezed state, which take advantage of both of these approaches for the problem of transmission estimation. We show that, in the limit of large squeezing, these states approach the maximum possible quantum Fisher information per photon for transmission estimation that is achieved with the Fock state and the vacuum two-mode squeezed state. Since the bright states we consider can be generated at powers much higher than those of the quantum states that achieve the maximum quantum Fisher information per photon, they can achieve a much higher absolute precision as quantified by the quantum Cram\'er-Rao bound. We discuss the effects of losses external to the system on the precision of transmission estimation and identify simple measurement techniques that can saturate the quantum Cram\'er-Rao bound for the bright squeezed states even in the presence of such external losses.
Two-photon absorption (TPA) is of fundamental importance in super-resolution imaging and spectroscopy. Its nonlinear character allows for the prospect of using quantum resources, such as entanglement, to improve measurement precision or to gain new information on, e.g., ultrafast molecular dynamics. Here, we establish the metrological properties of nonclassical squeezed light sources for precision measurements of TPA cross sections. We find that the Cram\'er-Rao bound does not provide a fundamental limit for the precision achievable with squeezed states in the limit of very small cross sections. Considering the most relevant measurement strategies---namely, photon-counting and quadrature measurements---we determine the quantum advantage provided by squeezed states as compared to coherent states. We find that squeezed states outperform the precision achievable by coherent states when performing quadrature measurements, which provide improved scaling of the Fisher information with respect to the mean photon number $\ensuremath{\sim}{n}^{4}$. Due to the interplay of the incoherent nature and the nonlinearity of the TPA process, unusual scaling can also be obtained with coherent states, which feature an $\ensuremath{\sim}{n}^{3}$ scaling in both quadrature and photon-counting measurements.
Quantum estimation of parameters defining open-system dynamics may be enhanced by using ancillas that are entangled with the probe but are not submitted to the dynamics. Here we consider the important problem of estimation of transmission of light by a sample, with losses due to absorption and scattering. We show, through the determination of the quantum Fisher information, that the ancilla strategy leads to the best possible precision in single-mode estimation—the one obtained for a Fock-state input—through joint photon counting of probe and ancilla, which are modes of a bimodal squeezed state produced by an optical parametric amplifier. This proposal overcomes the challenge of producing and detecting high-photon-number Fock states, and it is quite robust in the presence of additional noise: We show that it is immune to phase noise and the precision does not change if the incoming state gets disentangled. Furthermore, the quantum gain is still present under moderate photon losses of the input beams. We also discuss an alternative to joint photon counting, which is readily implementable with present technology and approaches the quantum Fisher information result for weak absorption, even with moderate photon losses of the input beams before the sample is probed: a time-reversal procedure, placing the sample between two optical parametric amplifiers, with the second undoing the squeezing produced by the first one. The precision of estimation of the loss parameter is obtained from the average outgoing total photon number and its variance. In both procedures, the state of the probe and the detection procedure are independent of the value of the parameter. Published by the American Physical Society 2024
Recently, there has been significant interest in multiple-parameter quantum estimation techniques that exploit quantum resources. In particular, the estimation of optical transmission is a crucial parameter in various scientific fields and industries. In optical-based sensing, precision can be enhanced through two approaches: increasing the number of photons that interact with the samples and utilizing quantum states of light. In this paper, we investigate multiple transmission estimation using bright two-mode squeezed states (bTMSSs), which combine the advantages of both bright light and quantum states. We calculate the precision bound for multiple transmission estimation by employing multiple copies of bTMSSs with experimentally feasible optimal measurement, determining both the quantum Cramer-Rao bound and the Cramer-Rao bound. Our results demonstrate that multiple copies of bTMSSs can achieve quantum-enhanced sensitivity for multiple transmissions compared to coherent states, and the ultimate limit of precision can be attained in regions with high nonlinear gain. Furthermore, as an application, we show the quantum-enhanced sensing in circular dichroism sensing using a pair of bTMSSs. Our strategy for multiple transmission estimation offers a practical platform for exploring real-world quantum sensing applications.
Phase-insensitive amplifiers (PIAs), as a class of important quantum devices, have found significant applications in the subtle manipulation of multiple quantum correlation and multipartite quantum entanglement. Gain is a very important parameter for quantifying the performance of a PIA. Its absolute value can be defined as the ratio of the output light beam power to the input light beam power, while its estimation precision has not been extensively investigated yet. Therefore, in this work, we theoretically study the estimation precision from the vacuum two-mode squeezed state (TMSS), the estimation precision of the coherent state, and the bright TMSS scenario, which has the following two advantages: it has more probe photons than the vacuum TMSS and higher estimation precision than the coherent state. The advantage in terms of estimation precision of the bright TMSS compared with the coherent state is researched. We first simulate the effect of noise from another PIA with gain M on the estimation precision of the bright TMSS, and we find that a scheme in which the PIA is placed in the auxiliary light beam path is more robust than two other schemes. Then, a fictitious beam splitter with transmission T is used to simulate the noise effects of propagation loss and imperfect detection, and the results show that a scheme in which the fictitious beam splitter is placed before the original PIA in the probe light beam path is the most robust. Finally, optimal intensity difference measurement is confirmed to be an accessible experimental technique to saturate estimation precision of the bright TMSS. Therefore, our present study opens a new avenue for quantum metrology based on PIAs.