Enhancing the precision of a measurement requires maximizing the information that can be gained about the quantity of interest from probing a system. For optical-based measurements, such an enhancement can be achieved through two approaches, increasing the number of photons used to interrogate the system and using quantum states of light to increase the amount of quantum Fisher information gained per photon. Here we consider the use of quantum states of light with a large number of photons, namely the bright single-mode squeezed state and the bright two-mode squeezed state, which take advantage of both of these approaches for the problem of transmission estimation. We show that, in the limit of large squeezing, these states approach the maximum possible quantum Fisher information per photon for transmission estimation that is achieved with the Fock state and the vacuum two-mode squeezed state. Since the bright states we consider can be generated at powers much higher than those of the quantum states that achieve the maximum quantum Fisher information per photon, they can achieve a much higher absolute precision as quantified by the quantum Cram\'er-Rao bound. We discuss the effects of losses external to the system on the precision of transmission estimation and identify simple measurement techniques that can saturate the quantum Cram\'er-Rao bound for the bright squeezed states even in the presence of such external losses.
Enhancing the precision of a measurement requires maximizing the information that can be gained about the quantity of interest from probing a system. For optical-based measurements, such an enhancement can be achieved through two approaches, increasing the number of photons used to interrogate the system and using quantum states of light to increase the amount of quantum Fisher information gained per photon. Here we consider the use of quantum states of light with a large number of photons, namely the bright single-mode squeezed state and the bright two-mode squeezed state, which take advantage of both of these approaches for the problem of transmission estimation. We show that, in the limit of large squeezing, these states approach the maximum possible quantum Fisher information per photon for transmission estimation that is achieved with the Fock state and the vacuum two-mode squeezed state. Since the bright states we consider can be generated at powers much higher than those of the quantum states that achieve the maximum quantum Fisher information per photon, they can achieve a much higher absolute precision as quantified by the quantum Cram'er-Rao bound. We discuss the effects of losses external to the system on the precision of transmission estimation and identify simple measurement techniques that can saturate the quantum Cram'er-Rao bound for the bright squeezed states even in the presence of such external losses.
The minimum possible uncertainty when estimating a parameter, in this case transmission, is bounded by the quantum Cramér-Rao bound (QCRB). This bound is independent of the measurement technique and as result can be used to quantify how close a measurement is to the optimal one for a given system and probing state, as an optimal measurement saturates the QCRB. The ability to perform transmission measurements through an optical system at the QCRB can lead to enhancements in the calibration of optimal states for interferometers, the characterization of high efficiency photodetectors, or the sensitivity of sensing devices based on transmission, such as plasmonic sensors or spectroscopy. We show theoretically that the ultimate sensitivity limit per photon in the estimation of transmission, achievable with Fock states or vacuum two-mode squeezed states (vTMSS), can be approached through the use of bright quantum states of light, such as bright single-mode squeezed states (bSMSS) or bright two-mode squeezed states (bTMSS). The use of bright quantum states has the advantage that they can be generated with a significantly larger number of photons, which leads to an absolute sensitivity that can be many orders of magnitude larger than the one achieved with Fock states or vTMSS. We identify a measurement strategy that saturates the QCRB for these bright quantum states and shown experimentally that transmission estimation at the QCRB can be achieved with bTMSS through optimized intensity difference measurements.
The field of quantum metrology seeks to apply quantum techniques and/or resources to classical sensing approaches with the goal of enhancing the precision in the estimation of a parameter beyond what can be achieved with classical resources. Theoretically, the fundamental minimum uncertainty in the estimation of a parameter for a given probing state is bounded by the quantum Cramér-Rao bound. From a practical perspective, it is necessary to find physical measurements that can saturate this fundamental limit and to show experimentally that it is possible to perform measurements with the required precision to do so. Here we perform experiments that saturate the quantum Cramér-Rao bound for transmission estimation over a wide range of transmissions when probing the system under study with a continuous wave bright two-mode squeezed state. To properly take into account the imperfections in the generation of the quantum state, we extend our previous theoretical results to incorporate the measured properties of the generated quantum state. For our largest transmission level of 84%, we show a 62% reduction over the optimal classical protocol in the variance in transmission estimation when probing with a bright two-mode squeezed state with -8 dB of intensity-difference squeezing. Given that transmission estimation is an integral part of many sensing protocols, such as plasmonic sensing, spectroscopy, calibration of the quantum efficiency of detectors, etc., the results presented promise to have a significant impact on a number of applications in various fields of research.
Recently, there has been significant interest in multiple-parameter quantum estimation techniques that exploit quantum resources. In particular, the estimation of optical transmission is a crucial parameter in various scientific fields and industries. In optical-based sensing, precision can be enhanced through two approaches: increasing the number of photons that interact with the samples and utilizing quantum states of light. In this paper, we investigate multiple transmission estimation using bright two-mode squeezed states (bTMSSs), which combine the advantages of both bright light and quantum states. We calculate the precision bound for multiple transmission estimation by employing multiple copies of bTMSSs with experimentally feasible optimal measurement, determining both the quantum Cramer-Rao bound and the Cramer-Rao bound. Our results demonstrate that multiple copies of bTMSSs can achieve quantum-enhanced sensitivity for multiple transmissions compared to coherent states, and the ultimate limit of precision can be attained in regions with high nonlinear gain. Furthermore, as an application, we show the quantum-enhanced sensing in circular dichroism sensing using a pair of bTMSSs. Our strategy for multiple transmission estimation offers a practical platform for exploring real-world quantum sensing applications.
Absorption and gain processes are fundamental to any light-matter interaction and a precise measurement of these parameters is important for various scientific and technological applications. Quantum probes, specifically the squeezed states, have proved very successful, particularly in the applications that deal with phase shift and force measurements. In this paper, we focus on improving the sensitivity of the estimation of the photon-loss coefficient of a weakly absorbing medium as well as the estimation of the gain parameter using a two-mode bright squeezed state. The generation of this state combines the advantage of a coherent beam for its large photon number with the quantum properties of the two-mode squeezing operation in an optical parametric amplifier. We present two measurement schemes: balanced photodetection and time-reversed metrology, both utilizing two-mode bright squeezed light. The maximum quantum advantage we can achieve using two-mode bright squeezed light is 3.7 times for the absorption parameter $\ensuremath{\alpha}=0.05$ and 8.4 times for $\ensuremath{\alpha}=0.01$ as compared to using only the coherent state. Similarly, the maximum quantum advantage for the estimation of optical gain is found around 2.95 times for the gain coefficient G=1.05 and around 6.35 times for G=1.01. We discuss the significance of using one measurement scheme over the other under different squeezing conditions. We compare our results with the Cram\'er-Rao bound for a two-mode bright squeezed state to assess the quality of the proposed methodologies.
Abstract Estimating transmission or loss is at the heart of spectroscopy. To achieve the ultimate quantum resolution limit, one must use probe states with definite photon number and detectors capable of distinguishing the number of photons impinging thereon. In practice, one can outperform classical limits using two-mode squeezed light, which can be used to herald definite-photon-number probes, but the heralding is not guaranteed to produce the desired probes when there is loss in the heralding arm or its detector is imperfect. We show that this paradigm can be used to simultaneously measure distinct loss parameters in both modes of the squeezed light, with attainable quantum advantages. We demonstrate this protocol on Xanadu’s X8 chip, accessed via the cloud, building photon-number probability distributions from 106 shots and performing maximum likelihood estimation (MLE) on these distributions 103 independent times. Because pump light may be lost before the squeezing occurs, we also simultaneously estimate the actual input power, using the theory of nuisance parameters. MLE converges to estimate the transmission amplitudes in X8’s eight modes to be 0.392 02(6), 0.307 06(8), 0.369 37(6), 0.287 30(9), 0.382 06(6), 0.304 41(8), 0.372 29(6), and 0.286 21(8) and the squeezing parameters, which are proxies for effective input coherent-state amplitudes, their losses, and their nonlinear interaction times, to be 1.3000(2), 1.3238(3), 1.2666(2), and 1.3425(3); all of these uncertainties are within a factor of two of the quantum Cramér–Rao bound. This study provides crucial insight into the intersection of quantum multiparameter estimation theory, MLE convergence, and the characterization and performance of real quantum devices.