Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2403.13071 · ACS Photonics

Strong Coupling and Single-Photon Nonlinearity in Free-Electron Quantum Optics

Aviv Karnieli, Charles Roques‐Carmes, Nicholas Rivera, Shanhui Fan

Published Jul 29, 2024• 25 citations
arXivHTMLPDF

Abstract

A central challenge in the emerging field of free-electron quantum optics is to achieve strong quantum interaction and single-photon nonlinearity between a flying free electron and a photonic mode. Existing schemes are intrinsically limited by electron diffraction, which puts an upper bound on the interaction length and, therefore, on the strength of quantum coupling and nonlinearity. Here, we propose “free-electron fibers”: effectively one-dimensional photonic systems where free electrons copropagate with two guided modes. The first mode applies a ponderomotive trap to the free electron, removing the limitations due to electron diffraction. The second mode strongly couples to the guided free electron with an enhanced coupling that is orders of magnitude larger than previous designs. The extended interaction lengths enabled by our scheme allow for strong single-photon nonlinearities mediated by free electrons. We predict novel quantum effects in our system such as deterministic single-photon emission and nonlinear multimode dynamics. Our proposal paves the way toward the realization of heralded macroscopic nonclassical light generation, deterministic single-photon sources, and quantum gates controlled by free-electron–photon interactions.

DOI
10.1021/acsphotonics.4c00908

Related papers

Free-electron ponderomotive guiding for strong coupling and single-photon nonlinearity

Aviv Karnieli, Nicholas Rivera, Charles Roques‐Carmes +1 more

We show how ponderomotive guiding of free electrons inside hollow optical fibers enables strong electron-photon coupling, together with exceptionally high single photon nonlinearities.

•Jan 1, 2024•0 citations

Upper limit to quantum interaction strength between free electrons and electromagnetic single modes

Zetao Xie, Zeling Chen, Hao Li +6 more

Free–electron quantum optics facilitates electron-photon entanglement for quantum information processing. The challenge is finding specialized photonic-structures optimizing electron-photon interactions. We present a first-principle upper limit on the interaction strength, guiding the design of future structures.

•Jan 1, 2024•0 citations

Quantum optics with free electrons: from quantum sensing to strong coupling and single-photon nonlinearity

Aviv Karnieli, Charles Roques‐Carmes, Renwen Yu +1 more

Free electrons are an emerging new type of quantum probe, with high quantum coherence, sub fsec – sub-nm resolution, high tunability and pristine coherent control. Recent experimental and theoretical advancements showcased the quantum nature of the interaction between a free electron and light and bound-electron qubits, with demonstrations of strong electron-photon coupling and coincidence, and proposals for quantum light generation.

Optical and Quantum Sensing and Precision Metrology II•Mar 19, 2025•0 citations

Quantum sensing and metrology with free electrons

Cruz I. Velasco, F. Javier Garcı́a de Abajo

The quantum properties of matter and radiation can be leveraged to surpass classical limits of sensing and detection. Quantum optics does so by creating and measuring nonclassical light. However, better performance requires higher photon-number states, which are challenging to generate and detect. Here, we combine photons and free electrons to solve the problem of generating and detecting high-number states well beyond those reachable with light alone and further show that an unprecedented level of sensitivity and resolution is gained based on the measurement of free-electron currents after suitably designed electron-light interactions. Our enabling ingredient is the strong electron-light coupling produced by aloof electron reflection on an optical waveguide, leading to the emission or absorption of a high number of guided photons by every single electron. We establish through rigorous theory that, by combining electron-beam splitters with two electron-waveguide interactions, the sensitivity to detect optical-phase changes can be enhanced dramatically using currently attainable technology. These results inaugurate a disruptive quantum technology relying on free electrons and their strong interaction with waveguided light.

arXiv:2505.06124•Nature Communications•Dec 23, 2025•2 citations

Temporal trapping: a route to strong coupling and deterministic optical quantum computation

Ryotatsu Yanagimoto, Edwin Ng, Marc Jankowski +2 more

The realization of deterministic photon–photon gates is a central goal in optical quantum computation and engineering. A longstanding challenge is that optical nonlinearities in scalable, room-temperature material platforms are too weak to achieve the required strong coupling, due to the critical loss-confinement trade-off in existing photonic structures. In this work, we introduce a spatio-temporal confinement method, dispersion-engineered temporal trapping, to circumvent the trade-off, enabling a route to all-optical strong coupling. Temporal confinement is imposed by an auxiliary trap pulse via cross-phase modulation, which, combined with the spatial confinement of a waveguide, creates a “flying cavity” that enhances the nonlinear interaction strength by at least an order of magnitude. Numerical simulations confirm that temporal trapping confines the multimode nonlinear dynamics to a single-mode subspace, enabling high-fidelity deterministic quantum gate operations. With realistic dispersion engineering and loss figures, we show that temporally trapped ultrashort pulses could achieve strong coupling on near-term nonlinear nanophotonic platforms. Our results highlight the potential of ultrafast nonlinear optics to become the first scalable, high-bandwidth, and room-temperature platform that achieves strong coupling, opening a path to quantum computing, simulation, and light sources.

arXiv:2203.11909•Optica•Oct 18, 2022•33 citations

Electron-Photon Quantum State Heralding Using Photonic Integrated Circuits

Guanhao Huang, Nils J. Engelsen, Ofer Kfir +2 more

Recently, integrated photonic circuits have brought new capabilities to electron microscopy and been used to demonstrate efficient electron phase modulation and electron-photon correlations.Here, we quantitatively analyze the feasibility of high-fidelity and high-purity quantum state heralding using a free electron and a photonic integrated circuit with parametric coupling, and propose schemes to shape useful electron and photonic states in different application scenarios.Adopting a dissipative quantum electrodynamics treatment, we formulate a framework for the coupling of free electrons to waveguide spatial-temporal modes.To avoid multimode-coupling-induced state decoherence, we show that with proper waveguide design, the interaction can be reduced to a single-mode coupling to a quasi-TM 00 mode.In the single-mode coupling limit, we go beyond the conventional state ladder treatment, and show that the electron-photon energy correlations within the ladder subspace can still lead to a fundamental purity and fidelity limit on complex optical and electron state preparations through heralding schemes.We propose applications that use this underlying correlation to their advantage, but also show that the imposed limitations for general applications can be overcome by using photonic integrated circuits with an experimentally feasible interaction length, showing its promise as a platform for free-electron quantum optics.

arXiv:2206.08098•PRX Quantum•Jun 26, 2023•33 citations
A central challenge in the emerging field of free-electron quantum optics is to achieve strong quantum interaction and single-photon nonlinearity between a flying free electron and a photonic mode. Existing schemes are intrinsically limited by electron diffraction, which puts an upper bound on the interaction length and, therefore, on the strength of quantum coupling and nonlinearity. Here, we propose “free-electron fibers”: effectively one-dimensional photonic systems where free electrons copropagate with two guided modes. The first mode applies a ponderomotive trap to the free electron, removing the limitations due to electron diffraction. The second mode strongly couples to the guided free electron with an enhanced coupling that is orders of magnitude larger than previous designs. The extended interaction lengths enabled by our scheme allow for strong single-photon nonlinearities mediated by free electrons. We predict novel quantum effects in our system such as deterministic single-photon emission and nonlinear multimode dynamics. Our proposal paves the way toward the realization of heralded macroscopic nonclassical light generation, deterministic single-photon sources, and quantum gates controlled by free-electron–photon interactions.
The quantum properties of matter and radiation can be leveraged to surpass classical limits of sensing and detection. Quantum optics does so by creating and measuring nonclassical light. However, better performance requires higher photon-number states, which are challenging to generate and detect. Here, we combine photons and free electrons to solve the problem of generating and detecting high-number states well beyond those reachable with light alone and further show that an unprecedented level of sensitivity and resolution is gained based on the measurement of free-electron currents after suitably designed electron-light interactions. Our enabling ingredient is the strong electron-light coupling produced by aloof electron reflection on an optical waveguide, leading to the emission or absorption of a high number of guided photons by every single electron. We establish through rigorous theory that, by combining electron-beam splitters with two electron-waveguide interactions, the sensitivity to detect optical-phase changes can be enhanced dramatically using currently attainable technology. These results inaugurate a disruptive quantum technology relying on free electrons and their strong interaction with waveguided light.
The realization of deterministic photon–photon gates is a central goal in optical quantum computation and engineering. A longstanding challenge is that optical nonlinearities in scalable, room-temperature material platforms are too weak to achieve the required strong coupling, due to the critical loss-confinement trade-off in existing photonic structures. In this work, we introduce a spatio-temporal confinement method, dispersion-engineered temporal trapping, to circumvent the trade-off, enabling a route to all-optical strong coupling. Temporal confinement is imposed by an auxiliary trap pulse via cross-phase modulation, which, combined with the spatial confinement of a waveguide, creates a “flying cavity” that enhances the nonlinear interaction strength by at least an order of magnitude. Numerical simulations confirm that temporal trapping confines the multimode nonlinear dynamics to a single-mode subspace, enabling high-fidelity deterministic quantum gate operations. With realistic dispersion engineering and loss figures, we show that temporally trapped ultrashort pulses could achieve strong coupling on near-term nonlinear nanophotonic platforms. Our results highlight the potential of ultrafast nonlinear optics to become the first scalable, high-bandwidth, and room-temperature platform that achieves strong coupling, opening a path to quantum computing, simulation, and light sources.
Recently, integrated photonic circuits have brought new capabilities to electron microscopy and been used to demonstrate efficient electron phase modulation and electron-photon correlations.Here, we quantitatively analyze the feasibility of high-fidelity and high-purity quantum state heralding using a free electron and a photonic integrated circuit with parametric coupling, and propose schemes to shape useful electron and photonic states in different application scenarios.Adopting a dissipative quantum electrodynamics treatment, we formulate a framework for the coupling of free electrons to waveguide spatial-temporal modes.To avoid multimode-coupling-induced state decoherence, we show that with proper waveguide design, the interaction can be reduced to a single-mode coupling to a quasi-TM 00 mode.In the single-mode coupling limit, we go beyond the conventional state ladder treatment, and show that the electron-photon energy correlations within the ladder subspace can still lead to a fundamental purity and fidelity limit on complex optical and electron state preparations through heralding schemes.We propose applications that use this underlying correlation to their advantage, but also show that the imposed limitations for general applications can be overcome by using photonic integrated circuits with an experimentally feasible interaction length, showing its promise as a platform for free-electron quantum optics.