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arXiv:2402.15556 · Physical Review Letters

Controlling Markovianity with Chiral Giant Atoms

Federico Roccati, Dario Cilluffo

Published Aug 9, 2024• 41 citations
arXivHTMLPDF

Abstract

Giant artificial atoms are promising and flexible building blocks for the implementation of analog quantum simulators. They are realized via a multilocal pattern of couplings of two-level systems to a waveguide, or to a two-dimensional photonic bath. A hallmark of giant-atom physics is their non-Markovian character in the form of self-coherent feedback, leading, e.g., to nonexponential atomic decay. The timescale of their non-Markovianity is essentially given by the time delay proportional to the distance between the various coupling points. In parallel, with the state-of-the-art experimental setups, it is possible to engineer complex phases in the atom-light couplings. Such phases simulate an artificial magnetic field, yielding a chiral behavior of the atom-light system. Here, we report a surprising connection between these two seemingly unrelated features of giant atoms, showing that the chirality of a giant atom controls its Markovianity. In particular, by adjusting the couplings' phases, a giant atom can, counterintuitively, enter an exact Markovian regime, irrespectively of any inherent time delay. We illustrate this mechanism as an interference process and via a collision model picture. Our findings significantly advance the understanding of giant atom physics, and open new avenues for the control of quantum nanophotonic networks.

DOI
10.1103/physrevlett.133.063603

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Giant artificial atoms are promising and flexible building blocks for the implementation of analog quantum simulators. They are realized via a multilocal pattern of couplings of two-level systems to a waveguide, or to a two-dimensional photonic bath. A hallmark of giant-atom physics is their non-Markovian character in the form of self-coherent feedback, leading, e.g., to nonexponential atomic decay. The timescale of their non-Markovianity is essentially given by the time delay proportional to the distance between the various coupling points. In parallel, with the state-of-the-art experimental setups, it is possible to engineer complex phases in the atom-light couplings. Such phases simulate an artificial magnetic field, yielding a chiral behavior of the atom-light system. Here, we report a surprising connection between these two seemingly unrelated features of giant atoms, showing that the chirality of a giant atom controls its Markovianity. In particular, by adjusting the couplings' phases, a giant atom can, counterintuitively, enter an exact Markovian regime, irrespectively of any inherent time delay. We illustrate this mechanism as an interference process and via a collision model picture. Our findings significantly advance the understanding of giant atom physics, and open new avenues for the control of quantum nanophotonic networks.
We study the generation of quantum entanglement between two giant atoms coupled to a common one-dimensional waveguide. Here each giant atom interacts with the waveguide at two separate coupling points. Within the Wigner-Weisskopf framework for single coupling points, we obtain the time-delayed quantum master equations governing the evolution of the two giant atoms for three different coupling configurations: separated, braided, and nested couplings. For each coupling configuration, we consider both the Markovian and non-Markovian entanglement dynamics of the giant atoms, which are initially in two different separable states: single- and double-excitation states. Our results show that the generated entanglement depends on the phase shift, time delay, atomic initial state, and the coupling configuration. For the single-excitation initial state, there exists the steady-state entanglement for each coupling in both the Markovian and non-Markovian regimes due to the appearance of the dark state. For the double-excitation initial state, we observe entanglement sudden birth via adjusting the phase shift in both regimes. In particular, the maximally achievable entanglement for the nested coupling is about one order of magnitude larger than those of separate and braided couplings. We also find that the maximal entanglement for these three coupling configurations can be enhanced in the case of small time delays. This work can be utilized for the generation and control of entanglement in quantum networks based on giant-atom waveguide-QED systems, which have wide potential applications in quantum information processing.
In this paper we investigate the non-Markovian dynamics of a giant atom coupled to a one-dimensional photonic lattice with synthetic gauge fields. By engineering a complex-valued hopping amplitude, we break reciprocity and explore how chiral propagation and phase-induced interference affect spontaneous emission, bound-state formation, and atom–field entanglement. The giant atom interacts with the lattice at multiple, spatially separated sites, leading to rich interference effects and decoherence-free subspaces. We derive an exact expression for the self-energy and perform real-time Schrödinger simulations in the single-excitation subspace, for the atomic population, von Neumann entropy, field localization, and asymmetry in emission. Our results show that the hopping phase ϕ governs not only the directionality of emitted photons but also the degree of atom–bath entanglement and photon localization. Remarkably, we observe robust bound states inside the photonic band and directional asymmetry, due to interference from spatially separated coupling points. These findings provide a basis for engineering non-reciprocal, robust, and entangled light–matter interactions in structured photonic systems.
We investigate single-photon scattering in a waveguide-QED setup, where a giant molecule composed of two frequency-detuned giant atoms is coupled to two parallel waveguides via multiple connection points. The competition between coherent atom--atom coupling and the effective decay rates dictates the splitting of a single resonance into a doublet in the transmission (reflection) spectra. By tailoring the asymmetry of the decay rates and the atomic detuning, one can engineer photon-path interference to optimize the transfer between waveguides; under chiral coupling conditions, this interference can be further harnessed to realize fully deterministic routing. In the non-Markovian regime, retardation effects can reshape the spectra and actively drive transitions between the weak- and strong-coupling regimes, converting an unsplit Markovian resonance into a clearly separated doublet, or conversely merging a split doublet back into a single resonance. For sufficiently long time delays, it further generates multiple resonances and avoided crossings, enriching the spectral response. Our results demonstrate how atomic detuning, decay-rate asymmetry, and non-Markovian retardation cooperate to provide versatile, interference-based control over single-photon routing in multi-port quantum networks.
Dynamics of quantum coherence and non-Markovianity of a three-level giant atom coupling to a one-dimensional waveguide and a classical field are investigated theoretically. The time delay of the photo propagation in the waveguide is taken into account and our aim is to access the collective impact of a waveguide and classical control of the system on the time evolution of coherence and non-Markovianity. For a giant atom, we find that the various values of the accumulated phase and time delay does not make much difference for the coherence evolution but there exists non-Markovian behavior for the vast majority of the chosen parameter values. With regard to the initial relative phase, the quantum coherence takes a monotonic behavior for a small atom but decreases with oscillations for a giant atom with majority values of the initial relative phase. Quantum coherence of a small atom decreases monotonically with regardless of the Rabi frequency and the atom’s detuning to a large extent but a large Rabi frequency or a large atom’s detuning will induce non-Markovian behavior for a giant atom. With a comparative analysis, the coherence evolution is enhanced significantly in that there is non-Markovian behavior for the dynamics of quantum coherence in a much larger range of scaled time for a giant atom than that for a small atom. Our study provide clues to preserve and to enhance quantum coherence in qutrit systems.
Chiral interactions enable directional control of quantum light, providing new routes for nonreciprocal photon dynamics. While previous studies focused on single photon regimes, this work explores the non-Markovian multiphoton regime in a giant nonlinear system nonlocally coupled to a one-dimensional waveguide, with a tunable phase difference breaking parity symmetry. We show that single-photon transport remains reciprocal, but multiphoton dynamics become chiral, generating direction-dependent higher-order correlations and enabling deterministic creation of multiphoton states with nontrivial statistics from a single input direction, even under strong dissipation. The non-Markovian nature allows tuning of transmitted photon statistics via the coupling-point separation. At a specific phase, internal dynamics become Markovian while output photons retain non-Markovian features. Under strong coherent driving, we uncover nonreciprocal dissipative phase transitions and demonstrate how non-Markovianity shapes the critical response. This framework offers a general strategy for controlling chiral multiphoton dynamics in nonlocally coupled waveguide QED systems. Chiral light-matter interactions offer directional control of quantum states. This work demonstrates that a giant quantum emitter with tunable nonlocal coupling to a waveguide enables direction-dependent multiphoton correlations and dissipative phase transitions, providing a route to engineer non-Markovian chiral dynamics.
We explore the collective Zeno dynamics of giant artificial atoms that are coupled, via multiple coupling points, to a common photonic or acoustic reservoir. In this regime, the establishment of atomic cooperativity and the revivification of exponential decay are highly intertwined, which is utterly beyond the non-Markovian regime with only retarded backaction. We reveal that giant atoms build up their collective emission smoothly from the decay rate of zero to that predicted by Markovian approximation and show great disparity between different waveguide QED setups. As a comparison, the steplike growth of instantaneous decay rates in the retardation-only picture has also been shown. All of these theoretical pictures predict the same collective behavior in the long time limit. From a phenomenological standpoint, we observe that the atomic superradiance exhibits significant directional property. In addition, the subradiant photons feature prolonged oscillation in the early stage of collective radiance, where the energy is exchanged remarkably between giant emitters and the field. Our results might be probed in state-of-art waveguide QED experiments and fundamentally broaden the fields of collective emission in systems with giant atoms. Published by the American Physical Society 2024