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arXiv:2402.10330 · Physical review. B./Physical review. B

Quantum dynamics of semiconductor quantum dot Josephson junctions

Utkan Güngördü, Rusko Ruskov, Silas Hoffman, Kyle Serniak, Andrew J. Kerman, Charles Tahan

Published Jun 2, 2025• 2 citations
arXivHTMLPDF

Abstract

Josephson junctions constructed from superconductor-semiconductor-superconductor heterostructures have been used to realize a variety of voltage-tunable superconducting quantum devices, including qubits and parametric amplifiers. To date, theoretical descriptions of these systems have been restricted to small quantum fluctuations of the junction phase, making them inapplicable to many experiments. In this paper, we relax this, employing a path-integral formulation where the phase quantum dynamics is obtained self-consistently from an underlying many-body formalism. Our method recovers previously known results for small phase fluctuations, and predicts effects outside of that limit: (i) system capacitances undergo a gate-voltage-dependent renormalization; and (ii) an additional charge offset appears for asymmetric junctions. Our main results can be summarized in terms of a single-particle Hamiltonian, which can be directly compared to that of an ordinary Josephson junction. This more general theory could be a first step towards designing new quantum devices that go qualitatively beyond voltage-tunable variants of previously known circuits.

DOI
10.1103/physrevb.111.214503

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Josephson junctions constructed from superconductor-semiconductor-superconductor heterostructures have been used to realize a variety of voltage-tunable superconducting quantum devices, including qubits and parametric amplifiers. To date, theoretical descriptions of these systems have been restricted to small quantum fluctuations of the junction phase, making them inapplicable to many experiments. In this paper, we relax this, employing a path-integral formulation where the phase quantum dynamics is obtained self-consistently from an underlying many-body formalism. Our method recovers previously known results for small phase fluctuations, and predicts effects outside of that limit: (i) system capacitances undergo a gate-voltage-dependent renormalization; and (ii) an additional charge offset appears for asymmetric junctions. Our main results can be summarized in terms of a single-particle Hamiltonian, which can be directly compared to that of an ordinary Josephson junction. This more general theory could be a first step towards designing new quantum devices that go qualitatively beyond voltage-tunable variants of previously known circuits.
Gatemon qubits are based on a superconductor-quantum dot-superconductor (S-QD-S) junction which enables in situ electrostatic tuning via a gate electrode. For a single-channel QD this structure gives rise to two subgap Andreev bound states (ABSs), and generally leads to a richer quantum phase dynamics as compared to conventional transmons. In a recent work [Phys. Rev. B 111, 214503 (2025)] we derived the quantum phase dynamics from a many-body treatment which leads to an effective gate voltage-dependent Hamiltonian that self-consistently incorporates the phase quantization. It predicts (i) a renormalization of the junction's effective capacitance and (ii) the presence of gate voltage and occupation-dependent charge offsets in junctions with tunneling asymmetry. Here, we quantify the observable impact of these effects on the qubit's energy spectrum and anharmonicity, by studying the interplay of the two Andreev branches as a function of dot-gate voltages and junction transparencies. We show the relation of these predictions to simplified gatemon models and propose a protocol to experimentally detect the predicted charge offsets.
Properties of weak links between two superconductors, or Josephson junctions, make them interesting for fundamental physics research. Since their discovery over four decades ago, they have provided a unique way to study the behavior of the superconducting quantum phase. More recently, ultra small, or mesoscopic, Josephson junctions with substantial single Cooper pair charging energy have gained interest due to their behavior as macroscopic quantum objects. In addition to the theoretical interest, Josephson junctions can be used as active elements in circuit applications. Particularly, in this Thesis we study two different devices. We develop the required theoretical treatments, derive device properties, and compare the results with experimental data. The first application is a Josephson voltage standard based on externally damped Superconductor - Insulator - Superconductor junctions. It consists of an array of large Josephson junctions connected in series and irradiated with a 70 GHz microwave signal. Phase locking the Josephson dynamics into the signal leads to the quantization of the voltage. This is utilized in metrology. We introduce a new circuit solution based on frequency dependent damping of the junctions. Optimization and some designs for practical arrays are presented. The purpose is to find such a design that the array is fast, has low power consumption and is as stable as possible. Arrays able to generate DC voltages of order 1 volt with metrological accuracy are demonstrated experimentally and their applicability in AC voltage calibrations is analyzed. The second application is the Bloch Oscillating Transistor (BOT). The BOT is based on controlling the Cooper pair current in an ultra small Josephson junction by means of quasiparticles tunneling through a normal junction. As part of the thesis work, the principle of operation is first demonstrated computationally. The model is then refined to yield quantitative predictions of the characteristics. Finally, an analytic theory for the device is developed and the properties as an amplifier are derived.
Quantum fluctuations of the charge at a current-biased Josephson junction and of the Josephson current couple to the quasiparticle tunneling when the system is at equilibrium in the zero-voltage state. The effect of reducing the capacitance of the junction is studied by means of a model Hamiltonian. When this becomes smaller, charge fluctuations are reduced, but the effective dissipation is also lowered so that the junction displays an underdamped behavior. The Josephson branch is shifted at the voltage e/2C because of charging due to the quasiparticles. A path-integral formulation of the model leads to a high dynamical subgap resistance at I\ensuremath{\rightarrow}0, as recently found experimentally.
The theory of superconducting phase qubits---also known as current-biased Josephson junctions---is presented. In the first part of this thesis, I introduce quantum computation, quantum simulation, and their deep connection with symplectic integration. I then consider the fundamental many-body theory of superconductivity and Josephson junctions and show how the quantum dynamics of a single macroscopic degree of freedom, the gauge invariant phase difference, emerges. A complete study of the Hilbert space structure of such a variable is performed for the current-biased junction. The resulting resonance structure is studied in detail, using various formalisms including the WKB approximation, instanton methods, the complex scaling transformation, basis set stabilization, numerical integration, and dynamical simulation using Lie algebraic wave-packet propagation. The second part of this thesis explores how the current-biased junction can be used as an element of a quantum computer---a quantum bit (qubit). Single qubit operations are studied, followed by the presentation of the theory of coupled qubit devices. My key result is the design and optimization of quantum logic gates with high fidelity (F ~ 0.9999) for capacitively coupled phase qubits with short gate times (~ 10 ns). Finally, I examine an advanced qubit-coupling scheme, a resonant coupling method utilizing a harmonic oscillator as the auxiliary degree of freedom. The models and methods presented here have been developed in direct collaboration with an experimental program. These experiments are the first to show spectroscopic evidence for entanglement between two and three macroscopic degrees of freedom in a superconducting circuit.
The quantized Josephson junction equation that underpins the behaviour of charge qubits and other tunnel devices is usually derived through canonical quantization of the classical macroscopic Josephson relations. However, this approach may neglect effects due to the fact that the charge qubit consists of a superconducting island of finite size connected to a large superconductor. We show that the well-known quantized Josephson equation can be derived directly and simply from a microscopic many-body Hamiltonian. By choosing the appropriate strong-coupling limit we produce a highly simplified Hamiltonian that nevertheless allows us to go beyond the mean-field limit and predict further finite-size terms in addition to the basic equation.
We realize a hybrid superconductor-semiconductor transmon device in which the Josephson effect is controlled by a gate-defined quantum dot in an InAs-Al nanowire.Microwave spectroscopy of the transition spectrum of the transmon allows us to probe the ground-state parity of the quantum dot as a function of the gate voltages, the external magnetic flux, and the magnetic field applied parallel to the nanowire.The measured parity phase diagram is in agreement with that predicted by a single-impurity Anderson model with superconducting leads.Through continuous-time monitoring of the circuit, we furthermore resolve the quasiparticle dynamics of the quantum dot Josephson junction across the phase boundaries.Our results can facilitate the realization of semiconductor-based 0-π qubits and Andreev qubits.