Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2402.08537 · Nature Physics

Self-induced superradiant masing

Wenzel Kersten, Nikolaus de Zordo, Oliver Diekmann, Elena S. Redchenko, Andrew N. Kanagin, Andreas Angerer, William J. Munro, Kae Nemoto, I. E. Mazets, Stefan Rotter, Thomas Pohl, Jörg Schmiedmayer

Published Jan 1, 2026• 6 citations
arXivHTMLPDF

Abstract

In cavity quantum electrodynamics and particularly superradiance, emitters are typically assumed to be independent, interacting only through light shared via a common mode. Although such photon-mediated interactions lead to a wide range of collective optical effects, direct dipole-dipole interactions within the emitter ensemble are generally viewed as a source of decoherence. Here we report the role of direct spin-spin interactions as a drive for the superradiant dynamics of a hybrid system of nitrogen-vacancy centre spins in a diamond coupled to a superconducting microwave cavity. After an initial fast superradiant burst, we observe a train of subsequent emission pulses followed by quasi-continuous masing for up to one millisecond. We show that this behaviour arises from spectral hole refilling, where spin inversion is redistributed into the superradiant window of spins resonant with the cavity. We report measurements that exclude other cavity-related effects and perform microscopic simulations that confirm that the observed behaviour is driven by dipole-dipole interactions between the spins. These findings open pathways for exploring complex spin-spin interactions in dense disordered systems and offer possibilities for ultranarrow-linewidth solid-state superradiant masers powered purely by microwave-driven spin control.

DOI
10.1038/s41567-025-03123-0

Related papers

Self-induced Superradiant Masing

Kersten, W., De Zordo, N., Diekmann, O. +9 more

In cavity quantum electrodynamics (cQED) and particularly superradiance, emitters are typically assumed to be independent, interacting only through light shared via a common mode. While such photon-mediated interactions lead to a rich spectrum of collective optical effects, direct dipole-dipole interactions within the emitter ensemble are generally viewed as a source of decoherence. Here, we uncover a new role for direct spin-spin interactions as a drive for the superradiant dynamics of a hybrid system of nitrogen-vacancy center spins in diamond coupled to a superconducting microwave cavity. After an initial fast superradiant burst, we observe an unexpected train of subsequent emission pulses followed by quasi-continuous masing for up to one millisecond. We show that this surprising behavior arises from spectral hole refilling, where spin inversion is redistributed into the superradiant window of spins resonant with the cavity. We report measurements that clearly exclude other cQED-related effects, and performed microscopic simulations of up to one million spins, which demonstrate that the observed self-induced masing is indeed driven by dipole-dipole interactions between the spins. These findings open new pathways for exploring complex spin-spin interactions in dense disordered systems and offer possibilities for ultra-narrow linewidth solid-state superradiant masers powered purely by microwave-driven spin control.

•Nov 5, 2025•0 citations

Observation of Tunable Superradiant Frequency Combs

Tian Xie, Rikuto Fukumori, Wai-Keong Mok +3 more

Cavity quantum electrodynamics (QED) with quantum emitters coupled to resonators provides a powerful platform for engineering light-matter interactions and exploring collective phenomena. In particular, superradiance, arising from collective quantum interference among emitters, has been explored as a route to ultrastable continuous radiation. However, engineering superradiance in the time domain to realize periodic pulsed sources or frequency combs remains largely unexplored. Here, we investigate the non-equilibrium many-body dynamics of a driven spin ensemble coupled to an on-chip superconducting resonator and uncover a dynamical phase transition from continuous-wave to periodic pulsed superradiant emission. To quantitatively capture the observed dynamical phases, we introduce a driven-dissipative cavity-QED model that elucidates how the periodic pulsed superradiant phase emerges from collective, periodically repeating spin dynamics stabilized by the interplay of coherence growth, disorder, and dissipation. We also find that rare-earth ion spin systems exhibiting both optical and microwave transitions enable phase-synchronized, dual-rail superradiant frequency combs in both the microwave and optical domains. Our results not only open new avenues for dual-rail frequency-comb applications in quantum metrology and information processing, but also establish a fundamental connection between periodic pulsed superradiance and the emergence of a continuous time crystal as a novel nonequilibrium phase in driven open systems.

quant-pharXiv:2604.14601•Apr 17, 2026•0 citations

Triggered Superradiance and Spin Inversion Storage in a Hybrid Quantum System

Wenzel Kersten, Nikolaus de Zordo, Oliver Diekmann +6 more

We study the superradiant emission of an inverted spin ensemble strongly coupled to a superconducting cavity. After fast inversion, we detune the spins from the cavity and store the inversion for tens of milliseconds, during which the remaining transverse spin components disappear. Switching back on resonance enables us to study the onset of superradiance. A weak trigger pulse of a few hundred photons shifts the superradiant burst to earlier times and imprints its phase onto the emitted radiation. For long hold times, the inversion decreases below the threshold for spontaneous superradiance. There, the energy stored in the ensemble can be used to amplify microwave pulses passing through the cavity.

arXiv:2301.04100•Physical Review Letters•Jul 25, 2023•12 citations

Sustained macroscopic quantum coherence in a superradiant solid under ambient conditions

Wei-Jiang Wu, Da-Wu Xiao, Wen-Tao Wang +5 more

Macroscopic quantum coherence, such as in laser, Bose-Einstein condensates, superfluids, and superconductors, is important to fundamental physics and useful for quantum technologies. Superradiance provides a mechanism to produce coherence among a large number of particles and photons. Its implementation, however, has been limited to gaseous systems, solids at very low temperature, or short pulses. Here we demonstrate a solid-state superradiant maser under ambient conditions, which establishes long-lived coherence among about $10^{14}$ nitrogen-vacancy center spins in diamond and about $10^9$ photons in a microwave cavity. By varying the system parameters to access the above-threshold, well-above-threshold, and deep-above-threshold regimes, we observed continuous-wave masing, periodic amplitude modulation, and sequences of superradiant bursts, which are attributed, correspondingly, to macroscopic spin coherence synchronized at a fixed frequency, a coherent time crystal of large spins, and unsynchronized superradiant transients. This work demonstrates that macroscopic quantum coherence can be spontaneously generated and maintained in solids under ambient conditions and provides a solid-state platform for exploring bright quantum lights with many-body correlations.

quant-pharXiv:2608.23748•Aug 26, 2026•0 citations

Quantum theory of the diamond maser: Stimulated and superradiant emission

Christoph W. Zollitsch, Jonathan Breeze

We present a quantum theory of diamond masers operating at any temperature using a cavity quantum electrodynamical framework. Special attention is paid to the recently demonstrated room-temperature solid-state masers based on nitrogen-vacancy (NV) defect centers in diamond, but the model can easily be modified for other photoexcited chromophores such as pentacene-doped paraterphenyl, vacancies in silicon-carbide or boron nitride. We show that the eight energy levels involved in the optically pumped NV center polarization process can be mapped to a simple pumped two-level-system. We then derive simple analytical expressions for the optical pump threshold condition for masing as well as the steady-state microwave output power which can be used to design and predict maser performance. Finally, we investigate second-order correlations and find that typical diamond masers operate in an intermediate regime between the good and bad cavity limits where photon emission is driven by both stimulated and superradiant processes.

Physical Review A•May 14, 2025•2 citations

Cavity-mediated coherence protection and one-axis twisting for spins in solids

Rikuto Fukumori, Chengyi Luo, Alexey Tiranov +3 more

Long-range interactions between emitters give rise to collective phenomena, including superradiance, spin squeezing, and coherence protection, that are important to both fundamental physics and quantum technologies. Despite progress in cold atoms, coherent cavity-mediated all-to-all interactions have not yet been realized in a solid-state ensemble. Here we demonstrate such interactions in a $^{171}$Yb$^{3+}$:CaWO$_4$ crystal coupled to a microwave resonator, observing superradiant emission on resonance and unitary one-axis twisting dynamics in the dispersive regime. The same interaction also opens a many-body energy gap that suppresses inhomogeneous dephasing, extending the ensemble Ramsey coherence time from tens of microseconds to milliseconds without decoupling pulses. These results establish a solid-state platform for collective many-body physics with direct implications for quantum technologies. Specifically, the observed one-axis twisting dynamics opens a path towards spin squeezing for entanglement-enhanced quantum metrology, and the extended coherence due to gap-protection is relevant for both microwave photon storage and precision measurement.

quant-pharXiv:2604.26909•Apr 30, 2026•0 citations
In cavity quantum electrodynamics and particularly superradiance, emitters are typically assumed to be independent, interacting only through light shared via a common mode. Although such photon-mediated interactions lead to a wide range of collective optical effects, direct dipole-dipole interactions within the emitter ensemble are generally viewed as a source of decoherence. Here we report the role of direct spin-spin interactions as a drive for the superradiant dynamics of a hybrid system of nitrogen-vacancy centre spins in a diamond coupled to a superconducting microwave cavity. After an initial fast superradiant burst, we observe a train of subsequent emission pulses followed by quasi-continuous masing for up to one millisecond. We show that this behaviour arises from spectral hole refilling, where spin inversion is redistributed into the superradiant window of spins resonant with the cavity. We report measurements that exclude other cavity-related effects and perform microscopic simulations that confirm that the observed behaviour is driven by dipole-dipole interactions between the spins. These findings open pathways for exploring complex spin-spin interactions in dense disordered systems and offer possibilities for ultranarrow-linewidth solid-state superradiant masers powered purely by microwave-driven spin control.
In cavity quantum electrodynamics (cQED) and particularly superradiance, emitters are typically assumed to be independent, interacting only through light shared via a common mode. While such photon-mediated interactions lead to a rich spectrum of collective optical effects, direct dipole-dipole interactions within the emitter ensemble are generally viewed as a source of decoherence. Here, we uncover a new role for direct spin-spin interactions as a drive for the superradiant dynamics of a hybrid system of nitrogen-vacancy center spins in diamond coupled to a superconducting microwave cavity. After an initial fast superradiant burst, we observe an unexpected train of subsequent emission pulses followed by quasi-continuous masing for up to one millisecond. We show that this surprising behavior arises from spectral hole refilling, where spin inversion is redistributed into the superradiant window of spins resonant with the cavity. We report measurements that clearly exclude other cQED-related effects, and performed microscopic simulations of up to one million spins, which demonstrate that the observed self-induced masing is indeed driven by dipole-dipole interactions between the spins. These findings open new pathways for exploring complex spin-spin interactions in dense disordered systems and offer possibilities for ultra-narrow linewidth solid-state superradiant masers powered purely by microwave-driven spin control.
Cavity quantum electrodynamics (QED) with quantum emitters coupled to resonators provides a powerful platform for engineering light-matter interactions and exploring collective phenomena. In particular, superradiance, arising from collective quantum interference among emitters, has been explored as a route to ultrastable continuous radiation. However, engineering superradiance in the time domain to realize periodic pulsed sources or frequency combs remains largely unexplored. Here, we investigate the non-equilibrium many-body dynamics of a driven spin ensemble coupled to an on-chip superconducting resonator and uncover a dynamical phase transition from continuous-wave to periodic pulsed superradiant emission. To quantitatively capture the observed dynamical phases, we introduce a driven-dissipative cavity-QED model that elucidates how the periodic pulsed superradiant phase emerges from collective, periodically repeating spin dynamics stabilized by the interplay of coherence growth, disorder, and dissipation. We also find that rare-earth ion spin systems exhibiting both optical and microwave transitions enable phase-synchronized, dual-rail superradiant frequency combs in both the microwave and optical domains. Our results not only open new avenues for dual-rail frequency-comb applications in quantum metrology and information processing, but also establish a fundamental connection between periodic pulsed superradiance and the emergence of a continuous time crystal as a novel nonequilibrium phase in driven open systems.
We study the superradiant emission of an inverted spin ensemble strongly coupled to a superconducting cavity. After fast inversion, we detune the spins from the cavity and store the inversion for tens of milliseconds, during which the remaining transverse spin components disappear. Switching back on resonance enables us to study the onset of superradiance. A weak trigger pulse of a few hundred photons shifts the superradiant burst to earlier times and imprints its phase onto the emitted radiation. For long hold times, the inversion decreases below the threshold for spontaneous superradiance. There, the energy stored in the ensemble can be used to amplify microwave pulses passing through the cavity.
Macroscopic quantum coherence, such as in laser, Bose-Einstein condensates, superfluids, and superconductors, is important to fundamental physics and useful for quantum technologies. Superradiance provides a mechanism to produce coherence among a large number of particles and photons. Its implementation, however, has been limited to gaseous systems, solids at very low temperature, or short pulses. Here we demonstrate a solid-state superradiant maser under ambient conditions, which establishes long-lived coherence among about 101410^{14}1014 nitrogen-vacancy center spins in diamond and about 10910^9109 photons in a microwave cavity. By varying the system parameters to access the above-threshold, well-above-threshold, and deep-above-threshold regimes, we observed continuous-wave masing, periodic amplitude modulation, and sequences of superradiant bursts, which are attributed, correspondingly, to macroscopic spin coherence synchronized at a fixed frequency, a coherent time crystal of large spins, and unsynchronized superradiant transients. This work demonstrates that macroscopic quantum coherence can be spontaneously generated and maintained in solids under ambient conditions and provides a solid-state platform for exploring bright quantum lights with many-body correlations.
We present a quantum theory of diamond masers operating at any temperature using a cavity quantum electrodynamical framework. Special attention is paid to the recently demonstrated room-temperature solid-state masers based on nitrogen-vacancy (NV) defect centers in diamond, but the model can easily be modified for other photoexcited chromophores such as pentacene-doped paraterphenyl, vacancies in silicon-carbide or boron nitride. We show that the eight energy levels involved in the optically pumped NV center polarization process can be mapped to a simple pumped two-level-system. We then derive simple analytical expressions for the optical pump threshold condition for masing as well as the steady-state microwave output power which can be used to design and predict maser performance. Finally, we investigate second-order correlations and find that typical diamond masers operate in an intermediate regime between the good and bad cavity limits where photon emission is driven by both stimulated and superradiant processes.
Long-range interactions between emitters give rise to collective phenomena, including superradiance, spin squeezing, and coherence protection, that are important to both fundamental physics and quantum technologies. Despite progress in cold atoms, coherent cavity-mediated all-to-all interactions have not yet been realized in a solid-state ensemble. Here we demonstrate such interactions in a 171^{171}171Yb3+^{3+}3+:CaWO4_44​ crystal coupled to a microwave resonator, observing superradiant emission on resonance and unitary one-axis twisting dynamics in the dispersive regime. The same interaction also opens a many-body energy gap that suppresses inhomogeneous dephasing, extending the ensemble Ramsey coherence time from tens of microseconds to milliseconds without decoupling pulses. These results establish a solid-state platform for collective many-body physics with direct implications for quantum technologies. Specifically, the observed one-axis twisting dynamics opens a path towards spin squeezing for entanglement-enhanced quantum metrology, and the extended coherence due to gap-protection is relevant for both microwave photon storage and precision measurement.