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arXiv:2402.07722 · Physical review. B./Physical review. B

Path integral Monte Carlo study of a doubly dipolar Bose gas

Ratheejit Ghosh, Matteo Ciardi, Rejish Nath, Fabio Cinti

Published Jul 16, 2024• 4 citations
arXivHTMLPDF

Abstract

By combining first-principles path integral Monte Carlo methods and mean-field techniques, we explore the properties of cylindrically trapped doubly dipolar Bose gases. We first verify the emergence of a pancake quantum droplet at low temperatures, validating previous mean-field calculations. In a regime of small doubly dipolar interactions, first-principles calculations agree with the generalized Gross-Pitaevskii equation. Such an accordance disappears in a large interaction limit. Here the path integral Monte Carlo method estimates the strong doubly dipolar regime with accuracy. In contrast, the Gross-Pitaevskii equation does not seize quantum fluctuations in full. We also provide a complete description of the system's quantum behavior in a wide range of parameters. When the system forms a droplet, the superfluid fraction exhibits an anisotropic behavior if compared to the usual Bose gas regime. Interestingly, we observe that the transition temperature from thermal gas to droplet is higher than that of the thermal gas to a Bose-Einstein condensate, indicating the robustness of the droplet against thermal fluctuations. Further, we investigate the anisotropic behavior of the superfluid fraction during the structural transition from a pancake to a cigar-shaped droplet by varying the ratio between electric and magnetic dipole interaction strengths. Our findings furnish evidence that the stability of doubly dipolar Bose-Einstein condensates can be detected in experiments by means of dysprosium atoms.

DOI
10.1103/physrevb.110.014513

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By combining first-principles path integral Monte Carlo methods and mean-field techniques, we explore the properties of cylindrically trapped doubly dipolar Bose gases. We first verify the emergence of a pancake quantum droplet at low temperatures, validating previous mean-field calculations. In a regime of small doubly dipolar interactions, first-principles calculations agree with the generalized Gross-Pitaevskii equation. Such an accordance disappears in a large interaction limit. Here the path integral Monte Carlo method estimates the strong doubly dipolar regime with accuracy. In contrast, the Gross-Pitaevskii equation does not seize quantum fluctuations in full. We also provide a complete description of the system's quantum behavior in a wide range of parameters. When the system forms a droplet, the superfluid fraction exhibits an anisotropic behavior if compared to the usual Bose gas regime. Interestingly, we observe that the transition temperature from thermal gas to droplet is higher than that of the thermal gas to a Bose-Einstein condensate, indicating the robustness of the droplet against thermal fluctuations. Further, we investigate the anisotropic behavior of the superfluid fraction during the structural transition from a pancake to a cigar-shaped droplet by varying the ratio between electric and magnetic dipole interaction strengths. Our findings furnish evidence that the stability of doubly dipolar Bose-Einstein condensates can be detected in experiments by means of dysprosium atoms.
The work of this thesis concerns the properties of a Bose gas of polarised dipoles that have long-range and anisotropic interactions. Our work is divided into two parts. First, the stability of a dipolar Bose gas at finite temperature (both above and below the critical Bose-Einstein condensation (BEC) temperature Tc). Second, the fluctuations of a dipolar BEC at zero and small finite temperature (T ≪ Tc) in a regime where rotonic excitations emerge. \n \nPart I: Stability of a Trapped Finite Temperature Dipolar Bose Gas: Above Tc we implement a semiclassical Hartree-Fock theory and characterise the dependence of the stability boundary on temperature, trap geometry and the strength of the dipole-dipole interaction and contact interaction. We find that stability is greatly enhanced above Tc and that trap geometry continues to play a key role. Furthermore, we find that for oblate traps a novel double instability feature emerges. \nTo extend our stability analysis to the low temperature regime, T < Tc, we develop a beyond semiclassical Hartree theory. We use this to characterise the stability boundary as a function of geometry. Interestingly, we find large beyond semiclassical effects above Tc for prolate trapping geometries. We characterise thermal effects on biconcave condensate states. \n \nPart II: Rotons and Fluctuations in a Trapped Dipolar Condensate: To study density fluctuations we implement a numerical scheme to solve the Gross-Pitaevskii equation and the Bogoliubov de Gennes equations. We find that the phonon and roton gases spatially separate and we characterise the role of the anomalous density on the density fluctuations of the thermally activated rotons. We develop a numerical scheme that calculates number fluctuations within cells of various shapes and sizes, and find a strong peak in the fluctuations when the cell size is around half the roton wavelength, which should be detectable by current experiments. By tailoring the cell shape we predict that experiments should be able to detect the effects of individual roton modes. \nFor the study of zero temperature fluctuations we deploy the Gross-Pitaevskii and Bogoliubov de Gennes equations to calculate the dynamic and static structure factors for a highly oblate BEC. We find a clear signature of the roton gas dispersion relation within the structure factors. This signature should be detectible in current experiments using Bragg spectroscopy.
Droplet states of ultracold gases which are stabilized by fluctuations have recently been observed in dipolar and two-component Bose gases. These systems present an alternate form of equilibrium where an instability at the mean-field level is arrested by higher-order correlations, making the droplet states sensitive probes of fluctuations. In a recent paper, we argued that thermal fluctuations can play an important role for droplets even at low temperatures where the noncondensed density is much smaller than the condensate density. We used the Hartree-Fock-Bogoliubov theory together with the local density approximation for fluctuations to obtain a generalized Gross-Pitaevskii (GP) equation and solved it with a Gaussian variational ansatz to show that the transition between the low density and droplet states can be significantly modified by the temperature. In this paper, we first solve the same GP equation numerically with a time-splitting spectral method to check the validity of the Gaussian variational ansatz. Our numerical results are in good agreement with the Gaussian ansatz for a large parameter regime and show that the density of the gas is most strongly modified by temperature near the abrupt transition between a pancake-shaped cloud and the droplet. For cigar-shaped condensates, as in the recent Er experiments, the dependence of the density on temperature remains quite small throughout the smooth transition. We then consider the effect of temperature on the collective oscillation frequencies of the droplet using both a time-dependent Gaussian variational ansatz and real-time numerical evolution. We find that the oscillation frequencies depend significantly on the temperature close to the transition for the experimentally relevant temperature regime ($\ensuremath{\simeq}100\phantom{\rule{4pt}{0ex}}\mathrm{nK}$).
We study thermal properties of a trapped Bose-Bose mixture in a dilute regime using quantum Monte Carlo methods. Our main aim is to investigate the dependence of the superfluid density and the condensate fraction on temperature for the mixed and separated phases. To this end we use the diffusion Monte Carlo method in the zero-temperature limit and the path-integral Monte Carlo method for finite temperatures. The results obtained are compared with solutions of the coupled Gross-Pitaevskii equations for the mixture at zero temperature. We notice the existence of an anisotropic superfluid density in some phase-separated mixtures. Our results also show that the temperature evolution of the superfluid density and condensate fraction is slightly different, showing noteworthy situations where the superfluid fraction is smaller than the condensate fraction.
Gases of doubly dipolar particles, with both magnetic and electric dipole moments, offer intriguing novel possibilities. We show that the interplay between doubly dipolar interactions, quantum stabilization, and external confinement results in a rich ground-state physics of supersolids and incoherent droplet arrays in doubly dipolar condensates. Our study reveals novel possibilities for engineering quantum droplets and droplet supersolids, including supersolid-supersolid transitions and the realization of supersolid arrays of pancake droplets.