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arXiv:2401.17353

Theory of a Strange Metal in a Quantum Superconductor to Metal Transition

Jaewon Kim, Erez Berg, Ehud Altman

Published Jan 30, 2024• 0 citations
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Abstract

Recent experiments with nanopatterned thin films revealed an unusual quantum superconductor to metal phase transition (QSMT) with a linear in temperature resistivity. In contrast, most known examples of such transitions and standard theoretical considerations predict a temperature-independent sheet resistance of order $R_Q = \frac{\hbar}{e^2}$. We propose an effective theory of a disordered superconductor which features a QSMT with robust $T$ linear resistivity at the critical point. The crucial ingredient in our model is spatial disorder in the pairing interaction. Such random pairing mirrors the emergent phase disorder seen in a recent mean field study of a microscopic $d$-wave superconductor subject to potential disorder. We also make the prediction that in such systems the diamagnetic susceptibility diverges as $\log\fracΛ{T}$, which starkly differs from the power law divergence in standard XY transitions.

DOI
10.48550/arxiv.2401.17353

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Recent experiments with nanopatterned thin films revealed an unusual quantum superconductor to metal phase transition (QSMT) with a linear in temperature resistivity. In contrast, most known examples of such transitions and standard theoretical considerations predict a temperature-independent sheet resistance of order RQ=ℏe2R_Q = \frac{\hbar}{e^2}RQ​=e2ℏ​. We propose an effective theory of a disordered superconductor which features a QSMT with robust TTT linear resistivity at the critical point. The crucial ingredient in our model is spatial disorder in the pairing interaction. Such random pairing mirrors the emergent phase disorder seen in a recent mean field study of a microscopic ddd-wave superconductor subject to potential disorder. We also make the prediction that in such systems the diamagnetic susceptibility diverges as log⁡ΛT\log\fracΛ{T}logTΛ​, which starkly differs from the power law divergence in standard XY transitions.
Fermi liquid theory forms the basis for our understanding of the majority of metals, which is manifested in the description of transport properties that the electrical resistivity goes as temperature squared in the limit of zero temperature. However, the observations of strange metal states in various quantum materials, notably high-temperature superconductors, bring this spectacularly successful theoretical framework into crisis. When electron scattering rate 1/τ hits its limit, kBT/{\hbar} where {\hbar} is the reduced Planck's constant, T represents absolute temperature and kB denotes Boltzmann's constant, Planckian dissipation occurs and lends strange metals a surprising link to black holes, gravity, and quantum information theory. Here, we show the characteristic signature of strange metallicity arising unprecedentedly in a bosonic system. Our nanopatterned YBa2Cu3O7-δ(YBCO) film arrays reveal T-linear resistance as well as B-linear magnetoresistance over an extended temperature and magnetic field range in a quantum critical region in the phase diagram. Moreover, the slope of the T-linear resistance α_cp appears bounded by α_cp {\approx} h/2e^2 [1/T]_c^onset where T_c^onset is the temperature at which Cooper pairs form, intimating a common scale-invariant transport mechanism corresponding to Planckian dissipation.In contrast to fermionic systems where the temperature and magnetic field dependent scattering rates combine in quadrature of {\hbar}/τ {\approx} {\sqrt} (((k_B T)^2+(μ_B B)^2)), both terms linearly combine in the present bosonic system, i.e. {\hbar}/τ {\approx} (k_B T+[γμ]_B B), where γ is a constant. By extending the reach of strange metal phenomenology to a bosonic system, our results suggest that there is a fundamental principle governing their transport which transcends particle statistics.
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Despite much theoretical effort, there is no complete theory of the "strange" metal state of the high temperature superconductors, and its linear-in-temperature T resistivity.Recent experiments showing an unexpected linear-in-field B magnetoresistivity have deepened the puzzle.We propose a simple model of itinerant electrons, interacting via random couplings, with electrons localized on a lattice of "quantum dots" or "islands."This model is solvable in a particular large-N limit and can reproduce observed behavior.The key feature of our model is that the electrons in each quantum dot are described by a Sachdev-Ye-Kitaev model describing electrons without quasiparticle excitations.For a particular choice of the interaction between the itinerant and localized electrons, this model realizes a controlled description of a diffusive marginal-Fermi liquid (MFL) without momentum conservation, which has a linear-in-T resistivity and a T ln T specific heat as T → 0. By tuning the strength of this interaction relative to the bandwidth of the itinerant electrons, we can additionally obtain a finite-T crossover to a fully incoherent regime that also has a linear-in-T resistivity.We describe the magnetotransport properties of this model and show that the MFL regime has conductivities that scale as a function of B=T; however, the magnetoresistance saturates at large B. We then consider a macroscopically disordered sample with domains of such MFLs with varying densities of electrons and islands.Using an effective-medium approximation, we obtain a macroscopic electrical resistance that scales linearly in the magnetic field B applied perpendicular to the plane of the sample, at large B. The resistance also scales linearly in T at small B, and as TfðB=TÞ at intermediate B. We consider implications for recent experiments reporting linear transverse magnetoresistance in the strange metal phases of the pnictides and cuprates.
The strange metal behavior, usually characterized by a linear-in-temperature (T) resistivity, is a still unsolved mystery in solid-state physics. Usually it is associated with the proximity to a quantum critical point (a second order transition at temperature T = 0) focusing on the related divergent order parameter correlation length. Here, we propose a paradigmatic shift, focusing on a divergent characteristic time scale due to a divergent dissipation acting on the fluctuating critical modes, while their correlation length stays finite. To achieve a divergent dissipation, we propose a mechanism based on the coupling between a local order parameter fluctuation and electronic diffusive modes, that accounts both for the linear-in-T resistivity and for the logarithmic specific heat versus temperature ratio C_V/T ~ log(1/T), down to low temperatures.
The strange metal phase of correlated electrons materials was described in a recent theory by a model of a Fermi surface coupled a two-dimensional quantum critical bosonic field with a spatially random Yukawa coupling. With the assumption of self-averaging randomness, similar to that in the Sachdev-Ye-Kitaev model, numerous observed properties of a strange metal were obtained for a wide range of intermediate temperatures, including the linear in temperature resistivity. The Harris criterion implies that spatial fluctuations in the local position of the critical point must dominate at lower temperatures. For an [Formula: see text]-component boson with [Formula: see text], we use multiple graphics processing units (GPUs) to compute the real frequency spectrum of the boson propagator in a self-consistent mean-field treatment of the boson self-interactions, but an exact treatment of multiple realizations of the spatial randomness from the random boson mass. We find that Landau damping from the fermions leads to the emergence of the physics of the random transverse-field Ising model at low temperatures, as has been proposed by Hoyos, Kotabage, and Vojta. This regime is controlled by localized overdamped eigenmodes of the bosonic scalar field, also has a resistivity which is nearly linear-in-temperature, and extends into a "quantum critical phase" away from the quantum critical point, as observed in several cuprates. For the [Formula: see text] Ising scalar, the mean-field treatment is not applicable, and so we use Hybrid Monte Carlo simulations running on multiple GPUs; we find a rounded transition and localization physics, with strange metal behavior in an extended region around the transition.
When subject to a pair-breaking perturbation, the pairing susceptibility of a disordered superconductor exhibits substantial long-ranged mesoscopic fluctuations. Focusing on a thin film subject to a parallel magnetic field, it is proposed that the quantum phase transition to the bulk superconducting condensate may be pre-empted by the formation of a glass-like phase with multi-fractal correlations of a complex order parameter. Although not universal, we argue that such behaviour may be a common feature of quantum critical phenomena in disordered environments.