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arXiv:2205.10876

Disorder-driven dissipative quantum criticality as a source of strange metal behavior

M. Grilli, C. Di Castro, G. Seibold, S. Caprara

Published May 22, 2022• 0 citations
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Abstract

The strange metal behavior, usually characterized by a linear-in-temperature (T) resistivity, is a still unsolved mystery in solid-state physics. Usually it is associated with the proximity to a quantum critical point (a second order transition at temperature T = 0) focusing on the related divergent order parameter correlation length. Here, we propose a paradigmatic shift, focusing on a divergent characteristic time scale due to a divergent dissipation acting on the fluctuating critical modes, while their correlation length stays finite. To achieve a divergent dissipation, we propose a mechanism based on the coupling between a local order parameter fluctuation and electronic diffusive modes, that accounts both for the linear-in-T resistivity and for the logarithmic specific heat versus temperature ratio C_V/T ~ log(1/T), down to low temperatures.

DOI
10.48550/arxiv.2205.10876

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The strange metal behavior, usually characterized by a linear-in-temperature (T) resistivity, is a still unsolved mystery in solid-state physics. Usually it is associated with the proximity to a quantum critical point (a second order transition at temperature T = 0) focusing on the related divergent order parameter correlation length. Here, we propose a paradigmatic shift, focusing on a divergent characteristic time scale due to a divergent dissipation acting on the fluctuating critical modes, while their correlation length stays finite. To achieve a divergent dissipation, we propose a mechanism based on the coupling between a local order parameter fluctuation and electronic diffusive modes, that accounts both for the linear-in-T resistivity and for the logarithmic specific heat versus temperature ratio C_V/T ~ log(1/T), down to low temperatures.
The strange metal behavior, usually characterized by a linear-in-temperature (T) resistivity, is a still unsolved mystery in solid-state physics. It is often associated with the proximity to a quantum critical point (a second order transition at temperature T=0, leading to a broken symmetry phase) focusing on the related divergent order parameter correlation length. Here, we propose a paradigmatic shift, focusing on a divergent characteristic time scale due to a divergent dissipation acting on the fluctuating critical modes while their correlation length stays finite. To achieve a divergent dissipation, we propose a mechanism based on the coupling between a local order parameter fluctuation and electron density diffusive modes that accounts both for the linear-in-T resistivity and for the logarithmic specific heat versus temperature ratio CV/T∼log(1/T), down to low temperatures.
Strange metals—ubiquitous in correlated quantum materials—transport electrical charge at low temperatures but not by the individual electronic quasiparticle excitations, which carry charge in ordinary metals. In this work, we consider two-dimensional metals of fermions coupled to quantum critical scalars, the latter representing order parameters or fractionalized particles. We show that at low temperatures ( T ), such metals generically exhibit strange metal behavior with a T -linear resistivity arising from spatially random fluctuations in the fermion-scalar Yukawa couplings about a nonzero spatial average. We also find a T ln(1/ T ) specific heat and a rationale for the Planckian bound on the transport scattering time. These results are in agreement with observations and are obtained in the large N expansion of an ensemble of critical metals with N fermion flavors.
Resilient strange metal at an unconventional quantum critical point in d=2d=2d=2
Properties of the two-dimensional Hubbard model with nearest-neighbor hopping are under scrutiny in cold-atom experiments and diagrammatic quantum Monte Carlo. Given the controlled nature of these approaches, it is timely to make predictions about strange-metal behavior and its relation to quantum-critical properties. Even for interaction strengths below the Mott transition, several peculiarities occur at the quantum critical point separating Fermi liquid and incommensurate spin-density wave order. Here, we predict, using the non-perturbative improved two-particle self-consistent approach, that for correlation lengths ranging from about one to one hundred lattice spacings, Kohn anomalies on the underlying Fermi surface lead to unconventional critical exponents. The temperature dependence of the single-particle self-energy acquires strong momentum dependence along the Fermi surface with no clear evidence of Landau quasiparticles. Nevertheless, we observe strange-metal behavior, namely, resistivity that scales linearly with temperature as T→0T\rightarrow{0}T→0. Our work shows that a linear temperature dependence of resistivity arises without a linear-in-temperature self-energy along the Fermi surface, as is often assumed.
“Strange” metals that do not follow the predictions of Fermi liquid theory are prevalent in materials that feature superconductivity arising from electron interactions. In recent years, it has been hypothesized that spatial randomness in electron interactions must play a crucial role in strange metals for their hallmark linear-in-temperature ( T ) resistivity to survive down to low temperatures where phonon and umklapp processes are ineffective, as is observed in experiments. However, a clear picture of how this happens has not yet been provided in a realistic model free from artificial constructions, such as large- N limits and replica tricks. We study a realistic model of two-dimensional metals with spatially random antiferromagnetic interactions in a nonperturbative regime, using numerically exact high-performance, large-scale hybrid Monte Carlo simulation and exact averages over the quenched spatial randomness. Our simulations reproduce strange metals’ key experimental signature of linear-in- T resistivity with a universal “Planckian” transport scattering rate Γ tr ∼ k B T / ℏ that is independent of coupling constants. We further find that strange metallicity in these systems is not associated with a quantum critical point and, instead, arises from a phase of matter with gapless antiferromagnetic fluctuations that lacks long-range correlations and spans an extended region of parameter space: A feature that is also observed in several experiments. These gapless antiferromagnetic fluctuations take the form of spatially localized overdamped modes, whose presence could possibly be detected using recently developed nanoscale magnetometry methods. Our work paves the way for an eventual microscopic understanding of the role of spatial disorder in determining important properties of correlated-electron materials.
The strange metal phase of correlated electrons materials was described in a recent theory by a model of a Fermi surface coupled a two-dimensional quantum critical bosonic field with a spatially random Yukawa coupling. With the assumption of self-averaging randomness, similar to that in the Sachdev-Ye-Kitaev model, numerous observed properties of a strange metal were obtained for a wide range of intermediate temperatures, including the linear in temperature resistivity. The Harris criterion implies that spatial fluctuations in the local position of the critical point must dominate at lower temperatures. For an [Formula: see text]-component boson with [Formula: see text], we use multiple graphics processing units (GPUs) to compute the real frequency spectrum of the boson propagator in a self-consistent mean-field treatment of the boson self-interactions, but an exact treatment of multiple realizations of the spatial randomness from the random boson mass. We find that Landau damping from the fermions leads to the emergence of the physics of the random transverse-field Ising model at low temperatures, as has been proposed by Hoyos, Kotabage, and Vojta. This regime is controlled by localized overdamped eigenmodes of the bosonic scalar field, also has a resistivity which is nearly linear-in-temperature, and extends into a "quantum critical phase" away from the quantum critical point, as observed in several cuprates. For the [Formula: see text] Ising scalar, the mean-field treatment is not applicable, and so we use Hybrid Monte Carlo simulations running on multiple GPUs; we find a rounded transition and localization physics, with strange metal behavior in an extended region around the transition.
Zero-temperature or quantum phase transitions in itinerant electronic systems both with and without quenched disordered are discussed. Phase transitions considered include, the ferromagnetic transition, the antiferromagnetic transition, the superconductor-metal transition, and various metal-insulator transitions. Emphasis is placed on how to determine the universal properties that characterize these quantum phase transitions. For the first three of the phase transitions listed above, one of the main physical ideas established is that in zero-temperature systems there are soft or slow modes that exist in addition to the soft order parameter fluctuations, and that these modes can couple to the critical modes. These extra soft modes are shown to have a profound effect on the quantum critical properties. For quantum phase transitions involving zero wavenumber order parameters, i.e., the ferromagnetic and superconductor-metal transitions, these extra modes effectively lead to long-ranged effective interactions between order parameter fluctuations, which in turn lead to exactly soluble critical behaviors. For the antiferromagnetic case, we argue that while in low enough dimensions disorder fluctuation effects tend to destroy long-range order, quantum fluctuations counteract this effect and in some parameter regions manage to re-establish antiferromagnetic long-range order. For the metal-insulator transition, some recent new ideas are reviewed. In particular, it is pointed out that for interacting disordered electrons, one expects that in high dimensions the metal-insulator transition is related to the phase transition that occurs in random-field magnets in high dimensions. If the analogy also holds in three dimensions this suggests that the metal-insulator transition might have glassy characteristics.