The strongly ferromagnetic spin-1 Bose-Einstein condensate has recently been realized with atomic Li7 . It was predicted that a strong ferromagnetic interaction can drive the normal gas into a magnetized phase at a temperature above the superfluid transition, and Li7 likely satisfies the criterion. We reexamine this theoretical proposal employing the two-particle-irreducible effective potential, and conclude that there exists no stable normal magnetized phase for a dilute ferromagnetic Bose gas. For Li7 , we predict that the normal gas undergoes a joint first-order transition and jumps directly into a state with finite condensate density and magnetization. We estimate the size of the first-order jump and examine how a partial spin polarization in the initial sample affects the first-order transition. We propose a qualitative phase diagram at fixed temperature for the trapped gas. Published by the American Physical Society 2024
The strongly ferromagnetic spin-1 Bose-Einstein condensate has recently been realized with atomic Li7 . It was predicted that a strong ferromagnetic interaction can drive the normal gas into a magnetized phase at a temperature above the superfluid transition, and Li7 likely satisfies the criterion. We reexamine this theoretical proposal employing the two-particle-irreducible effective potential, and conclude that there exists no stable normal magnetized phase for a dilute ferromagnetic Bose gas. For Li7 , we predict that the normal gas undergoes a joint first-order transition and jumps directly into a state with finite condensate density and magnetization. We estimate the size of the first-order jump and examine how a partial spin polarization in the initial sample affects the first-order transition. We propose a qualitative phase diagram at fixed temperature for the trapped gas. Published by the American Physical Society 2024
We find the conditions under which the normal state of a spin-1 Bose gas is unstable toward condensation, ferromagnetism, liquid crystalline-like nematicity, and Bardeen-Cooper-Schrieffer-like pairing. When the spin-dependent interactions are much weaker than the density-density interaction there is direct transition from a featureless normal state to a fully ordered Bose-Einstein condensate with either ferromagnetic or nematic order. When the spin-independent and spin-dependent interactions are of comparable magnitude, we find several different symmetry breaking transitions at intermediate temperatures above the Bose-condensation transition temperature. We make predictions for the Tc for these transitions, and assess the role of magnetic field and finite system size.
Spinor Bose gases may exhibit both phase and ferromagnetic order. Consequently, they may support superflow of both mass and spin currents. In this thesis we utilize a stochastic Gross-Pitaevskii model to investigate the superfluid properties of a two-dimensional spin-1 Bose gas with ferromagnetic interactions. Owing to the low dimensionality, the superfluidity of this system can not be attributed to the presence of a Bose-Einstein condensate, with thermal fluctuations precluding long-range order. Rather, mass and spin superfluidity emerge via respective Berezinskii-Kosterlitz-Thouless (BKT) transitions. Such transitions are characterized by the emergence of quasi-long-range order, driven by the binding of topological defect pairs. First, we consider an easy-plane ferromagnetic gas. We find the system superfluidity may be understood by direct application of existing BKT theory. In particular, mass and spin superfluidity are respectively associated with quasi-long-range order in the global phase and local magnetization. The former arises from the binding of mass vortex pairs, while the latter arises from the binding of polar-core spin vortex pairs. Following this, we introduce axial magnetization, and consider a gas in the broken-axisymmetric phase. We find axial magnetization acts to couple mass and spin superflows via a mechanism analogous to the superfluid drag exhibited by two-component superfluids. This coupling renders invalid the direct applicability of existing BKT theory: here mass and spin superfluidity may each be associated with both phase and magnetic order. We remedy this with a generalization making concrete the relation between superfluidity and quasi-long-range order in this system. In addition, through variations of the quadratic Zeeman energy and axial magnetization we identify three distinct superfluid phases, which serve as finite-temperature generalizations of the polar, broken-axisymmetric, and easy-axis ferromagnetic ground states.
By studying the zero-temperature and nonzero-temperature phase diagrams of the ferromagnetic spin-1 Bose-Hubbard model under an external magnetic field, we find that the competition between ferromagnetism and the quadratic Zeeman energy yields two superfluid phases, which feature discontinuous first-order phase transitions between them for a strongly spinor Bose gas such as 7Li, contrary to the corresponding continuum system.
Bose-Einstein condensation, observed in either strongly interacting liquid helium or weakly interacting atomic Bose gases, is widely known to be a second-order phase transition. Here we predict a first-order Bose-Einstein condensation in a cloud of harmonically trapped bosons interacting with both attractive two-body interaction and repulsive three-body interaction, characterized respectively by an s-wave scattering length a<0 and a three-body scattering hypervolume D>0. It happens when the harmonic trapping potential is weak, so with increasing temperature the system changes from a low-temperature liquidlike quantum droplet to a normal gas and therefore experiences a first-order liquid-to-gas transition. At large trapping potential, however, the quantum droplet can first turn into a superfluid gas, rendering the condensation transition occurring later from a superfluid gas to a normal gas smooth. We determine a rich phase diagram and show the existence of a tricritical point, where the three phases, i.e., quantum droplet, superfluid gas, and normal gas, meet. We argue that an ensemble of spin-polarized tritium atoms could be a promising candidate to observe the predicted first-order Bose-Einstein condensation, across which the condensate fraction or central condensate density jumps to zero and the surface-mode frequencies diverge.
We compute the finite-temperature phase diagram of a pseudospin-1/2 Bose gas with contact interactions, using two complementary methods: the random-phase approximation and self-consistent Hartree-Fock theory. We show that the spin-dependent interactions, which break the (pseudo-) spin-rotational symmetry of the Hamiltonian, generally lead to the appearance of a magnetically ordered phase at temperatures above the superfluid transition. In three dimensions, we predict a normal easy-axis (easy-plane) ferromagnet for sufficiently strong repulsive (attractive) interspecies interactions, respectively. The normal easy-axis ferromagnet is the bosonic analog of Stoner ferromagnetism known in electronic systems. For the case of interspecies attraction, we also discuss the possibility of a bosonic analog of the Cooper-paired phase. This state is shown to significantly lose in energy to the transverse ferromagnet in three dimensions, but is more energetically competitive in lower dimensions. Extending our calculations to a spin-orbit-coupled Bose gas with equal Rashba and Dresselhaus-type couplings (as recently realized in experiment), we investigate the possibility of stripe ordering in the normal phase. Within our approximations, however, we do not find an instability towards stripe formation, suggesting that the stripe order melts below the condensation temperature, which is consistent with the experimental observations of Ji et al. [Ji et al., Nat. Phys. 10, 314 (2014)].
In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field B. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field Bc, asymptotic values of n0 (relative atom number in mF=0 state) at large B and the phase diagram of n0. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of n0. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" Ts and the ``kinetic temperature" Tk with Ts≪Tk, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.