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arXiv:2401.10665 · Physical Review Letters

Optoacoustic Entanglement in a Continuous Brillouin-Active Solid State System

Changlong Zhu, Claudiu Genes, Birgit Stiller

Published Nov 13, 2024• 12 citations
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Abstract

Entanglement in hybrid quantum systems comprised of fundamentally different degrees of freedom, such as light and mechanics, is of interest for a wide range of applications in quantum technologies. Here, we propose to engineer bipartite entanglement between traveling acoustic phonons in a Brillouin active solid state system and the accompanying light wave. The effect is achieved by applying optical pump pulses to state-of-the-art waveguides, exciting a Brillouin Stokes process. This pulsed approach, in a system operating in a regime orthogonal to standard optomechanical setups, allows for the generation of entangled photon-phonon pairs, resilient to thermal fluctuations. We propose an experimental platform where readout of the optoacoustics entanglement is done by the simultaneous detection of Stokes and anti-Stokes photons in a two-pump configuration. The proposed mechanism presents an important feature in that it does not require initial preparation of the quantum ground state of the phonon mode.

DOI
10.1103/physrevlett.133.203602

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Entanglement in hybrid quantum systems comprised of fundamentally different degrees of freedom, such as light and mechanics, is of interest for a wide range of applications in quantum technologies. Here, we propose to engineer bipartite entanglement between traveling acoustic phonons in a Brillouin active solid state system and the accompanying light wave. The effect is achieved by applying optical pump pulses to state-of-the-art waveguides, exciting a Brillouin Stokes process. This pulsed approach, in a system operating in a regime orthogonal to standard optomechanical setups, allows for the generation of entangled photon-phonon pairs, resilient to thermal fluctuations. We propose an experimental platform where readout of the optoacoustics entanglement is done by the simultaneous detection of Stokes and anti-Stokes photons in a two-pump configuration. The proposed mechanism presents an important feature in that it does not require initial preparation of the quantum ground state of the phonon mode.
Storage and retrieval of optical quantum states are key elements for the realization of quantum communication and quantum networks. Here, we propose to realize a memory for light states in Brillouin-active waveguides. It is achieved by transferring quantum states between optical photons and acoustic phonons via Brillouin anti-Stokes scattering. By controlling the optoacoustic interaction with pulsed pumps, we demonstrate that it is possible to write, store, and read out of optical quantum states with high fidelity in state-of-the-art Brillouin-active waveguides.
Quantum memories for optical states are essential resources for quantum communication and information processing. We propose a quantum memory protocol based on coherent photon-phonon transduction in a Brillouin-active optical waveguide supporting traveling acoustic modes. A pulsed pump drives an effective beam-splitter interaction between optical and acoustic fields, enabling the mapping of a propagating optical quantum state onto a traveling phononic excitation and its subsequent retrieval on demand. Using a continuum optoacoustic model, we show that the protocol enables broadband quantum state storage in a distributed medium without relying on discrete cavity modes. Analytical and numerical results demonstrate high-fidelity storage and retrieval of squeezed and entangled states under experimentally realistic parameters. The memory bandwidth is set by the Brillouin interaction and can reach hundreds of MHz. Our results identify continuum Brillouin optomechanical systems as a scalable platform for broadband quantum memories and multimode quantum signal processing.
Brillouin optomechanics provides a way to coherently control traveling acoustic excitations in waveguides system, which enables the manipulation and processing of classical and quantum information. Although Brillouin optomechanics has been largely investigated in the steady-state regime using continuous waves [1]–[3], waveguide experiments are often realized by using optical pulses for example for Brillouin-based memory [4], [5]. This requires a dynamic framework treatment for the temporal domain including the noise dynamics.
Optical and acoustic waves can interact over the nonlinear effect of stimulated Brillouin scattering (SBS), which is a coherent process. By using traveling acoustic waves, we recently showed proof-of-principle experiments of Brillouin-based light storage. The particularity of Brillouin-based light storage is the strict phase-matching condition. This allows for different features: simultaneous storage at multiple wavelengths, cascaded storage at different spatial positions, and nonreciprocal storage with a GHz bandwidth. However, the delay time of this technique has so far been limited to the acoustic lifetime of about 10 ns. In this talk, I will discuss our recent results on coherent photon-phonon interaction. One focus will be on a proof-of-principle experiments on how to reinforce acoustic phonons. This enables us to overcome the obstacle of the limited acoustic lifetime by optically reinforcing the acoustic wave.
We propose a molecular optomechanical platform to generate robust entanglement among bosonic modes-photons, phonons, and plasmons-under ambient conditions. The system integrates a high-Q whispering-gallery-mode (WGM) optical resonator with a plasmonic nanocavity formed by a metallic nanoparticle and a single molecule. This hybrid architecture offers two critical advantages over stand-alone plasmonic systems: (i) efficient redirection of Stokes photons from the lossy plasmonic mode into the long-lived WGM resonator and (ii) suppression of molecular absorption and sustaining vibrational ground states via plasmon-WGM interactions. These features enable entanglement to redistribute from the fragile plasmon-phonon bipartition to a robust photon-phonon bipartition in the blue-detuned regime, yielding robust stationary entanglement resilient to environmental noise. Remarkably, the achieved entanglement surpasses the theoretical bound for conventional two-mode squeezing in certain parameter regimes. Our scheme establishes a universal approach to safeguard entanglement in open quantum systems and opens avenues for noise-resilient quantum information technologies.