Multimode squeezed states of light are a resource for achieving quantum advantage in computing and sensing, where spatial or temporal modes have been the experimental norm. In our experiments, we generated highly frequency-multimode infrared quantum light, and show how adiabatic frequency conversion can be used to convert the quantum state to visible wavelengths, while concurrently manipulating the joint spectrum by realizing a configurable many-port frequency-domain-beamsplitter unitary transformation. We report near-unity-efficiency quantum frequency conversion over a bandwidth >45 THz, which allowed us to measure the state with an electron-multiplying CCD (EMCCD) camera-based spectrometer, at non-cryogenic temperatures. The parametric amplification and conversion of >400 frequency modes yielded an overall mean of approximately 700 visible photons per shot, and photon statistics consistent with squeezing. Our work shows how many-mode quantum states of light can be generated, manipulated, and measured with efficient use of hardware resources, motivating the use of frequency encoding in quantum optics.
Multimode squeezed states of light are a resource for achieving quantum advantage in computing and sensing, where spatial or temporal modes have been the experimental norm. In our experiments, we generated highly frequency-multimode infrared quantum light, and show how adiabatic frequency conversion can be used to convert the quantum state to visible wavelengths, while concurrently manipulating the joint spectrum by realizing a configurable many-port frequency-domain-beamsplitter unitary transformation. We report near-unity-efficiency quantum frequency conversion over a bandwidth >45 THz, which allowed us to measure the state with an electron-multiplying CCD (EMCCD) camera-based spectrometer, at non-cryogenic temperatures. The parametric amplification and conversion of >400 frequency modes yielded an overall mean of approximately 700 visible photons per shot, and photon statistics consistent with squeezing. Our work shows how many-mode quantum states of light can be generated, manipulated, and measured with efficient use of hardware resources, motivating the use of frequency encoding in quantum optics.
Quantum frequency conversion, the process of shifting the frequency of an optical quantum state while preserving quantum coherence, can be used to produce non-classical light at otherwise unapproachable wavelengths. We present experimental results based on highly efficient sum-frequency generation (SFG) between a vacuum squeezed state at 1064 nm and a tunable pump source at 850 nm ± 50 nm for the generation of bright squeezed light at 472 nm ± 4 nm, currently limited by the phase-matching of the used nonlinear crystal. We demonstrate that the SFG process conserves part of the quantum coherence as a 4.2(±0.2) dB 1064 nm vacuum squeezed state is converted to a 1.6(±0.2) dB tunable bright blue squeezed state. We furthermore demonstrate simultaneous frequency- and spatial-mode conversion of the 1064-nm vacuum squeezed state, and measure 1.1(±0.2) dB and 0.4(±0.2) dB of squeezing in the TEM01 and TEM02 modes, respectively. With further development, we foresee that the source may find use within fields such as sensing, metrology, spectroscopy, and imaging.
Quantum frequency conversion, the process of shifting the frequency of an optical quantum state while preserving quantum coherence, can be used to produce non-classical light at otherwise unapproachable wavelengths. We present experimental results based on highly efficient sum-frequency generation (SFG) between a vacuum squeezed state at 1064 nm and a tunable pump source at 850 nm ± 50 nm for the generation of bright squeezed light at 472~nm ± 4~nm, currently limited by the phase-matching of the used nonlinear crystal. We demonstrate that the SFG process conserves part of the quantum coherence as a 4.2(±0.2)~dB 1064 nm vacuum squeezed state is converted to a 1.6($\pm0.2)dBtunablebrightbluesqueezedstate.Wefurthermoredemonstratesimultaneousfrequency−andspatial−modeconversionofthe1064−nmvacuumsqueezedstate,andmeasure1.1(\pm0.2)dBand0.4(\pm0.2)dBofsqueezingintheTEM_{01}$ and TEM02 modes, respectively. With further development, we foresee that the source may find use within fields such as sensing, metrology, spectroscopy, and imaging.
Photonics offers the potential for large-scale, room-temperature, and ultrafast quantum operations. Multiplexing pulses of light allows for high throughput speeds and dense encoding, with tens of thousands of optical modes being present in a time as short as a microsecond. However, the measurement speed of electronic devices such as photodetectors is currently one bottleneck in such time-multiplexed scalability, because many quantum optical protocols rely on measurement, including state preparation, feed-forward, and feedback. Furthermore, characterization of quantum states and modes is essential for their effective use. Using nanophotonic optical parametric amplifiers (OPAs) presents one way to circumvent the measurement limitations of current quantum photonic schemes. Their large amplification bandwidth, enabled by dispersion engineering on nanophotonic integrated platforms, allows information encoded in femtosecond-scale, THz-bandwidth, multimode quantum optical states to be accessed with nonlinear optical interactions. In this work, we show how ultra-broadband integrated nanophotonic OPAs can be used to measure ultrafast and multimode quantum states of light. First, we explore the single-photon detection capabilities of OPAs, showing that current OPAs operating in the Gaussian regime are capable of 250 MHz photon count rates with 26% efficiency and a 2% dark count probability. We also show how non-Gaussian operation through pump depletion, with performance that approaches state-of-the-art photon detectors in terms of efficiency and dark count rate while retaining ultrafast operation, can become experimentally possible with a higher nonlinear coupling rate and lower loss. Next, we use nanophotonic OPAs to both generate and characterize multimode ultrafast squeezed vacuum. We use the photocurrent distribution of amplified squeezed vacuum to recover 2.41 dB of squeezing in one mode of a 154-fs multimode squeezed pulse and reconstruct its Wigner distribution. Finally, we investigate the capabilities of broadband nanophotonic OPAs to determine the temporal mode structure and quadrature variances of ultra-broadband temporally multimode quantum states by adapting frequency-resolved optical gating to the quantum regime. We numerically show the successful full characterization of a multimode squeezed state, even in the presence of noise. Together, these results establish OPAs as a valuable measurement device for measuring ultrafast quantum pulses and learning the structure of multimode quantum states, and they provide one building block towards a framework for scalable continuous-variable quantum photonics in which state generation, manipulation, and characterization occur within the same nanophotonic platform.
Multimode entangled states of light are key resources for high-dimensional photonic quantum technologies, particularly for continuous-variable quantum computing and quantum information processing. Exploiting their full capabilities requires detection strategies that can efficiently and simultaneously access a large number of modes and their quantum correlations. Multimode optical parametric amplification (MOPA) provides a promising approach by amplifying multiple quadratures prior to detection, rendering the measurement robust against subsequent optical losses while enabling broadband operation. Here, we demonstrate the spectral multimode capability of MOPA by simultaneously characterizing a broadband 60-node dual-rail continuous-variable cluster state. We reconstruct the cluster-state nullifiers across the spectral modes and observe nearly uniform squeezing ranging from -7.2 to -6.5 dB. Furthermore, by evaluating the van Loock-Furusawa criterion across all relevant bipartitions, we verify genuine multipartite entanglement throughout the 60-node state. These results establish MOPA as a promising platform for scalable high-dimensional quantum information processing in the spectral domain.
Quantum optics has been, from its beginning, a driving force both for the exploration of fundamental limits of the quantum world and for conceiving seminal ideas and applications of the so-called quantum technologies. The last 20 years have seen a rapid development of ideas and proof-of-principle experiments involving the fields of quantum communication, quantum computation, quantum metrology and quantum simulation. The so called continuous variable (CV) approach to quantum optics, which uses many photon in collective states, and continuous observables like the quadratures of the electric field to encode information, has many interesting properties, especially from a communications perspective. It is inherently broadband and compatible with standard telecom infrastructures. Moreover, in CV, entanglement, one of the fundamental resource of quantum optics, can be generated deterministically. One of the main challenges for all quantum information technologies is scalability, being able to generate and manipulate a large number of quantum resources to achieve practical tasks efficiently. One approach to solve the issue of scalability is to use highly multimode quantum states. The quantum description of the electromagnetic field associate each photon (particle of light) with a mode (way for light to propagate). In a mutlimodal approach, we look at the quantum state bases and optical modes bases conjointly and tailor quantum fields not only in given modes, but also optimize the spatio-temporal shapes of the modes in which the state is defined. This opens wide perspectives for treating complex quantum states. In particular, using ultra-fast pulses of light which contain many temporal/spectral modes, we are able to generate large and complex entangled states of light using simple resources. In this thesis, we used an optical parametric oscillator pumped synchronously (SPOPO) with a frequency comb to generate multimode squeezed vacuum states which can be used to form cluster states: a large collection of modes (the nodes) entangled to each other in a certain way. These state are the basic resource for Measurement Based Quantum Computation (MBQC). This set-up has the advantage to generate entanglement in many mode with a single device. It is also highly tunable. Indeed, by tuning the spectrum of the OPO pump with a pulse shaper, one can tailor the properties of the generated quantum state. In this work, we focus on the optimization of the pump spectral shape to generate specific states. Using simulations based on Machine Learning Algorithms (MLA), we find optimal pump profile for typical target states. We then implement those shapes on the experimental set-up and measure the resulting states using multipixel homodyne detection. We also study intra-cavity dispersion effects. Dispersion inside the SPOPO cavity is indeed one of the main factor that limits the number of entangled modes in the generated quantum states. A systematic study of dispersion effects is therefore necessary to model the SPOPO output accurately. This works paves the way toward a fully tunable device that can be optimized in real time to generate specific quantum resources tailored for specific tasks.