Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2401.04717 · Journal of Physics B Atomic Molecular and Optical Physics

Analytical solutions for optimal photon absorption into inhomogeneous spin memories

József Zsolt Bernád, Michael Schilling, Yutian Wen, Matthias M. Müller, Tommaso Calarco, Patrice Bertet, Felix Motzoi

Published Jan 21, 2025• 3 citations
arXivHTMLPDF

Abstract

Abstract We investigate for optimal photon absorption a quantum electrodynamical model of an inhomogeneously-broadened spin ensemble coupled to a single-mode cavity. Solutions to this problem under experimental assumptions are developed in the Schrödinger picture without using perturbation theory concerning the cavity-spin interactions. Furthermore, we exploit the possibility of modulating the frequency and coupling rate of the resonator. We consider a one-photon input pulse and show some optimal scenarios, where exact formulas and numerical results are obtained for the absorption probabilities and the optimal pulse shapes. In particular, if the external loss dominates the internal loss of the cavity, we find the optimal cooperativity for different parameters and identify cases where absorption with a success probability larger than 99% is achieved.

DOI
10.1088/1361-6455/adacbf

Related papers

Optimally Controlled Storage of a Qubit in an Inhomogeneous Spin Ensemble

Rahul Gupta, Florian Mintert, Himadri Shekhar Dhar

The storage of quantum information in spin-ensembles is limited by practically unavoidable inhomogeneous broadening, and the macroscopic number of spins in such an ensemble makes the design of control solutions to increase the coherence time a challenging task. Together with a concurrently developed Krylov theory that allows us to treat the control problem efficiently, we design optimal cavity modulation for such spin ensembles that achieve an order of magnitude enhancement in qubit lifetime compared to the losses due to inhomogeneity and cavity decay.

quant-pharXiv:2604.13904•Apr 16, 2026•0 citations

Optimal storage of a single photon by a single intra-cavity atom

Luigi Giannelli, Tom Schmit, Tommaso Calarco +3 more

We theoretically analyze the efficiency of a quantum memory for single photons. The photons propagate along a transmission line and impinge on one of the mirrors of a high-finesse cavity. The quantum memory is constituted by a single atom within the optical resonator. Photon storage is realized by the controlled transfer of the photonic excitation into a metastable state of the atom and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom. Our study is supported by numerical simulations, in which we include the modes of the transmission line and we use the experimental parameters of existing experimental setups. It reproduces the results derived using input–output theory in the corresponding regimes and can be extended to compute dynamics where the input–output formalism cannot be straightforwardly applied. Our analysis determines the maximal storage efficiency, namely, the maximal probability to store the photon in a stable atomic excitation, in the presence of spontaneous decay and cavity parasitic losses. It further delivers the form of the laser pulse that achieves the maximal efficiency by partially compensating parasitic losses. We numerically assess the conditions under which storage based on adiabatic dynamics is preferable to non-adiabatic pulses. Moreover, we systematically determine the shortest photon pulse that can be efficiently stored as a function of the system parameters.

arXiv:1804.10558•New Journal of Physics•Oct 10, 2018•41 citations

Figure of merit for single-photon generation based on cavity quantum electrodynamics

Hayato Goto, Shota Mizukami, Yuuki Tokunaga +1 more

We investigate a tradeoff relation between the internal generation efficiency and the escape efficiency for single-photon generation based on cavity quantum electrodynamics, where cavity internal loss is treated explicitly. Consequently, we analytically derive an upper bound on the overall efficiency. The bound is expressed only with an internal cooperativity, introduced here as the cooperativity parameter with respect to the cavity internal loss rate. This result means that the internal cooperativity is a figure of merit for single-photon generation based on cavity QED. The bound is derived by optimizing the cavity external loss rate, which can be experimentally controlled by designing or tuning the transmissivity of the output coupler. The model here is general enough to treat various cavity-QED effects, such as the Purcell effect, on-resonant or off-resonant cavity-enhanced Raman scattering, and vacuum-stimulated Raman adiabatic passage. For typical optical systems, we additionally take into account a ``reexcitation'' process, where the atom is reexcited after its decay to the initial ground state.

arXiv:1808.10077•Physical Review A•May 28, 2019•40 citations

Non-Markovian dynamics of a single-mode cavity strongly coupled to an inhomogeneously broadened spin ensemble

Dmitry O. Krimer, Stefan Putz, Johannes Majer +1 more

We study the dynamics of a spin ensemble strongly coupled to a single-mode resonator driven by external pulses. When the mean frequency of the spin ensemble is in resonance with the cavity mode, damped Rabi oscillations are found between the spin ensemble and the cavity mode which we describe very accurately, including the dephasing effect of the inhomogeneous spin broadening. We demonstrate that a precise knowledge of this broadening is crucial both for a qualitative and a quantitative understanding of the temporal spin-cavity dynamics. On this basis we show that coherent oscillations between the spin ensemble and the cavity can be enhanced by a few orders of magnitude, when driving the system with pulses that match special resonance conditions. Our theoretical approach is tested successfully with an experiment based on an ensemble of negatively charged nitrogen-vacancy centers in diamond strongly coupled to a superconducting coplanar single-mode waveguide resonator.

arXiv:1410.0728•Physical Review A•Oct 24, 2014•42 citations

Proposal for a coherent quantum memory for propagating microwave photons

Afzelius, M., Nicolas Sangouard, Göran Johansson +2 more

We describe a multi-mode quantum memory for propagating microwave photons that combines a solid-state spin ensemble resonantly coupled to a frequency tunable single-mode microwave cavity. We first show that high efficiency mapping of the quantum state transported by a free photon to the spin ensemble is possible both for strong and weak coupling between the cavity mode and the spin ensemble. We also show that even in the weak coupling limit unit efficiency and faithful retrieval can be obtained through time reversal inhomogeneous dephasing based on spin echo techniques. This is possible provided that the cavity containing the spin ensemble and the transmission line are impedance matched. We finally discuss the prospects for an experimental implementation using a rare-earth doped crystal coupled to a superconducting resonator.

•Jan 1, 2013•21 citations

Proposal for a coherent quantum memory for propagating microwave photons

M Afzelius, Nicolas Sangouard, G Johansson +2 more

We describe a multi-mode quantum memory for propagating microwave photons that combines a solid-state spin ensemble resonantly coupled to a frequency tunable single-mode microwave cavity. We first show that high efficiency mapping of the quantum state transported by a free photon to the spin ensemble is possible both for strong and weak coupling between the cavity mode and the spin ensemble. We also show that even in the weak coupling limit unit efficiency and faithful retrieval can be obtained through time reversal inhomogeneous dephasing based on spin echo techniques. This is possible provided that the cavity containing the spin ensemble and the transmission line are impedance matched. We finally discuss the prospects for an experimental implementation using a rare-earth doped crystal coupled to a superconducting resonator.

arXiv:1301.1858•New Journal of Physics•Jun 17, 2013•55 citations
Abstract We investigate for optimal photon absorption a quantum electrodynamical model of an inhomogeneously-broadened spin ensemble coupled to a single-mode cavity. Solutions to this problem under experimental assumptions are developed in the Schrödinger picture without using perturbation theory concerning the cavity-spin interactions. Furthermore, we exploit the possibility of modulating the frequency and coupling rate of the resonator. We consider a one-photon input pulse and show some optimal scenarios, where exact formulas and numerical results are obtained for the absorption probabilities and the optimal pulse shapes. In particular, if the external loss dominates the internal loss of the cavity, we find the optimal cooperativity for different parameters and identify cases where absorption with a success probability larger than 99% is achieved.
The storage of quantum information in spin-ensembles is limited by practically unavoidable inhomogeneous broadening, and the macroscopic number of spins in such an ensemble makes the design of control solutions to increase the coherence time a challenging task. Together with a concurrently developed Krylov theory that allows us to treat the control problem efficiently, we design optimal cavity modulation for such spin ensembles that achieve an order of magnitude enhancement in qubit lifetime compared to the losses due to inhomogeneity and cavity decay.
We theoretically analyze the efficiency of a quantum memory for single photons. The photons propagate along a transmission line and impinge on one of the mirrors of a high-finesse cavity. The quantum memory is constituted by a single atom within the optical resonator. Photon storage is realized by the controlled transfer of the photonic excitation into a metastable state of the atom and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom. Our study is supported by numerical simulations, in which we include the modes of the transmission line and we use the experimental parameters of existing experimental setups. It reproduces the results derived using input–output theory in the corresponding regimes and can be extended to compute dynamics where the input–output formalism cannot be straightforwardly applied. Our analysis determines the maximal storage efficiency, namely, the maximal probability to store the photon in a stable atomic excitation, in the presence of spontaneous decay and cavity parasitic losses. It further delivers the form of the laser pulse that achieves the maximal efficiency by partially compensating parasitic losses. We numerically assess the conditions under which storage based on adiabatic dynamics is preferable to non-adiabatic pulses. Moreover, we systematically determine the shortest photon pulse that can be efficiently stored as a function of the system parameters.
We investigate a tradeoff relation between the internal generation efficiency and the escape efficiency for single-photon generation based on cavity quantum electrodynamics, where cavity internal loss is treated explicitly. Consequently, we analytically derive an upper bound on the overall efficiency. The bound is expressed only with an internal cooperativity, introduced here as the cooperativity parameter with respect to the cavity internal loss rate. This result means that the internal cooperativity is a figure of merit for single-photon generation based on cavity QED. The bound is derived by optimizing the cavity external loss rate, which can be experimentally controlled by designing or tuning the transmissivity of the output coupler. The model here is general enough to treat various cavity-QED effects, such as the Purcell effect, on-resonant or off-resonant cavity-enhanced Raman scattering, and vacuum-stimulated Raman adiabatic passage. For typical optical systems, we additionally take into account a ``reexcitation'' process, where the atom is reexcited after its decay to the initial ground state.
We study the dynamics of a spin ensemble strongly coupled to a single-mode resonator driven by external pulses. When the mean frequency of the spin ensemble is in resonance with the cavity mode, damped Rabi oscillations are found between the spin ensemble and the cavity mode which we describe very accurately, including the dephasing effect of the inhomogeneous spin broadening. We demonstrate that a precise knowledge of this broadening is crucial both for a qualitative and a quantitative understanding of the temporal spin-cavity dynamics. On this basis we show that coherent oscillations between the spin ensemble and the cavity can be enhanced by a few orders of magnitude, when driving the system with pulses that match special resonance conditions. Our theoretical approach is tested successfully with an experiment based on an ensemble of negatively charged nitrogen-vacancy centers in diamond strongly coupled to a superconducting coplanar single-mode waveguide resonator.
We describe a multi-mode quantum memory for propagating microwave photons that combines a solid-state spin ensemble resonantly coupled to a frequency tunable single-mode microwave cavity. We first show that high efficiency mapping of the quantum state transported by a free photon to the spin ensemble is possible both for strong and weak coupling between the cavity mode and the spin ensemble. We also show that even in the weak coupling limit unit efficiency and faithful retrieval can be obtained through time reversal inhomogeneous dephasing based on spin echo techniques. This is possible provided that the cavity containing the spin ensemble and the transmission line are impedance matched. We finally discuss the prospects for an experimental implementation using a rare-earth doped crystal coupled to a superconducting resonator.
We describe a multi-mode quantum memory for propagating microwave photons that combines a solid-state spin ensemble resonantly coupled to a frequency tunable single-mode microwave cavity. We first show that high efficiency mapping of the quantum state transported by a free photon to the spin ensemble is possible both for strong and weak coupling between the cavity mode and the spin ensemble. We also show that even in the weak coupling limit unit efficiency and faithful retrieval can be obtained through time reversal inhomogeneous dephasing based on spin echo techniques. This is possible provided that the cavity containing the spin ensemble and the transmission line are impedance matched. We finally discuss the prospects for an experimental implementation using a rare-earth doped crystal coupled to a superconducting resonator.