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arXiv:2312.16101 · Nature Nanotechnology

Universal control of four singlet–triplet qubits

Xin Zhang, Elizaveta Morozova, Maximilian Rimbach-Russ, Daniel Jirovec, Tzu-Kan Hsiao, Pablo Cova Fariña, Chien-An Wang, Stefan D. Oosterhout, Amir Sammak, Giordano Scappucci, Menno Veldhorst, Lieven M. K. Vandersypen

Published Oct 31, 2024• 50 citations
arXivHTMLPDF

Abstract

The coherent control of interacting spins in semiconductor quantum dots is of strong interest for quantum information processing and for studying quantum magnetism from the bottom up. Here we present a 2 × 4 germanium quantum dot array with full and controllable interactions between nearest-neighbour spins. As a demonstration of the level of control, we define four singlet-triplet qubits in this system and show two-axis single-qubit control of each qubit and SWAP-style two-qubit gates between all neighbouring qubit pairs, yielding average single-qubit gate fidelities of 99.49(8)-99.84(1)% and Bell state fidelities of 73(1)-90(1)%. Combining these operations, we experimentally implement a circuit designed to generate and distribute entanglement across the array. A remote Bell state with a fidelity of 75(2)% and concurrence of 22(4)% is achieved. These results highlight the potential of singlet-triplet qubits as a competing platform for quantum computing and indicate that scaling up the control of quantum dot spins in extended bilinear arrays can be feasible.

DOI
10.1038/s41565-024-01817-9

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Scientific Reports•Nov 1, 2013•10 citations
The coherent control of interacting spins in semiconductor quantum dots is of strong interest for quantum information processing and for studying quantum magnetism from the bottom up. Here we present a 2 × 4 germanium quantum dot array with full and controllable interactions between nearest-neighbour spins. As a demonstration of the level of control, we define four singlet-triplet qubits in this system and show two-axis single-qubit control of each qubit and SWAP-style two-qubit gates between all neighbouring qubit pairs, yielding average single-qubit gate fidelities of 99.49(8)-99.84(1)% and Bell state fidelities of 73(1)-90(1)%. Combining these operations, we experimentally implement a circuit designed to generate and distribute entanglement across the array. A remote Bell state with a fidelity of 75(2)% and concurrence of 22(4)% is achieved. These results highlight the potential of singlet-triplet qubits as a competing platform for quantum computing and indicate that scaling up the control of quantum dot spins in extended bilinear arrays can be feasible.
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
Singlet-triplet qubits offer an attractive encoding for semiconductor quantum computing, combining ancilla-free readout, reduced sensitivity to common-mode noise, and baseband voltage control. However, the Zeeman energy difference ΔEZΔE_\mathrm{Z}ΔEZ​ is typically fixed by local magnetic field gradients or ggg-factor inhomogeneities, leaving the exchange interaction JJJ as the only dynamically tunable parameter. This always-on ΔEZΔE_\mathrm{Z}ΔEZ​ precludes orthogonal control of the qubit's rotation axes and introduces unwanted state rotations during idling. Here we demonstrate all-electrical orthogonal control of a degenerate singlet-triplet (DST) qubit formed by two hole spins in a germanium double quantum dot. Exploiting the electrically tunable anisotropic ggg-factors of the two spins, we identify a regime where both ΔEZΔE_\mathrm{Z}ΔEZ​ and JJJ vanish, making the SSS and T0T_0T0​ states degenerate at the idle point. By applying only baseband voltage pulses, we independently control both JJJ and ΔEZΔE_\mathrm{Z}ΔEZ​, enabling fully orthogonal ZZZ- and XXX-axis rotations. Randomized benchmarking yields an average physical single-qubit gate fidelity of 99.53\% for a gate duration of approximately 100 ns. Finally, we electrically tune the degenerate point across a wide range of magnetic field orientations, enabling operation in a regime of enhanced coherence time and offering a route towards multi-qubit scaling under a shared global magnetic field.
The individual confinement and two-axis qubit operations of two-electron spin qubits in a GaAs gate-defined sextuple quantum dot array with an integrated micromagnet are reported in this study. As a first step toward multiple-qubit operations, we demonstrate coherent manipulations of three singlet-triplet qubits showing underdamped Larmor and Ramsey oscillations in all double dot sites. An accurate measurement of site-dependent field gradients as well as root-mean-squared electric and magnetic noise is provided, which is followed by a discussion of the adequacy of a simple rectangular micromagnet for practical use in multiple quantum dot arrays. Current limitations and possible strategies for achieving simultaneous multi-qubit operations in extended linear arrays are also presented.
Quantum dots can confine single electrons or holes to define spin qubits that can be operated with high fidelity. Experimental work has progressed from linear to two-dimensional arrays of quantum dots, enabling qubit interactions that are essential for quantum simulation and computation. Here, we explore architectures beyond planar geometries by constructing quantum dot arrays in three dimensions. We realize an eight-quantum dot system in a silicon-germanium heterostructure comprising two stacked germanium quantum wells, where quantum dots are positioned at the vertices of a cuboid. Using electrostatic gate control, we load a single hole into any of the eight quantum dots. To demonstrate the potential of multilayer quantum dot systems, we show coherent spin control and hopping-induced spin rotations by shuttling between the quantum wells. The ability to extend quantum dot arrays in three dimensions provides opportunities for novel quantum hardware and high-connectivity quantum circuits.
This thesis addresses the concept of quantum computing with semiconductor quantum dots. The basic unit of a quantum computer is a quantum mechanical two-level system, the so-called quantum bit (qubit). The qubit can be defined as the spin of an electron confined in a quantum dot or as a two-dimensional subspace of the Hilbert space for several spins. Some semiconductors have several minima in their conduction band, socalled valleys. A two-dimensional valley degree of freedom can also be considered as a qubit. In this thesis, quantum registers storing spin as well as valley qubits are described theoretically. Virtual hopping yields an exchange interaction between neighboring quantum dots, which reduces the energy of antisymmetric spin-valley states according to the Pauli principle. Considering the spin and the valley degrees of freedom of two electrons in neighboring quantum dots as qubits, the exchange interaction is a four-qubit interaction. In this thesis, it will be shown that it is, nevertheless, possible to generate a universal two-qubit gate for spin qubits or for valley qubits by combining the exchange interaction and individual single-qubit gates. The exchange interaction in this two-electron double quantum dot directly provides a universal two-qubit gate for one spin and one valley qubit as well. For this, the qubits are defined as suitable subspaces, spanned by the singlet and one triplet state of the spin and the valley states, respectively, Using those gates, arbitrary quantum operations can be performed for single-spin and single-valley qubits in the same quantum register, where in one double quantum dot the quantum states are restricted to the singlet-triplet subspace. While in this register single-spin and single-valley rotations are required, these gates are dispensable in a quantum register storing spin and valley singlet-triplet qubits. The single-qubit operations, in this case, can be provided by the exchange interaction and a gradient in the energy splitting of spin and valley states when the spin qubit is stored in a double quantum dot with spin degrees of freedom only and when the spin states in the double quantum dot which stores the valley qubit are polarized. For providing the two-qubit gate, the spin and the valley qubits need to be stored in the same double quantum dot. The crucial task for this register is to interchange the spin of a spin-only and a spin-valley quantum dot in order to switch between the single-qubit and the two-qubit operation mode. This interchanging of the spin can be achieved by a valley-depending virtual hopping between the quantum dots. Furthermore, echo sequences for a so-called exchange-only qubit are considered. An exchange-only qubit is defined as a subspace in a system of three electron spins in a triple quantum dot. An inhomogeneous magnetic field, which may be caused by nuclear spins in the semiconductor, can lead to decoherence and leakage, i.e., the state might leave the qubit subspace. Suppressing this effect by an echo sequence which consists of pulses interchanging neighboring spin states, so-called SWAP gates, was proposed. Controllability over these quantum operations is provided via the exchange interaction. In this thesis, the performance of different such sequences is investigated. The analysis shows that optimization strategies developed for single spin echoes can be adapted for the three spin system. The echo sequences can be different in their order of applied SWAP gates interchanging the spins in the first and second dots or in the second and third dots. The noise suppression performance depends slightly on this order of SWAP gates. For two spins in a double quantum dot a scheme for quantum state tomography is presented. The corresponding measurement operators are constructed from a set of mutually unbiased bases of the four-dimensional two-qubit Hilbert space. These measurements are represented by short sequences of no more than three elementary quantum gates and projective measurements by the well-established spin-to-charge conversion.
A pair of self-assembled InGaAs quantum dots filled with two electrons can act as a singlet-triplet spin qubit that is robust against nuclear spin fluctuations as well as charge noise. This results in a T2* coherence time two orders of magnitude longer than that of a single electron, provided the qubit is operated at a particular "sweet spot" in gate voltage. However, at this fixed operating point the ground-state splitting can no longer be tuned into resonance with e.g. another qubit, limiting the options for coupling multiple qubits. Here, we propose using a four-electron coupled quantum dot to implement a singlet-triplet qubit that features a magnetically tunable level splitting. As a first step towards full experimental realization of this qubit design, we use optical spectroscopy to demonstrate the tunability of the four-electron singlet-triplet splitting in a moderate magnetic field.