A key set of observables for investigating quantum systems are the n -body correlation functions, which provide a powerful tool for experimentally determining coherence and directly probing the many-body wave function. While the (bosonic) correlations of photonic systems are well explored, the correlations present in matter-wave systems, particularly for fermionic atoms, are still an emerging field. In this work, we use the unique single-atom detection properties of He*3 atoms to perform simultaneous measurements of the n -body quantum correlations, up to the fifth order, of a degenerate Fermi gas. In a direct demonstration of the Pauli exclusion principle, we observe clear antibunching at all orders and find good agreement with predicted correlation volumes. Our results pave the way for using correlation functions to probe some of the rich physics associated with fermionic systems. Published by the American Physical Society 2024
A key set of observables for investigating quantum systems are the n -body correlation functions, which provide a powerful tool for experimentally determining coherence and directly probing the many-body wave function. While the (bosonic) correlations of photonic systems are well explored, the correlations present in matter-wave systems, particularly for fermionic atoms, are still an emerging field. In this work, we use the unique single-atom detection properties of He*3 atoms to perform simultaneous measurements of the n -body quantum correlations, up to the fifth order, of a degenerate Fermi gas. In a direct demonstration of the Pauli exclusion principle, we observe clear antibunching at all orders and find good agreement with predicted correlation volumes. Our results pave the way for using correlation functions to probe some of the rich physics associated with fermionic systems. Published by the American Physical Society 2024
This thesis presents two experiments on ultracold gases of metastable Helium that constitute the extension, to matter waves, of experiments that have been fundamental for the development of quantum optics. Both experiments have been realized by using a single atom detector, that allows one to reconstruct the position of the atoms in three dimensions. In the first experiment we directly compared the two-body correlation function for a cold cloud of identical fermions and for a cold cloud of identical bosons at the same temperature issued from the same experimental apparatus. Since bosons and fermions obey different quantum statistics, the two-body correlation functions are different: identical bosons tend to be detected bunched in pairs, while identical fermions tend to antibunch because of the Pauli exclusion principle. In the second experiment we studied the correlation between pairs of bosonic atoms generated in the collision of two Bose-Einstein condensates. The measurement of the correlation function allows us to demonstrate that atoms flying back to back in the centre of mass frame are correlated in pairs. Furthermore the observation of a Hanbury Brown Twiss correlation between atoms with collinear velocity demonstrates that our system cannot be interpreted in terms of classical mechanics, but that the bosonic statistics plays a crucial role. A new version of the experiment will allow us to measure the angular dependence of the population of the scattering modes and the number difference squeezing between two correlated modes.
The Pauli exclusion principle is a fundamental law underpinning the structure of matter. Because of their antisymmetric wave function, no two fermions can occupy the same quantum state. Here, we report on the direct observation of the Pauli principle in a continuous system of up to six particles in the ground state of a two-dimensional harmonic oscillator. To this end, we sample the full many-body wave function by applying a single atom resolved imaging scheme in momentum space. We find so-called Pauli crystals as a manifestation of higher order correlations. In contrast to true crystalline phases, these unique high-order density correlations emerge even without any interactions present. Our work lays the foundation for future studies of correlations in strongly interacting systems of many fermions.
The field of atom optics has progressed rapidly over the past 20 years since the realisation of Bose-Einstein condensation, such that the wave behaviour of atomic gases is now routinely demonstrated. Furthermore, the study of quantum atom optics, which goes beyond a ‘mean-field’ description of quantum systems to consider the behaviour of single particles, has demonstrated both the similarities between photons and massive species, and their differences as a result of the internal structure and external interactions of atoms. An important class of observable quantities which allow such effects to be measured are nth order correlation functions, which can be interpreted as a result of either particle or wave behaviour. These functions provide a statistical description of fluctuations in n-tuples of particles in a source, which rigorously defines concepts such as coherence. The quantum statistics of a Bose-Einstein condensate should be the same as that for an optical laser, while an ideal thermal Bose gas matches the behaviour of incoherent light. However, correlation measurements can also be used to quantify the influence of interactions, dimensionality, confining potentials and waveguides, and the difference in quantum statistics between fermions and bosons, which illustrates the rich range of behaviour exhibited by atomic gases. In this thesis, several aspects of quantum atom optics are explored with experiments using ultracold metastable helium, a species with the unique advantage of facilitating simple single-atom detection with high resolution, while still allowing Bose-Einstein condensates to be formed. The coherence of atomic systems is shown to be maintained when outcoupled as pulsed atom lasers, and the long-range order characteristic of Bose-Einstein condensates is demonstrated to third order for the first time. Conversely, thermal bunching is observed for a variety of atomic systems, including the measurement of correlation functions up to sixth order with near-ideal interference contrast. These results clearly demonstrate the correspondence between the quantum statistics of photons and atoms as was formalised by Glauber, as well as confirming the validity of applying Wick’s theorem to simplify the statistics of atomic gases. Correlation functions are also shown to be an ideal tool to probe the quantum state of an ultracold gas, and were used to observe the phenomenon of transverse condensation in an elongated Bose gas, as well as characterise the mode occupancy of matter waves guided by an optical potential. Ultracold metastable helium is also suitable for exploring other fundamental topics in quantum optics such particle/wave duality. The notion of complementarity stimulated long running philosophical discussions about how apparently mutually exclusive behaviours can coexist, which culminated in Wheeler devising his famous ‘delayed choice’ gedankenexperiment. A proposed experimental method to realise Wheeler’s experiment with ultracold atoms is discussed, and preliminary measurements presented which indicate that the completion of this experiment could be achieved in the near future. Not only is this of interest in its own right, but the implementation of this experiment has also developed techniques which may enable further studies in quantum atom optics such as investigations of the Hong-Ou-Mandel effect and quantum entanglement with massive particles.
Pauli's exclusion principle forces fermions to occupy distinct quantum states, creating a filled region of momentum space at low temperature, the Fermi sea, whose topology governs the system's response to perturbations and the nature of its correlation functions. Recent theory predicts that for non-interacting fermions, the Euler characteristic of a D-dimensional Fermi sea -- the topological invariant that describes its shape -- is encoded in its (D+1)-point density correlations. Here we experimentally demonstrate this connection in a two-dimensional degenerate gas of neutral 6Li atoms using single-atom-resolved imaging. By measuring three- and four-point connected density correlations in real space, we directly extract topological invariants of the underlying Fermi sea, including the Euler characteristic. Our results are in remarkable agreement with ideal-gas predictions, despite the presence of sizeable interactions, and establish a new pathway for probing many-body topology through correlation measurements.
Confined quantum systems involving N identical interacting fermions are found in many areas of physics, including condensed matter, atomic, nuclear, and chemical physics. In a previous series of papers, a many-body perturbation method that is applicable to both weakly and strongly interacting systems of bosons has been set forth by the author and coworkers. A symmetry-invariant perturbation theory was developed that uses group theory coupled with the dimension of space as the perturbation parameter to obtain an analytic correlated wave function through first order for a system under spherical confinement with a general two-body interaction. In the present paper, we extend this formalism to large systems of fermions, circumventing the numerical demands of applying the Pauli principle by enforcing the Pauli principle on paper. The method does not scale in complexity with N and has minimal numerical cost. We apply the method to a unitary Fermi gas and compare to recent Monte Carlo values.
Abstract The measurement and characterisation of correlation functions has recently become one of the central themes in the studies of ultracold quantum gases. By probing complex many-body states of these interacting systems, correlation functions facilitate the most in-depth understanding of the underlying physics, not accessible through simple density profile measurements. In this thesis, we study the dynamics of second-order correlation functions for atoms created in pair-production processes such as molecular dissociation and atomic four-wave mixing. More specifically, in Chapter 3 we analyse the dynamics of correlated atom pairs created via controlled dissociation of a Bose-Einstein condensate of diatomic molecules. The atomic constituents can be either a pair of bosonic or fermionic atoms. The process provides a matter-wave analog of parametric down-conversion with photons, which was pivotal in the advancement of quantum optics by enabling experimental
demonstrations of the famous Einstein-Podolsky-Rosen paradox and violations of a classical Bell inequality. The atom-optics analogues of parametric down-conversion make it possible to envisage similar demonstrations using ensembles of massive particles in quantum gas regimes. In the case of fermionic constituents, molecular dissociation offers the possibility of a new paradigm in fermionic quantum-atom optics. By aiming at experimentally realistic modelling, we examine the role of spatial inhomogeneity of harmonically trapped molecular condensates on the strength and the shape of atom-atom correlations. Using the undepleted molecular-field approximation, we obtain explicit analytic results for the short-time asymptotic behaviour of the second-order correlation functions and for relative number squeezing between the dissociated atoms in one, two, and three spatial dimensions. Comparisons with the numerical results, which incorporate the molecular depletion and s-wave scattering
interactions, show that the analytic approaches employed here capture the main underlying physics and provide useful insights into the dynamics of dissociation for conversion efficiencies up to 10%. The results show explicitly how the strength of atom-atom correlations and relative number squeezing degrade with the reduction of the size of the molecular condensate. In Chapter 4, we study highly anisotropic molecular condensates in order to quantify the effects of bosonic stimulation and fermionic Pauli blocking on the dissociation dynamics. We show that the difference in quantum statistics of the atomic constituent is manifest as complementary geometric structures in the density profiles of the dissociated atoms. Atomic bosons are preferentially emitted along the long axis of the molecular condensate due to bosonic stimulation, while atomic fermions are preferentially emitted along the short axis due to Pauli blocking. This anisotropy potentially simplifies the measurement of
correlations between the atoms through relative number squeezing. In Chapter 5 we apply our analytic approaches to a related problem of atomic four-wave mixing and analyze atom-atom correlations in the s-wave scattering halo of two colliding condensates. The results in the short-time limit are in agreement with the first-principles simulations using the positive-P representation and provide analytic insights into the experimental observations of Perrin et al. [Phys. Rev. Lett. 99, 150405 2007]. The final chapter of the thesis, Chapter 6, is devoted to the first application of the Gaussian fermionic phase-space method to a dynamical simulation of a multimode fermion-boson system. As a first-principles approach, the method provides benchmarking of approximate approaches and can be used to validate dynamical probes for characterizing strongly correlated phases of fermionic systems. We have applied the Gaussian phase-space method to the problem of molecular dissociation in the simplest
uniform case and demonstrated a successful treatment of large molecular condensates containing up to 10^4 molecules and 10^3 distinct atomic modes. Simulating a system in such a large Hilbert space would be impossible using a more traditional exact numerical method based on the number-state representation. Our simulations reveal, in the long-time limit, significant deviations of atom-molecule and molecule-molecule correlations from the predictions of approximate pairing mean-field theories, as well as significant departures of atom-atom correlations from Wick's factorisation scheme. We have examined the accuracy and limitations of the fermionic phase-space results by comparison with the number-state calculations for small-size systems and via the analysis of conserved quantities. Future extensions of this work will have to incorporate spatial inhomogeneity and s-wave scattering interactions in order to enable first-principles dynamical simulations of a broader class of fermionic
systems of current experimental interest. To this end, we have implemented a phase-space treatment of the Fermi-Hubbard model and present some exploratory simulations of Hubbard dynamics.