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arXiv:2311.08641 · Physical Review Research

Fundamental limits to the generation of highly displaced bright squeezed light using linear optics and parametric amplifiers

Steve M. Young, Daniel Soh

Published Feb 3, 2025• 2 citations
arXivHTMLPDF

Abstract

High-quality squeezed light is an important resource for a variety of applications. Multiple methods for generating squeezed light are known, having been demonstrated theoretically and experimentally. However, the effectiveness of these methods—in particular, the inherent limitations to the signals that can be produced—has received little consideration. Here we present a comparative theoretical analysis for generating a highly displaced squeezed light from a linear optical method—a beamsplitter mixing a squeezed vacuum and a strong coherent state—and well-studied parametric amplification methods including an optical parametric oscillator, an optical parametric amplifier, and a dissipative optomechanical squeezer seeded with coherent states. We show that the quality of highly displaced squeezed states that can be generated using these methods is limited on a fundamental level by the physical mechanism utilized; across all methods there are significant trade-offs between displacement, squeezing, and overall uncertainty. We explore the nature and extent of these trade-offs specific to each mechanism and identify the optimal operation modes for each. Finally, we identify the conditions for minimum-uncertainty squeezing in arbitrary parametric amplifying systems and show that displacing the output signal will in general violate these conditions, adding noise and degrading squeezing.

DOI
10.1103/physrevresearch.7.013130

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High-quality squeezed light is an important resource for a variety of applications. Multiple methods for generating squeezed light are known, having been demonstrated theoretically and experimentally. However, the effectiveness of these methods—in particular, the inherent limitations to the signals that can be produced—has received little consideration. Here we present a comparative theoretical analysis for generating a highly displaced squeezed light from a linear optical method—a beamsplitter mixing a squeezed vacuum and a strong coherent state—and well-studied parametric amplification methods including an optical parametric oscillator, an optical parametric amplifier, and a dissipative optomechanical squeezer seeded with coherent states. We show that the quality of highly displaced squeezed states that can be generated using these methods is limited on a fundamental level by the physical mechanism utilized; across all methods there are significant trade-offs between displacement, squeezing, and overall uncertainty. We explore the nature and extent of these trade-offs specific to each mechanism and identify the optimal operation modes for each. Finally, we identify the conditions for minimum-uncertainty squeezing in arbitrary parametric amplifying systems and show that displacing the output signal will in general violate these conditions, adding noise and degrading squeezing.
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We perform a theoretical analysis of steady-state solutions and quantum noise in a below-threshold optical parametric oscillator (OPO) operating as an amplifier with an input seed wave. Both the amplitude-squeezed and phase-squeezed states of the output field are considered. We take into account the intracavity nonlinear losses due to intracavity frequency doubling of the signal wave and the quantum fluctuations of the seed and pump waves. Unlike the preceding theoretical studies of the problem, we show that squeezing in bright beams produced by the OPO depends on their intensity. For the amplitude-squeezed state, squeezing strongly degrades with increasing output intensity. In contrast, one can obtain good squeezing for phase-squeezed beams of high output intensity.
This thesis is primarily a theoretical study of degenerate parametric amplification as a means of generating squeezed-state light. i) A wideband traveling-wave formalism is developed for analyzing quantum mechanically a degenerate parametric amplifier. The formalism is based on spatial differential equations — spatial Langevin equations — that propagate temporal Fourier components of the field through the nonlinear medium. In addition to the parametric nonlinearity, the Langevin equations include absorption and associated fluctuations, dispersion, and pump quantum fluctuations. The dominant effects of dispersion and pump quantum fluctuations on the squeezing produced by a degenerate parametric amplifier are analyzed. ii) The wideband formalism of i) is used to carry out a more detailed analysis of the effects of phase mismatching. With the assumption of a lossless medium and a classical pump, we find that parametric amplification is capable of generating squeezed-state light over a wide band if materials with large χ(2) nonlinearities can be found, and that the squeezing bandwidth can be enhanced by phase mismatching away from degeneracy. iii) We consider again the effect of pump quantum fluctuations on the squeezing produced by parametric amplification. We perform discrete-mode calculations for a parametric amplifier with a quantum pump, and discuss some of the limitations of calculations of this sort in quantum optics. We derive stochastic differential equations (SDEs) for one- and two-mode parametric amplifiers, and from them obtain an iterative solution showing that pump quantum fluctuations impose a limitation on the degree of squeezing obtainable from a parametric amplifier. iv) A possible application of squeezing is considered; in particular, we study the effects of squeezing the intracavity noise in a laser oscillator. We solve the classical noise problem of a realistic laser model by making a bold — and possibly unrealizable — assumption, that the in-phase and quadrature Langevin sources which are responsible for the "noisiness" of the laser can be squeezed. We show that the effect of squeezing the in-phase quadrature is to reduce the phase noise, including the linewidth, of the laser but, due to amplitude-phase coupling, not to eliminate them altogether.
Squeezed states of light enable enhanced measurement precision by reducing noise below the standard quantum limit. A key application of squeezed light is nonlinear microscopy, where state-of-the-art performance is limited by photodamage and quantum-limited noise. Such microscopes require bright, pulsed light for optimal operation, yet generating and detecting bright pulsed squeezing at high levels remains challenging. In this work, we present an efficient technique to generate high levels of bright picosecond pulsed squeezed light using a χ2χ^2χ2 optical parametric amplification process in a waveguide. We measure −3.2 dB-3.2~\mathrm{dB}−3.2 dB of bright squeezing with optical power compatible with nonlinear microscopy, as well as −3.6 dB-3.6~\mathrm{dB}−3.6 dB of vacuum squeezing. Corrected for losses, these squeezing levels correspond to −15.4−8.7+2.7 dB-15.4^{+2.7}_{-8.7}~\mathrm{dB}−15.4−8.7+2.7​ dB of squeezing generated in the waveguide. The measured level of bright amplitude pulsed squeezing is to our knowledge the highest reported to date, and will contribute to the broader adoption of quantum-enhanced nonlinear microscopy in biological studies.
The minimum resolvable signal in optical metrology and sensing applications is usually limited by the so-called standard quantum limit. One way to improve the signal-to-noise ratio is to use squeezed states of light. Squeezed light can be generated using different types of nonlinear interactions either in solid-state nonlinear crystals or in atomic systems. One way to generate squeezed light is to use a phase sensitive amplifier that will amplify one quadrature of the considered mode and deamplify the other one. We have recently shown that metastable helium vapor at room temperature can exhibit strong four-wave mixing effects and behave like a perfect phase sensitive amplifier when it is prepared in coherent population trapping situation. In this talk, we will present the application of this phase sensitive amplification to the generation of squeezed vacuum states of light and detail the performances and limitations of the system