Controlling the frequency of nonclassical light is indispensable for implementing quantum computation, communication and bridging various quantum systems. However, frequency-shift devices for solid state single-photon sources that are easy to integrate are practically absent. Here, we propose an integrated single-photon frequency shifter based on acousto-optic modulation. The device consists of two Interdigital Transducers (IDTs) for surface acoustic wave (SAW) generation and a silicon waveguide periodically placed at the nodes the SAW to increase the interaction length. The Vπ*L of the device is 1.2v.cm. Under 133.2MHz driving frequency and 10 volt driving voltage, a shift up to 65.7GHz is achieved with near unity conversion efficiency. Our results demonstrate the feasibility of on-chip deterministic quantum spectral control in constructing hybrid quantum networks.
Controlling the frequency of nonclassical light is indispensable for implementing quantum computation, communication and bridging various quantum systems. However, frequency-shift devices for solid state single-photon sources that are easy to integrate are practically absent. Here, we propose an integrated single-photon frequency shifter based on acousto-optic modulation. The device consists of two Interdigital Transducers (IDTs) for surface acoustic wave (SAW) generation and a silicon waveguide periodically placed at the nodes the SAW to increase the interaction length. The Vπ*L of the device is 1.2v.cm. Under 133.2MHz driving frequency and 10 volt driving voltage, a shift up to 65.7GHz is achieved with near unity conversion efficiency. Our results demonstrate the feasibility of on-chip deterministic quantum spectral control in constructing hybrid quantum networks.
We propose a single optical photon source for quantum cryptography based on the acoustoelectric effect. Surface acoustic waves (SAWs) propagating through a quasi-one-dimensional channel have been shown to produce packets of electrons that reside in the SAW minima and travel at the velocity of sound. In our scheme, the electron packets are injected into a p-type region, resulting in photon emission. Since the number of electrons in each packet can be controlled down to a single electron, a stream of single- (or N-) photon states, with a creation time strongly correlated with the driving acoustic field, should be generated.
Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (±641 GHz or ±5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
Scaling quantum control for atoms, ions, and solid-state emitters requires gigahertz-frequency spectral control of high-power visible light in a volume-manufacturable platform. Silicon nitride photonics provides high power handling and CMOS-foundry compatibility but has no intrinsic mechanism for high-speed modulation. Integration with piezoelectric materials enables acousto-optic phase modulation, and mechanical resonant enhancement has made it efficient at gigahertz frequencies. However, a single resonance restricts the modulation waveform to a single tone, imposing Bessel-function sideband amplitudes and limiting frequency-shifting efficiency to 33.9%. Here we engineer a silicon nitride acousto-optic microstructure to support harmonically spaced resonances at 1.14 GHz and 2.28 GHz, each strongly optomechanically coupled to a 730 nm guided optical mode, so that tailored non-sinusoidal modulation waveforms can be resonantly synthesized. By piezoelectrically controlling the two mechanical amplitudes and their relative phase, we demonstrate 50% conversion to one sideband (1.5x the single-tone theoretical maximum), a flat seven-line comb, and a frequency shift with 60 dB carrier and 53 dB image suppression - to our knowledge the highest reported for an integrated modulator. The devices are fabricated in a 200 mm CMOS foundry, and we measure 91.7% yield without post-fabrication tuning across 36 devices from three wafers. We also show how the technique can be straightforwardly scaled to three or more harmonics. This result overcomes the trade-off between resonant enhancement and spectral programmability, with important consequences including improved single-qubit gate efficiency for hyperfine qubits.
Abstract Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of nonclassical light using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (± 641 GHz or ± 5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
This thesis presents work on a series of devices for the generation of photonic quantum states based on self-assembled InAs quantum dots, which are among the most technologically mature candidates for practical quantum photonic applications due to their high internal quantum efficiency, narrow linewidth, tunability and straightforward integration with photonic and electric components. The primary results presented concern sources of multi-photon entangled states and single-photon sources with high repetition rate, both of which are crucial components for emerging photonic quantum technologies. First, we propose a scheme for the sequential generation of entangled photon chains by resonant scattering of a laser field on a single charged particle in a cavity-enhanced quantum dot. The charge has an associated spin that can determine the time bin of a photon, allowing for information encoding in this degree of freedom. We demonstrate coherent operations on this spin and realize a proof-of-principle experiment of the proposed scheme by showing that the time bin of a single-photon is dependent on the measured state of the trapped spin. The second main avenue of work investigates the effects of a surface acoustic wave, a mechanical displacement wave confined to the surface of a substrate, on the optical properties of quantum dots. In particular, we exploit the dynamic acoustically-induced tuning of the emission energy to modulate the Purcell effect in a pillar microcavity. Under resonant optical excitation we demonstrate the conversion of the continuous wave laser into a pulsed single-photon stream inheriting the acoustic frequency of 1 GHz as the repetition rate. High resolution spectroscopy reveals the presence of narrow sidebands in the emission spectrum, whose relative intensity can be controlled by the acoustic power and laser detuning. Furthermore, we develop a platform for analogous in-plane experiments by transferring GaAs membranes hosting quantum dots onto LiNbO3 substrates and patterning them into whispering gallery mode optical resonators. In addition to Purcell enhancement and acoustic tuning of the emission, the devices exhibit strong localized mechanical resonances. Finally, we perform initial experiments on the effects of a surface acoustic wave on the spin of a charge trapped in a quantum dot. We integrate acoustic transducers with charge-tunable diodes, where the charge state of the dot can be precisely controlled by an applied bias voltage, and demonstrate the frustration of optical spin pumping by the acoustic wave.
Fast, efficient, and low power modulation of light at microwave frequencies is crucial for chip-scale classical and quantum processing as well as for long-range networks of superconducting quantum processors. A successful approach to bridge the gap between microwave and optical photons has been to use intermediate platforms such as acoustic waves, which can couple efficiently to a variety of quantum systems. Here, we use gigahertz-frequency focusing surface acoustic wave cavities on GaAs that are piezo-electrically coupled to superconducting circuits and parametrically coupled, via strain, to photons scattered from InAs quantum dots . We demonstrate strong modulation of single photons with a half-wave voltage as low as 44 mV, and subnatural modulation sideband linewidths. These demonstrations pave the way for efficient and low-noise transduction of quantum information between microwave and optical domains.