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arXiv:2310.16930 · Nature Communications

Spin-photon entanglement with direct photon emission in the telecom C-band

Petros Laccotripes, Tina Müller, R. M. Stevenson, J. Skiba-Szymanska, D. A. Ritchie, A. J. Shields

Published Nov 11, 2024• 28 citations
arXivHTMLPDF

Abstract

Quantum networks, relying on the distribution of quantum entanglement between remote locations, have the potential to transform quantum computation and secure long-distance quantum communication. However, a fundamental ingredient for fibre-based implementations of such networks, namely entanglement between a single spin and a photon directly emitted at telecom wavelengths, has been unattainable so far. Here, we use a negatively charged exciton in an InAs/InP quantum dot to implement an optically active spin qubit taking advantage of the lowest-loss transmission window, the telecom C-band. We investigate the coherent interactions of the spin-qubit system under resonant excitation, demonstrating high fidelity spin initialisation and coherent control using picosecond pulses. We further use these tools to measure the coherence of a single, undisturbed electron spin in our system. Finally, we demonstrate spin-photon entanglement in a solid-state system with entanglement fidelity F = 80.07 ± 2.9%, more than 10 standard deviations above the classical limit.

DOI
10.1038/s41467-024-53964-1

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Quantum networks, relying on the distribution of quantum entanglement between remote locations, have the potential to transform quantum computation and secure long-distance quantum communication. However, a fundamental ingredient for fibre-based implementations of such networks, namely entanglement between a single spin and a photon directly emitted at telecom wavelengths, has been unattainable so far. Here, we use a negatively charged exciton in an InAs/InP quantum dot to implement an optically active spin qubit taking advantage of the lowest-loss transmission window, the telecom C-band. We investigate the coherent interactions of the spin-qubit system under resonant excitation, demonstrating high fidelity spin initialisation and coherent control using picosecond pulses. We further use these tools to measure the coherence of a single, undisturbed electron spin in our system. Finally, we demonstrate spin-photon entanglement in a solid-state system with entanglement fidelity F = 80.07 ± 2.9%, more than 10 standard deviations above the classical limit.
Efficient generation of entanglement between a stationary matter-qubit and a propagating photonic-qubit is a scientific and technological challenge of utmost importance for the realisation of fully-fledged quantum networks. Solid-state quantum emitters in the telecom C-band are a promising platform due to the minimal absorption of photons at these wavelengths and deterministic generation of high purity single photon flying qubits. Here, we use an InAs/InP quantum dot to implement an optically active spin-qubit and demonstrate high fidelity spin initialisation and coherent spin control of the resident electron. Lastly, for the first time we demonstrate high-fidelity spin-photon entanglement in a solid-state system with direct emission into the telecom C-band and obtain a lower bound on the entanglement fidelity of 80.07 %.
Multiphoton entangled states are a key resource for quantum networks and measurement-based quantum computation. Scalable protocols for generating such states using solid-state spin-photon interfaces have recently emerged, but practical implementations have so far relied on emitters operating at short wavelengths, incompatible with low-loss fibre transmission. Here, we take a key step towards the generation of telecom wavelength multi-qubit entangled states using an InAs/InP quantum dot. After establishing that all essential criteria for generating cluster states using a ground state spin as the entangler are satisfied, we implement a scalable protocol to entangle the resident spin with sequentially emitted photons directly in the telecom C-band. We demonstrate a two-qubit (spin-photon) entanglement fidelity of 59.5±8.7%59.5\pm 8.7\%59.5±8.7% and a lower bound of three-qubit (spin-photon-photon) entanglement fidelity of 52.7±11.4%52.7\pm 11.4\%52.7±11.4%. Our results close the performance gap between short-wavelength quantum dot systems and the existing telecom infrastructure, establishing a route towards practical large photonic cluster states for fibre-based quantum network applications.
Quantum nonlocality, typically revealed through entanglement distribution across quantum networks, is a cornerstone of quantum information science. Long-distance distribution of entanglement requires the information carrier, i.e. flying photons, to operate in the minimum-loss telecom band of optical fiber. While extensive efforts have been devoted to the direct generation of entanglement between C-band telecom photons and various stationary spins, the verification of quantum nonlocality remains an outstanding challenge. Here, utilizing a dipole transition in rubidium atoms with a wavelength of 1530 nm and a cavity-assisted protocol, we achieve resonant excitation and direct emission of C-band telecom photons from a single atom, generating spin-photon entanglement with a measured Bell state fidelity exceeding 91.4%. We then verify Bell nonlocality by observing a Bell inequality violation of 2.455(77) > 2 using this high-quality entangled pair. These results extend the wavelength of a single-atom quantum emitter to the telecom C-band, achieving sufficiently high-fidelity spin-photon entanglement to finally verify Bell nonlocality. This work thereby provides a promising building block for a large-scale atom-based quantum network capable of distributed quantum metrology and long-distance quantum communication.
A practical way to link separate nodes in quantum networks is to send photons over the standard telecom fibre network. This requires sub-Poissonian photon sources in the telecom wavelength band around 1550 nm, where the photon coherence time has to be sufficient to enable the many interference-based technologies at the heart of quantum networks. Here, we show that droplet epitaxy InAs/InP quantum dots emitting in the telecom C-band can provide photons with coherence times exceeding 1 ns even under non-resonant excitation, more than a factor two longer than values reported for shorter wavelength quantum dots under similar conditions. We demonstrate that these coherence times enable near-optimal interference with a C-band laser qubit, with visibilities only limited by the quantum dot multiphoton emission. Using entangled photons, we further show teleportation of such qubits in six different bases with average fidelity reaching 88.3$\pm$4%. Beyond direct applications in long-distance quantum communication, the high degree of coherence in these quantum dots is promising for future spin based telecom quantum network applications.
Abstract A practical way to link separate nodes in quantum networks is to send photons over the standard telecom fibre network. This requires sub-Poissonian photon sources in the wavelength band around 1550 nm, with photon coherence times sufficient to enable the many interference-based technologies at the heart of quantum networks. Here, we show that droplet epitaxy InAs/InP quantum dots emitting in the telecom C-band can provide photons with coherence times exceeding 1 ns under low power non-resonant excitation, and demonstrate that these coherence times enable near-optimal interference with a C-band polarisation-encoded laser qubit, with visibilities only limited by the quantum dot multiphoton emission. Using entangled photons, we further show teleportation of such qubits in six different bases with average postselected fidelity reaching 88.3 ± 4.0%. Beyond direct applications in long-distance quantum communication, the high degree of coherence in these quantum dots is promising for future spin-based telecom quantum network applications.