In open quantum systems, dissipative phase transitions (DPTs) emerge from the interplay between unitary evolution, drive, and dissipation. While second-order DPTs have been predominantly investigated theoretically, first-order DPTs have been observed in single-photon-driven Kerr resonators. We present here an experimental and theoretical analysis of both first and second-order DPTs in a two-photon-driven superconducting Kerr resonator. We characterize the steady state at the critical points, showing squeezing below vacuum and the coexistence of phases with different photon numbers. Through time resolved measurements, we study the dynamics across the critical points and observe hysteresis cycles at the first-order DPT and spontaneous symmetry breaking at the second-order DPT. Extracting the timescales of the critical phenomena reveals slowing down across five orders of magnitude when scaling towards the thermodynamic limit. Our results showcase the engineering of criticality in superconducting circuits, advancing the use of parametric resonators for critically-enhanced quantum information applications.
In open quantum systems, dissipative phase transitions (DPTs) emerge from the interplay between unitary evolution, drive, and dissipation. While second-order DPTs have been predominantly investigated theoretically, first-order DPTs have been observed in single-photon-driven Kerr resonators. We present here an experimental and theoretical analysis of both first and second-order DPTs in a two-photon-driven superconducting Kerr resonator. We characterize the steady state at the critical points, showing squeezing below vacuum and the coexistence of phases with different photon numbers. Through time resolved measurements, we study the dynamics across the critical points and observe hysteresis cycles at the first-order DPT and spontaneous symmetry breaking at the second-order DPT. Extracting the timescales of the critical phenomena reveals slowing down across five orders of magnitude when scaling towards the thermodynamic limit. Our results showcase the engineering of criticality in superconducting circuits, advancing the use of parametric resonators for critically-enhanced quantum information applications.
We investigate and characterize the emergence of finite-component dissipative phase transitions (DPTs) in nonlinear photon resonators subject to n -photon driving and dissipation. Exploiting a semiclassical approach, we derive general results on the occurrence of second-order DPTs in this class of systems. We show that for all odd n , no second-order DPT can occur while, for even n , the competition between higher-order nonlinearities determines the nature of the criticality and allows for second-order DPTs to emerge only for n = 2 and n = 4 . As pivotal examples, we study the full quantum dynamics of three- and four-photon driven-dissipative Kerr resonators, confirming the prediction of the semiclassical analysis on the nature of the transitions. The stability of the vacuum and the typical timescales needed to access the different phases are also discussed. We also show a first-order DPT where multiple solutions emerge around zero, low, and high-photon numbers. Our results highlight the crucial role played by s t r o n g and w e a k symmetries in triggering critical behaviors, providing a Liouvillian framework to study the effects of high-order nonlinear processes in driven-dissipative systems, that can be applied to problems in quantum sensing and information processing.
Josephson junctions are a fundamental building block of superconducting quantum circuits. They provide the nonlinearity required to realize quantum bits and enable a wide range of nonlinear phenomena central to quantum technologies. This thesis explores two superconducting systems in which this nonlinearity plays a central role. In the first part, we investigate a superconducting resonator terminated by a superconducting quantum interference device (SQUID), an arrangement of two Josephson junctions connected in parallel. The SQUID provides a tunable Kerr nonlinearity and allows the resonator to be driven parametrically. Under the combined action of the parametric drive, Kerr nonlinearity, and dissipation to the environment, the state of the resonator can undergo abrupt changes as the pump frequency or amplitude is varied. We interpret these changes within the framework of dissipative phase transitions (DPTs). By implementing a finite-component thermodynamic limit, we experimentally and theoretically investigate both first- and second-order DPTs in this system. We characterize their steady-state and dynamical signatures, including squeezing below vacuum, phase coexistence, hysteresis, spontaneous symmetry breaking, and critical slowing down. Finally, we exploit the enhanced susceptibility near the second-order critical point to implement a frequency-estimation protocol. We show that the estimation precision scales quadratically with the effective system size, demonstrating that finite-component DPTs can provide a quantum advantage in a sensing protocol. In the second part, we investigate a novel architecture for the readout of superconducting qubits. Conventional dispersive readout relies on a transverse interaction between a transmon and a resonator, which can lead to Purcell decay and measurement-induced state transitions, ultimately limiting the readout fidelity. To overcome these limitations, we implement a nonlinear coupling by galvanically connecting the transmon and resonator through a Josephson junction. This interaction provides a strong cross-Kerr coupling for clear state discrimination, but also introduces a detrimental transverse interaction. We experimentally show that the exchange part of the transverse interaction can be suppressed by adding a capacitor in parallel with the coupling junction while preserving the strong cross-Kerr coupling. In addition, we show that the same circuit acts as an intrinsic Purcell filter, protecting the qubit against Purcell decay. The coupling junction also induces a Kerr nonlinearity in the resonator, which we exploit to implement a bifurcation readout with a 99.4 % fidelity in a 68 ns integration time. This performance is achieved without a dedicated Purcell filter or a near-quantum-limited amplifier. Overall, this thesis demonstrates the engineering of nonlinear superconducting circuits to investigate dissipative phase transitions, exploit criticality for enhanced quantum sensing, and develop a novel qubit readout architecture enabling fast, high-fidelity measurement.
We investigate nonequilibrium criticality and chaos in a two-photon-driven optomechanical system. The parametric drive preserves a discrete Z2 symmetry of the optical field, while radiation-pressure coupling transfers the resulting nonlinear dynamics to a mechanical oscillator. Combining semiclassical stability analysis, exact Liouvillian spectra, and stochastic quantum trajectories, we show that this driven-dissipative optomechanical model supports both first- and second-order dissipative phase transitions. At negative detuning a second-order transition yields spontaneous breaking of the cavity-parity symmetry in the thermodynamic limit. At positive detuning the same symmetry breaking coexists with a first-order transition, signaled by metastability and by an additional symmetric Liouvillian mode. At stronger pump power the mean-field dynamics loses all stable fixed points and develops limit cycles and chaotic attractors with positive Lyapunov exponent. Quantum trajectories in this regime display chaotic-like motion, enhanced steady-state entropy, and delocalization over many entropic Liouvillian modes. These results establish two-photon-driven optomechanics as a platform where dissipative criticality, symmetry breaking, and quantum signatures of chaos emerge within the same experimentally accessible setting.
Dissipative phase transitions (DPTs) are traditionally characterized through the spectrum of a time-independent Liouvillian superoperator. However, this definition does not apply to time-periodic (Floquet) systems that cannot be exactly recast as time-independent problems. Here, we develop a general framework to characterize DPTs in time-periodic open quantum systems through the spectrum of the Floquet propagator. We first study driven-dissipative Kerr resonators, known to display a DPT, showing that counter-rotating terms in the drive shift the critical point and significantly change the time scales associated with the transition. We then investigate DPTs in the driven quantum Rabi model and its time-independent approximation, the driven Jaynes-Cummings model, finding that the Rabi model exhibits distinct critical features as the ultrastrong coupling regime is approached. Moreover, our Floquet analysis unveils the disappearance of the DPT in the deep strong coupling regime, due to light-matter decoupling. Our approach sets the stage for the study of dissipative criticality in a broad class of time-dependent open quantum systems.
Nonequilibrium phase transitions exist in damped-driven open quantum systems when the continuous tuning of an external parameter leads to a transition between two robust steady states.In second-order transitions this change is abrupt at a critical point, whereas in first-order transitions the two phases can coexist in a critical hysteresis domain.Here, we report the observation of a first-order dissipative quantum phase transition in a driven circuit quantum electrodynamics system.It takes place when the photon blockade of the driven cavity-atom system is broken by increasing the drive power.The observed experimental signature is a bimodal phase space distribution with varying weights controlled by the drive strength.Our measurements show an improved stabilization of the classical attractors up to the millisecond range when the size of the quantum system is increased from one to three artificial atoms.The formation of such robust pointer states could be used for new quantum measurement schemes or to investigate multiphoton phases of finite-size, nonlinear, open quantum systems.
We study a dissipative Kerr resonator subject to both single- and two-photon detuned drives. Beyond a critical detuning threshold, the Kerr resonator exhibits a semiclassical first-order dissipative phase transition between two different steady states that are characterized by a π phase switch of the cavity field. This transition is shown to persist deep into the quantum limit of low photon numbers. Remarkably, the detuning frequency at which this transition occurs depends almost linearly on the amplitude of the single-photon drive. Based on this phase-switching feature, we devise a sensitive quantum transducer that translates the observed frequency of the parametric quantum phase transition to the detected single-photon amplitude signal. The effects of noise and temperature on the corresponding sensing protocol are addressed, and a realistic circuit-QED implementation is discussed.